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Conventional Li-ion battery ageing models, such as electrochemical, semi-empirical and empirical models, require a significant amount of time and experimental resources to provide accurate predictions under realistic operating conditions.…

Systems and Control · Electrical Eng. & Systems 2026-01-27 Lucu M. , Martinez-Laserna E. , Gandiaga I. , Liu K. , Camblong H. , Widanage W. D. , Marco J

Silicon-containing lithium-ion batteries can exhibit capacity gain early in life, which makes forecasting future cell behavior difficult. We have observed these anomalous trends even in conditions where known mechanisms, such as overhang…

Chemical Physics · Physics 2026-02-17 Marco-Tulio F. Rodrigues , Charles McDaniel , Stephen E. Trask , Daniel P. Abraham

Accurately predicting the lifetime of battery cells in early cycles holds tremendous value for battery research and development as well as numerous downstream applications. This task is rather challenging because diverse conditions, such as…

Signal Processing · Electrical Eng. & Systems 2023-11-27 Han Zhang , Yuqi Li , Shun Zheng , Ziheng Lu , Xiaofan Gui , Wei Xu , Jiang Bian

This paper presents a novel battery modeling framework based on the enhanced single particle model (ESPM) to account for degradation mechanisms of second-life batteries. While accounting for the transport and electrochemical phenomena in…

Systems and Control · Electrical Eng. & Systems 2021-08-19 Gabriele Pozzato , Seong Beom Lee , Simona Onori

Accurately predicting the lifespan of lithium-ion batteries is crucial for optimizing operational strategies and mitigating risks. While numerous studies have aimed at predicting battery lifespan, few have examined the interpretability of…

Machine Learning · Computer Science 2024-04-12 Jaewook Lee , Seongmin Heo , Jay H. Lee

The degradation process of lithium-ion batteries is intricately linked to their entire lifecycle as power sources and energy storage devices, encompassing aspects such as performance delivery and cycling utilization. Consequently, the…

Machine Learning · Computer Science 2023-08-16 Yue Xiang , Bo Jiang , Haifeng Dai

Solid electrolyte interphase (SEI), a thin layer that dynamically forms between active electrode and electrolyte during battery operation, critically governs the performance of rechargeable batteries1-5. An ideal SEI is expected to be…

Understanding battery degradation in electric vehicles (EVs) under real-world conditions remains a critical yet under-explored area of research. Central to this investigation is the challenge of estimating the specific degradation modes in…

Optimization and Control · Mathematics 2024-05-20 Raja Abhishek Appana , Faissal El Idrissi , Prashanth Ramesh , Marcello Canova , Chun Yong Kang , Kimoon Um

This article presents a novel empirical study for the estimation of the State of Charge (SOC) of a lithium-ion (Li-ion) battery which uses a deep learning model with three hidden layers. We model a series of ten vehicle drive cycles that…

Signal Processing · Electrical Eng. & Systems 2020-11-20 Alexandre Barbosa de Lima , Maurício B. C. Salles , José Roberto Cardoso

Conventional Li-ion battery ageing models, such as electrochemical, semi-empirical and empirical models, require a significant amount of time and experimental resources to provide accurate predictions under realistic operating conditions.…

Systems and Control · Electrical Eng. & Systems 2026-01-27 Lucu M. , Martinez-Laserna E. , Gandiaga I. , Liu K. , Camblong H. , Widanage W. D. , Marco J

Charge lost per unit surface area of a silicon electrode due to the formation of solid-electrolyte-interphase (SEI) layer during initial lithiation was quantified, and the species that constitute this layer were identified. Coin cells made…

The Doyle-Fuller-Newman (DFN) model is a common mechanistic model for lithium-ion batteries. The reaction rate constant and diffusivity within the DFN model are key parameters that directly affect the movement of lithium ions, thereby…

Systems and Control · Electrical Eng. & Systems 2025-04-15 Marc D. Berliner , Minsu Kim , Xiao Cui , Vivek N. Lam , Patrick A. Asinger , Martin Z. Bazant , William C. Chueh , Richard D. Braatz

In this article, we derive and discuss a physics-based model for impedance spectroscopy of lithium batteries. Our model for electrochemical cells with planar electrodes takes into account the solid-electrolyte interphase (SEI) as porous…

Chemical Physics · Physics 2020-04-03 Fabian Single , Birger Horstmann , Arnulf Latz

Capacity degradation of lithium-ion batteries under long-term cyclic aging is modelled via a flexible sigmoidal-type regression set-up, where the regression parameters can be interpreted. Different approaches known from the literature are…

Applications · Statistics 2019-07-31 Marcus Johnen , Simon Pitzen , Udo Kamps , Maria Kateri , Dirk Uwe Sauer

Early degradation prediction of lithium-ion batteries is crucial for ensuring safety and preventing unexpected failure in manufacturing and diagnostic processes. Long-term capacity trajectory predictions can fail due to cumulative errors…

Signal Processing · Electrical Eng. & Systems 2023-04-03 Seongyoon Kim , Hangsoon Jung , Minho Lee , Yun Young Choi , Jung-Il Choi

To further improve Lithium-ion batteries (LiBs), a profound understanding of complex battery processes is crucial. Physical models offer understanding but are difficult to validate and parameterize. Therefore, automated machine-learning…

Chemical Physics · Physics 2024-10-28 Micha C. J. Philipp , Yannick Kuhn , Arnulf Latz , Birger Horstmann

Monitoring the health of lithium-ion batteries' internal components as they age is crucial for optimizing cell design and usage control strategies. However, quantifying component-level degradation typically involves aging many cells and…

Computational Engineering, Finance, and Science · Computer Science 2024-04-09 Sina Navidi , Adam Thelen , Tingkai Li , Chao Hu

Accurate battery lifetime prediction is important for preventative maintenance, warranties, and improved cell design and manufacturing. However, manufacturing variability and usage-dependent degradation make life prediction challenging.…

Machine Learning · Computer Science 2024-04-23 Tingkai Li , Zihao Zhou , Adam Thelen , David Howey , Chao Hu

Battery health assessment and recuperation play a crucial role in the utilization of second-life Li-ion batteries. However, due to ambiguous aging mechanisms and lack of correlations between the recovery effects and operational states, it…

Signal Processing · Electrical Eng. & Systems 2024-04-04 Riko I Made , Jing Lin , Jintao Zhang , Yu Zhang , Lionel C. H. Moh , Zhaolin Liu , Ning Ding , Sing Yang Chiam , Edwin Khoo , Xuesong Yin , Guangyuan Wesley Zheng

Lithium-ion batteries are recognised as a key technology to power electric vehicles and integrate grid-connected renewable energy resources. The economic viability of these applications is affected by the battery degradation during its…

Applied Physics · Physics 2020-07-07 Ahmed Gailani , Rehab Mokidm , Moaath El-Dalahmeh , Maad El-Dalahmeh , Maher Al-Greer