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We investigate the phases of two-dimensional electron-hole systems strongly coupled to a microcavity photon field in the limit of extreme charge imbalance. Using variational wave functions, we examine the competition between different…

Mesoscale and Nanoscale Physics · Physics 2020-05-04 A. Tiene , J. Levinsen , M. M. Parish , A. H. MacDonald , J. Keeling , F. M. Marchetti

The disentanglement of single and many particle properties in 2D semiconductors and their dependencies on high carrier concentration is challenging to experimentally study by pure optical means. We establish an electrolyte gated WS2…

Mesoscale and Nanoscale Physics · Physics 2022-08-18 David Otto Tiede , Nihit Saigal , Hossein Ostovar , Vera Döring , Hendrik Lambers , Ursula Wurstbauer

The enhanced Coulomb interaction in two-dimensional (2D) semiconductors leads to the tightly bound electron-hole pairs known as excitons. The large binding energy of excitons enables the formation of Rydberg excitons with high principal…

Mesoscale and Nanoscale Physics · Physics 2024-02-21 Zhen Lian , Yun-Mei Li , Li Yan , Lei Ma , Dongxue Chen , Takashi Taniguchi , Kenji Watanabe , Chuanwei Zhang , Su-Fei Shi

Understanding high-order correlations or multi-particle entities in a many-body system is not only of fundamental importance in condensed matter physics, but also critical for many technological applications. So far, higher-order…

Materials Science · Physics 2024-05-06 Jiacheng Tang , Cun-Zheng Ning

Exciton polaritons in two-dimensional semiconductors inside microcavities are powerful platforms to explore hybrid light-matter quantum systems. Here, we study a macroscopic coherent population of the lowest energy state of…

Mesoscale and Nanoscale Physics · Physics 2021-10-26 Aleksi Julku , Miguel. A. Bastarrachea-Magnani , Arturo Camacho-Guardian , Georg M. Bruun

We present a many-body theory for Frenkel excitons which takes into account their composite nature exactly. Our approach is based on four commutators similar to the ones we previously proposed for Wannier excitons. They allow us to…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 M. Combescot , W. V. Pogosov

Atomically thin crystals of transition metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization and magnetic field effects. In this work, we investiagte the formation of exciton-polaritons in a…

We study the core hole-electron correlation in coherently coupled molecules by energy dispersive near edge X-ray absorption fine-structure spectroscopy. In a transient phase, which exists during the transition between two bulk arrangements,…

Materials Science · Physics 2013-12-03 M. Scholz , F. Holch , C. Sauer , M. Wiessner , A. Schöll , F. Reinert

Two dimensional materials and their heterostructures constitute a promising platform to study correlated electronic states as well as many body physics of excitons. Here, we present experiments that unite these hitherto separate efforts and…

Mesoscale and Nanoscale Physics · Physics 2020-05-12 Yuya Shimazaki , Ido Schwartz , Kenji Watanabe , Takashi Taniguchi , Martin Kroner , Ataç Imamoğlu

In order to discuss the exciton fine-structure of transition-metal dichalcogenides mono-layers, excitons are first defined in the subspace of electron- and hole states, including the lowest conduction band (LCB) and the uppermost valence…

Mesoscale and Nanoscale Physics · Physics 2019-06-25 Pierre Gilliot , Mathieu Gallart , Bernd Hönerlage

Many-body electron-hole complexes in a semiconductor are important both from a fundamental physics point of view and for practical device applications. A three-body system of electrons (e) and holes (h) (2e1h, or 1e2h) in a two-band…

Mesoscale and Nanoscale Physics · Physics 2024-05-06 Jiacheng Tang , Cun-Zheng Ning

We have measured circularly polarized photoluminescence in monolayer MoSe2 under perpendicular magnetic fields up to 10 T. At low doping densities, the neutral and charged excitons shift linearly with field strength at a rate of $\mp$ 0.12…

The optical properties of transition metal dichalcogenide monolayers are widely dominated by excitons, Coulomb-bound electron-hole pairs. These quasi-particles exhibit giant oscillator strength and give rise to narrow-band, well-pronounced…

Mesoscale and Nanoscale Physics · Physics 2018-07-13 Christian Schneider , Mikhail M. Glazov , Tobias Korn , Sven Höfling , Bernhard Urbaszek

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

Materials Science · Physics 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

Increasing the speed limits of conventional electronics requires innovative approaches to manipulate other quantum properties of electrons besides their charge. An alternative approach utilizes the valley degree of freedom in…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 A. O. Slobodeniuk , P. Koutenský , M. Bartoš , F. Trojánek , P. Malý , T. Novotný , M. Kozák

The region surrounding the excitonic insulator phase is a three-component plasma composed of electrons, holes, and excitons. Due to the extended nature of the excitons, their presence influences the surrounding electrons and holes. We…

Strongly Correlated Electrons · Physics 2015-06-22 B Zenker , D Ihle , F X Bronold , H Fehske

The coupling between a 2D semiconductor quantum well and an optical cavity gives rise to combined light-matter excitations, the exciton-polaritons. These were usually measured when the conduction band is empty, making the single polariton…

Strongly Correlated Electrons · Physics 2017-11-01 Dimitri Pimenov , Jan von Delft , Leonid Glazman , Moshe Goldstein

We present optical spectroscopy (photoluminescence and reflectance) studies of thin layers of the transition metal dichalcogenide WSe2, with thickness ranging from mono- to tetra-layer and in the bulk limit. The investigated spectra show…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 Ashish Arora , Maciej Koperski , Karol Nogajewski , Jacques Marcus , Clement Faugeras , Marek Potemski

Excitons and trions (or exciton-polarons) in transition metal dichalcogenides (TMDs) are known to decay predominantly through intravalley transitions. Electron-hole recombination across different valleys can also play a significant role in…

We investigate the interactions of photoexcited carriers with lattice vibrations in thin films of the layered transition metal dichalcogenide (TMDC) WSe$_2$. Employing femtosecond electron diffraction with monocrystalline samples and first…

Mesoscale and Nanoscale Physics · Physics 2017-07-26 Lutz Waldecker , Roman Bertoni , H. Hübener , Thomas Brumme , Thomas Vasileiadis , Daniela Zahn , Angel Rubio , Ralph Ernstorfer