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Disorder in crystals is rarely random, and instead involves local correlations whose presence and nature are hidden from conventional crystallographic probes. This hidden order can sometimes be controlled, but its importance for physical…

Materials Science · Physics 2023-10-05 Nikolaj Roth , Andrew L. Goodwin

Osmium, the least compressible metal, has recently been observed to undergo abrupt changes in the c/a ratio at extreme pressures. These are claimed to provide evidence for two unusual electronic behaviors: a crossing of the semicore 4f and…

Materials Science · Physics 2022-08-09 Gavin Armstrong Woolman , Graeme J. Ackland

Topotactic transition is a structural phase change in a matrix crystal lattice mediated by the ordered loss/gain and rearrangement of atoms, leading to unusual coordination environments and metal atoms with rare valent states. As early as…

Materials Science · Physics 2023-05-29 Ziang Meng , Han Yan , Peixin Qin , Xiaorong Zhou , Xiaoning Wang , Hongyu Chen , Li Liu , Zhiqi Liu

We studied the crystal structure of TiOCl up to pressures of $p$=25~GPa at room temperature by x-ray powder diffraction measurements. Two pressure-induced structural phase transitions are observed: At $p_{c1}$$\approx$15~GPa emerges an…

Strongly Correlated Electrons · Physics 2015-05-20 J. Ebad-Allah , A. Schönleber , S. van Smaalen , M. Hanfland , M. Klemm , S. Horn , S. Glawion , M. Sing , R. Claessen , C. A. Kuntscher

X-ray diffraction experiments under pressure in a diamond anvil cell have been performed to gauge any response of the crystalline lattice of URu2Si2 to the "hidden order" or antiferromagnetic transitions, the latter of which is accessible…

Strongly Correlated Electrons · Physics 2010-09-29 J. R. Jeffries , N. P. Butch , J. J. Hamlin , S. V. Sinogeikin , W. J. Evans , M. B. Maple

Pressure-induced transitions from ordered intermetallic phases to substitutional alloys to semi-ordered phases were studied in a series of bismuth tellurides. Using angle-dispersive x-ray diffraction, the compounds Bi4Te5, BiTe, and Bi2Te…

Materials Science · Physics 2016-06-28 I. Loa , J. -W. G. Bos , R. A. Downie , K. Syassen

We find an order-disorder transition from crystals to disordered crystals for static packings of frictionless spheres. While the geometric indicators are mostly blind to the transition, disordered crystals already exhibit properties apart…

Soft Condensed Matter · Physics 2015-10-26 Hua Tong , Peng Tan , Ning Xu

A novel stable crystallographic structure is discovered in a variety of ABO3, ABF3 and A2O3 compounds (including materials of geological relevance, prototypes of multiferroics, exhibiting strong spin-orbit effects, etc...), via the use of…

Materials Science · Physics 2015-01-20 Changsong Xu , Bin Xu , Yurong Yang , Huafeng Dong , A. R. Oganov , Shanying Wang , Wenhui Duan , Binglin Gu , L. Bellaiche

In many interesting physical settings, such as the vulcanization of rubber, the introduction of permanent random constraints between the constituents of a homogeneous fluid can cause a phase transition to a random solid state. In this…

Disordered Systems and Neural Networks · Physics 2009-10-31 Paul M. Goldbart

The present review covers the production of new materials under high pressures. A primary limitation on the use of pressures higher than 1 GPa is a small volume and mass of a produced material. Therefore, despite an extremely wide range of…

Materials Science · Physics 2015-06-25 V. V. Brazhkin

Uranium nitrides have been the subject of intense research owing to their potential applications as advanced nuclear fuels. However, the phase diagram of the U-N system at low temperature and high pressure still remains unclear. In this…

Computational Physics · Physics 2018-04-03 Dawei Zhou , JiaHui Yu , Chunying Pu , Yuling Song

Entropic forces in classical many-body systems, e.g. colloidal suspensions, can lead to the formation of new phases. Quantum fluctuations can have similar effects: spin fluctuations drive the superfluidity of Helium-3 and a similar…

Strongly Correlated Electrons · Physics 2018-05-23 Andrew G. Green , Gareth Conduit , Frank Kruger

The physics of an electron solid, held on a cryogenic liquid surface by a pressing electric field, is examined in a low-density regime that has not been explored before. We consider the effect of the pressing field in distorting the surface…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Masudul Haque , Indranil Paul , Sergey Pankov

The model of NH$_3$CH$_2$COOH$\cdot$H$_2$PO$_3$, modified by taking into account the piezoelectric coupling between the ordering structure elements and the strains $\varepsilon_i$, $\varepsilon_j$, is used for investigation of the effects…

Materials Science · Physics 2017-12-15 I. R. Zachek , R. R. Levitskii , A. S. Vdovych

We consider different structures, which can be obtained by polymerization of aromatic organic molecules under high pressures. These 2D and 3D covalently bonded organic polymers and their functionalization can pave the way to production of…

Materials Science · Physics 2021-11-30 V. V. Brazhkin , N. A. Nikolaev , Y. M. Shulga , Y. B. Lebed , M. V. Kondrin

Climate change motivates the search for non-carbon-emitting energy generation and storage solutions. Metal hydrides show promising characteristics for this purpose. They can be further stabilized by tailoring the negative pressure of…

Materials Science · Physics 2022-09-21 A. Tehranchi , P. Chakraborty , M. L. Freixes , E. McEniry , B. Gault , T. Hickel , J. Neugebauer

The behavior of metals at high pressure is of great importance to the fields of shock physics, geophysics, astrophysics, and nuclear materials. In order to further understand the properties of metals at high pressures we studied the…

Materials Science · Physics 2009-11-13 Michael J. Tambe , Nicola Bonini , Nicola Marzari

Perovskite-like oxides $AB'_{1/2}B''_{1/2}$O$_3$ may experience different ordering degrees of $B$-cations, that can be varied by suitable synthesis conditions or post-synthesis treatment. In this work the earlier proposed statistical model…

Materials Science · Physics 2020-03-20 N. V. Ter-Oganessian , V. P. Sakhnenko

This is the first study of the effect of pressure on transition metal dichalcogenides intercalated by atoms that order magnetically. Co$_{1/3}$NbS$_2$ is a layered system where the intercalated Co atoms order antiferromagnetically at T$_N$…

Strongly Correlated Electrons · Physics 2011-10-28 N. Barišić , I. Smiljanić , P. Popčević , A. Bilušić , E. Tutiš , A. Smontara , H. Berger , J. Jaćimović , O. Yuli , L. Forró

Classical phase transitions, like solid-liquid-gas or order-disorder spin magnetic phases, are all driven by thermal energy fluctuations by varying the temperature. On the other hand, quantum phase transitions happen at absolute zero…

Quantum Physics · Physics 2024-03-13 Sabre Kais