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We present LayerPCM, an extension of the polarizable-continuum model coupled to real-time time-dependent density-functional theory for an efficient and accurate description of the electrostatic interactions between molecules and…

Materials Science · Physics 2021-06-17 Jannis Krumland , Gabriel Gil , Stefano Corni , Caterina Cocchi

Coarse-grained molecular dynamics (CGMD) is a technique developed as a concurrent multiscale model that couples conventional molecular dynamics (MD) to a more coarse-grained description of the periphery. The coarse-grained regions are…

Materials Science · Physics 2009-11-11 Robert E. Rudd , Jeremy Q. Broughton

We report a Kelvin probe force microscopy (KPFM) implementation using the dissipation signal of a frequency modulation atomic force microscopy that is capable of detecting the gradient of electrostatic force rather than electrostatic force.…

Mesoscale and Nanoscale Physics · Physics 2017-04-21 Yoichi Miyahara , Peter Grutter

Since the invention of the atomic force microscope (AFM) in 1986, there has been a drive to apply this scanning probe technique or a form of this technique to various disciplines in nanoscale science. Magnetic force microscopy (MFM) is a…

Instrumentation and Detectors · Physics 2017-04-28 Gustavo Cordova , Brenda Yasie Lee , Zoya Leonenko

Imaging mechanisms in contact Kelvin Probe Force Microscopy (cKPFM) are explored via information theory-based methods. Gaussian Processes are used to achieve super-resolution in the cKPFM signal, effectively extrapolating across the spatial…

Primordial magnetic fields (PMF) can create polarization $B$-modes in the cosmic microwave background (CMB) through Faraday rotation (FR), leading to non-trivial 2-point and 4-point correlators of the CMB temperature and polarization. We…

Cosmology and Nongalactic Astrophysics · Physics 2013-05-30 Amit P. S. Yadav , Levon Pogosian , Tanmay Vachaspati

Coarse graining (CG) enables the investigation of molecular properties for larger systems and at longer timescales than the ones attainable at the atomistic resolution. Machine learning techniques have been recently proposed to learn CG…

Computational Physics · Physics 2022-09-28 Eleonora Ricci , George Giannakopoulos , Vangelis Karkaletsis , Doros N. Theodorou , Niki Vergadou

Piezoresponse force microscopy (PFM) is a powerful tool widely used to characterize piezoelectricity and ferroelectricity at the nanoscale. However, it is necessary to distinguish microscopic mechanisms between piezoelectricity and…

Materials Science · Physics 2018-04-26 Junxi Yu , Ehsan Nasr Esfahani , Qingfeng Zhu , Dongliang Shan , Tingting Jia , Shuhong Xie , Jiangyu Li

Fundamental mechanisms of energy storage, corrosion, sensing, and multiple biological functionalities are directly coupled to electrical processes and ionic dynamics at solid-liquid interfaces. In many cases, these processes are spatially…

Materials Science · Physics 2017-01-25 Liam Collins , Jason Kilpatrick , Sergei V. Kalinin , Brian J. Rodriguez

We present the design and experimental results of a near-field scanning microwave microscope (NSMM) working at a frequency of 1GHz. Our microscope is unique in that the sensing probe is separated from the excitation electrode to…

Materials Science · Physics 2009-11-13 K. Lai , M. B. Ji , N. Leindecker , M. A. Kelly , Z. X. Shen

Ferroelectric domain imaging with piezoresponse force microscopy (PFM) relies on the converse piezoelectric effect: a voltage applied to the sample leads to mechanical deformations. In case of PFM one electrode is realized by the tip,…

Materials Science · Physics 2015-06-25 T. Jungk , A. Hoffmann , E. Soergel

At first sight piezoresponse force microscopy (PFM) seems an ideal technique for the determination of piezoelectric coefficients (PCs), thus making use of its ultra-high vertical resolution (<0.1 pm/V). Christman et al. \cite{Chr98} first…

Materials Science · Physics 2009-11-13 T. Jungk , A. Hoffmann. , E. Soergel

Piezoresponse force microscopy (PFM) is a powerful characterization technique to readily image and manipulate ferroelectrics domains. PFM gives insight into the strength of local piezoelectric coupling as well as polarization direction…

The paper describes the peculiarities of acquirement and interpretation of images of current distribution through the sample surface when operating in I-AFM mode. It shows that I-AFM and SCM modes can be successfully used only for small…

Instrumentation and Detectors · Physics 2020-12-15 Olga V. Sviridova

A simple implementation of Kelvin probe force microscopy is reported that enables recording topographic images in the absence of any component of the electrostatic force. Our approach is based on a close loop z-spectroscopy operated in data…

Materials Science · Physics 2023-03-22 Aloïs Arrighi , Nathan Ullberg , Vincent Derycke , Benjamin Grévin

Four-dimensional scanning transmission electron microscopy (4D-STEM) provides rich, atomic-scale insights into materials structures. However, extracting specific physical properties - such as polarization directions essential for…

Photocurrent measurements provide a powerful means of studying the spatially resolved optoelectronic and electrical properties of a material or device. Generally speaking there are two classes of mechanism for photocurrent generation: those…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 Helin Cao , Grant Aivazian , Zaiyao Fei , Jason Ross , David H. Cobden , Xiaodong Xu

The mechanical, electrical and chemical properties of chemically modified graphene (CMG) are intrinsically linked to its structure. Here we report on our study of the topographic structure of free-standing CMG using atomic force microscopy…

Mesoscale and Nanoscale Physics · Physics 2011-04-12 N R Wilson , P A Pandey , R Beanland , J P Rourke , U Lupo , G Rowlands , R A Römer

The behavior of ferroelectricity at the nanoscale is the focus of increasing research activity because of intense interest in the fundamental nature of spontaneous order in condensed-matter systems and because of the many practical…

Near-field optical microscopy by means of infrared photocurrent mapping has rapidly developed in recent years. In this letter we introduce a near-field induced contrast mechanism arising when a conducting surface, exhibiting a magnetic…

Mesoscale and Nanoscale Physics · Physics 2019-02-13 E. Pfitzner , X. Hu , H. W. Schumacher , A. Hoehl , D. Venkateshvaran , M. Cubukcu , J. -W. Liao , S. Auffret , J. Heberle , J. Wunderlich , B. Kaestner