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Ultracold polar molecules offer the possibility of exploring quantum gases with interparticle interactions that are strong, long-range, and spatially anisotropic. This is in stark contrast to the dilute gases of ultracold atoms, which have…

Atomic Physics · Physics 2015-05-18 K. -K. Ni , S. Ospelkaus , D. Wang , G. Quemener , B. Neyenhuis , M. H. G. de Miranda , J. L. Bohn , J. Ye , D. S. Jin

By leveraging the hyperfine interaction between the rotational and nuclear spin degrees of freedom, we demonstrate extensive magnetic control over the electric dipole moments, electric dipolar interactions, and ac Stark shifts of…

Atomic Physics · Physics 2024-01-11 Rebekah Hermsmeier , Ana Maria Rey , Timur V. Tscherbul

We probe resonant dipolar interactions between ultracold $^{40}$K$^{87}$Rb molecules and Rydberg $^{87}$Rb atoms in an optically trapped ensemble. Through state-selective ionization detection of the KRb molecules, we observe resonant energy…

Atomic Physics · Physics 2025-04-10 Lingbang Zhu , Jeshurun Luke , Roy Shaham , Yi-Xiang Liu , Kang-Kuen Ni

Molecules are the building blocks of matter and their control is key to the investigation of new quantum phases, where rich degrees of freedom can be used to encode information and strong interactions can be precisely tuned. Inelastic…

Quantum Gases · Physics 2021-01-27 Giacomo Valtolina , Kyle Matsuda , William G. Tobias , Jun-Ru Li , Luigi De Marco , Jun Ye

We consider bosonic dipolar molecules in an optical lattice prepared in a mixture of different rotational states. The 1/r^3 interaction between molecules for this system is produced by exchanging a quantum of angular momentum between two…

Strongly Correlated Electrons · Physics 2009-11-11 Ryan Barnett , Dmitry Petrov , Mikhail Lukin , Eugene Demler

The interaction between light and matter is fundamental to developments in quantum optics and information. Over recent years enormous progress has been made in controlling the interface between light and single emitters including ions,…

We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…

Quantum Physics · Physics 2017-09-13 Elena Kuznetsova , Seth T. Rittenhouse , Hossein R. Sadeghpour , Susanne F. Yelin

The production of molecules from dual species atomic quantum gases has enabled experiments that employ molecules at nanoKelvin temperatures. As a result, every degree of freedom of these molecules is in a well-defined quantum state and…

Quantum Gases · Physics 2018-04-27 Jacob P. Covey , Steven A. Moses , Jun Ye , Deborah S. Jin

We show that topological phases with fractional excitations can occur in two-dimensional ultracold dipolar gases on a particular class of optical lattices. Due to the dipolar interaction and lattice confinement, a quantum dimer model…

Quantum Gases · Physics 2010-04-26 Kai Sun , Erhai Zhao , W. Vincent Liu

We study a means of creating multiparticle entanglement of neutral atoms using pairwise controlled dipole-dipole interactions in a three dimensional optical lattice. For tightly trapped atoms the dipolar interaction energy can be much…

Quantum Physics · Physics 2009-10-31 G. K. Brennen , I. H. Deutsch , P. S. Jessen

We examine the dynamics of Rydberg polaritons with dipolar interactions that propagate in multiple spatial modes. The dipolar excitation exchange between different Rydberg states mediates an effective exchange between polaritons that…

Quantum Physics · Physics 2019-09-17 Mohammad Khazali , Callum R. Murray , Thomas Pohl

We report the investigation on dipolar collisions in rotational state mixtures of ultracold bosonic $^{23}$Na$^{87}$Rb molecules. The large resonant dipole-dipole interaction between molecules in rotational states of opposite parities…

Atomic Physics · Physics 2021-01-13 Junyu He , Xin Ye , Junyu Lin , Mingyang Guo , Goulven Quéméner , Dajun Wang

The recent experimental realization of cold polar molecules in the rotational and vibrational ground state opens the door to the study of a wealth of phenomena involving long-range interactions. By applying an optical lattice to a gas of…

Quantum Gases · Physics 2015-03-13 J. R. Armstrong , N. T. Zinner , D. V. Fedorov , A. S. Jensen

We investigate theoretically the interaction of polar molecules with optical lattices and microwave fields. We demonstrate the existence of frequency windows in the optical domain where the complex internal structure of the molecule does…

Quantum Physics · Physics 2009-11-13 S. Kotochigova , E. Tiesinga

We design dipolar quantum many-body Hamiltonians that will facilitate the realization of exotic quantum phases under current experimental conditions achieved for polar molecules. The main idea is to modulate both single-body potential…

We consider an ultra-small system of polarized bosons on an optical lattice with a ring topology interacting via long range dipole-dipole interactions. Dipoles polarized perpendicular to the plane of the ring reveal sharp transitions…

Quantum Gases · Physics 2013-05-29 Michal Maik , Pierfrancesco Buonsante , Alessandro Vezzani , Jakub Zakrzewski

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational…

We show how state-dependent optical potentials can be used to trap a pair of molecules in different internal states at a separation much smaller than the wavelength of the trapping light. This close spacing greatly enhances the…

Atomic Physics · Physics 2021-04-05 L. Caldwell , M. R. Tarbutt

We show that dressing polar molecules with a far-off-resonant optical field leads to new types of intermolecular potentials, which undergo a crossover from the inverse-power to oscillating behavior depending on the intermolecular distance,…

Atomic Physics · Physics 2011-06-01 Mikhail Lemeshko

Quantum degenerate cold-atom gases provide a remarkable opportunity to study strongly interacting systems. Recent experimental progress in producing ultracold polar molecules with a net electric dipole moment opens up new possibilities to…

Quantum Gases · Physics 2010-12-16 Roman M. Lutchyn , Enrico Rossi , S. Das Sarma