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Optical spectroscopy of molecular radicals is an important tool in physical chemistry, and is a prerequisite for many experiments which use molecules for quantum science and precision measurement. However, even the simplest molecules have…

Chemical Physics · Physics 2025-05-07 Ashay N. Patel , Madison I. Howard , Timothy C. Steimle , Nicholas R. Hutzler

Microcombs - optical frequency combs generated in microresonators - have advanced tremendously in the last decade, and are advantageous for applications in frequency metrology, navigation, spectroscopy, telecommunications, and microwave…

Mid-infrared optical frequency combs are of significant interest for molecular spectroscopy due to the large absorption of molecular vibrational modes on one hand, and the ability to implement superior comb-based spectroscopic modalities…

Optical detection of individual nanometer-sized analytes, virus particles, and protein molecules holds great promise for understanding and control of biological samples and healthcare applications. As fluorescent labels impose restrictions…

Optics · Physics 2020-10-19 Martin Dieter Baaske , Peter Sebastian Neu , Michel Orrit

Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…

Optics · Physics 2024-03-08 Bingxin Xu , Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Optical frequency combs are laser sources which are capable of generating discrete, equal-spaced and highly coherent comb modes. Optical frequency comb technique provides a significant bridge to transfer the stability between optical…

Optics · Physics 2022-04-14 Haochen Tian

Direct comb spectroscopy is a useful tool for obtaining highly accurate spectroscopic information. However, as the number of comb modes is very large and the optical energy is dispersed over them, the optical energy per each comb mode is…

Optical frequency combs consist of equally spaced discrete optical frequency components and are essential tools for optical communications and for precision metrology, timing and spectroscopy. To date, wide-spanning combs are most often…

Microwave photonic technologies, which upshift the carrier into the optical domain to facilitate the generation and processing of ultrawide-band electronic signals at vastly reduced fractional bandwidths, have the potential to achieve…

Optical frequency combs enable coherent data transmission on hundreds of wavelength channels and have the potential to revolutionize terabit communications. Generation of Kerr combs in nonlinear integrated microcavities represents a…

Optical frequency combs and their spectra of evenly spaced discrete laser lines are essential to modern time and frequency metrology. Recent advances in integrated photonic waveguides enable efficient nonlinear broadening of an initially…

It is shown that a highly equidistant optical frequency comb can be generated by the parametric excitation of an optical bottle microresonator with nanoscale effective radius variation by its natural mechanical vibrations.

Optics · Physics 2017-10-11 M. Sumetsky

Recent development in quantum photonics allowed to start the process of bringing photonic-quantum-based systems out of the lab into real world applications. As an example, devices for the exchange of a cryptographic key secured by the law…

Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs…

Pattern Formation and Solitons · Physics 2017-01-25 Adarsh Ganesan , Cuong Do , Ashwin A. Seshia

By continuous wave pumping of a dispersion engineered, planar silicon nitride microresonator, continuously circulating, sub-30fs short temporal dissipative solitons are generated, that correspond to pulses of 6 optical cycles and constitute…

Quantum frequency combs from chip-scale integrated sources are promising candidates for scalable and robust quantum information processing (QIP). However, to use these quantum combs for frequency domain QIP, demonstration of entanglement in…

We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Dissipative Kerr solitons (DKS) in optical microresonators provide a highly miniaturized, chip-scale frequency comb source with unprecedentedly high repetition rates and spectral bandwidth. To date, such soliton frequency comb sources have…

Optics · Physics 2019-01-09 Maxim Karpov , Martin H. P. Pfeiffer , Tobias J. Kippenberg