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We directly measure the electronic structure of twisted graphene/MoS2 van der Waals heterostructures, in which both graphene and MoS2 are monolayers. We use cathode lens microscopy and microprobe angle-resolved photoemission spectroscopy…

Evidence for correlated insulating and superconducting phases around regions of high density of states was reported in the strongly spin-orbit coupled van-der Waals material twisted tungsten diselenide (tWSe$_2$). We investigate their…

Strongly Correlated Electrons · Physics 2023-03-15 Lennart Klebl , Ammon Fischer , Laura Classen , Michael M. Scherer , Dante M. Kennes

Van der Waals (vdW) layered materials have rather weaker interlayer bonding than the intra-layer bonding, therefore the exfoliation along the stacking direction enables the achievement of monolayer or few layers vdW materials with emerging…

Here we use low-temperature scanning tunneling microscopy and spectroscopy (STM/STS) to reveal the roles of the narrow electronic band in two 1T-TaS$_2$-related materials (bulk 1T-TaS$_2$ and 4Hb-TaS$_2$). 4Hb-TaS$_2$ is a superconducting…

Mesoscale and Nanoscale Physics · Physics 2024-08-19 Chenhaoping Wen , Jingjing Gao , Yuan Xie , Qing Zhang , Pengfei Kong , Jinghui Wang , Yilan Jiang , Xuan Luo , Jun Li , Wenjian Lu , Yu-Ping Sun , Shichao Yan

1T-TaS$_2$ is a prototypical charge-density-wave (CDW) system with a Mott insulating ground state. Usually, a Mott insulator is accompanied by an antiferromagnetic state. However, the antiferromagnetic order had never been observed in…

Strongly Correlated Electrons · Physics 2020-06-11 Q. Niu , W. Zhang , Y. T. Chan , E. C. T. O'Farrell , R. Doganov , K. Y. Yip , Kwing To Lai , W. C. Yu , B. Ozyilmaz , G. R. Stewart , J. S. Kim , Swee K. Goh

Transition metal dichalcogenides (TMDs) exist in various crystal structures with semiconducting, semi-metallic, and metallic properties. The dynamic control of these phases is of immediate interest for next generation electronics such as…

Materials Science · Physics 2026-01-21 Dante Zakhidov , Daniel A. Rehn , Evan J. Reed , Alberto Salleo

Charge density waves (CDW) and their concomitant periodic lattice distortions (PLD) govern the electronic properties in many layered transition-metal dichalcogenides. In particular, 1T-TaS2 undergoes a metal-to-insulator phase transition as…

The wave-like nature of electrons is evident from quantum interference effects observed during the photoemission process. When there are different nuclei in the unit cell of a crystal and/or structural distortions, photo-electron…

The recently investigated $1T$-polymorph of monolayer NbSe$_2$ revealed an insulating behaviour suggesting a star-of-David phase with $\sqrt{13}\,\times\sqrt{13}$ periodicity associated with a Mott insulator, reminiscent of $1T$-TaS$_2$. In…

Strongly Correlated Electrons · Physics 2018-07-18 Diego Pasquier , Oleg V. Yazyev

Layered transition metal dichalcogenides MoTe$_2$ and WTe$_2$ share almost similar lattice constants as well as topological electronic properties except their structural phase transitions. While the former shows a first-order phase…

Mesoscale and Nanoscale Physics · Physics 2017-05-10 Hyun-Jung Kim , Seoung-Hun Kang , Ikutaro Hamada , Young-Woo Son

Here we investigate how charge density waves (CDW), inherent to a monolayer, are effected by creating twisted van der Waals structures. Homobilayers of metallic transition metal dichalcogenides (TMDs), at small twist angles where there is…

Materials Science · Physics 2023-05-29 Zachary A. H. Goodwin , Vladimir I. Fal'ko

Twist between neighboring layers and variation of interlayer distance are two extra ways to control the physical properties of stacked two-dimensional van der Waals materials without alteration of chemical compositions or application of…

Materials Science · Physics 2024-04-19 Li-Ya Qiao , Xiu-Cai Jiang , Ze Ruan , Yu-Zhong Zhang

Stacking and twisting van der Waals materials provide a powerful tool to design quantum matter and engineer electron correlation. For instance, monolayers of 1T- and 1H-TaS2 are Mott insulating and metallic (also superconducting),…

Materials Science · Physics 2025-02-14 Hyeonhu Bae , Roser Valenti , Igor I. Mazin , Binghai Yan

Transitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking…

Materials Science · Physics 2017-11-09 L. Le Guyader , T. Chase , A. Reid , R. K. Li , D. Svetin , X. Shen , T. Vecchione , X. J. Wang , D. Mihailovic , H. A. Dürr

Twisted WSe$_2$ hosts superconductivity, metal-insulator phase transitions, and field-controllable Fermi-liquid to non-Fermi-liquid transport properties. In this work, we use dynamical mean-field theory to provide a coherent understanding…

We study the phases of correlated charge-density waves that form at a high magnetic field in two parallel graphene flakes separated by a thin insulator. The predicted phases include the square and hexagonal charge-density-wave bubbles, and…

Mesoscale and Nanoscale Physics · Physics 2014-10-28 Csaba Toke , Vladimir I. Fal'ko

We report on depinning of nearly-commensurate charge-density waves in 1T-TaS2 thin-films at room temperature. A combination of the differential current-voltage measurements with the low-frequency noise spectroscopy provide unambiguous means…

Mesoscale and Nanoscale Physics · Physics 2024-06-19 A. Mohammadzadeh , A. Rehman , F. Kargar , S. Rumyantsev , J. M. Smulko , W. Knap , R. K. Lake , A. A. Balandin

Sliding and twisting van der Waals layers with respect to each other gives rise to moir\'e structures with emergent electronic properties. Electrons in these moir\'e structures feel weak potentials that are typically in the tens of…

Mesoscale and Nanoscale Physics · Physics 2020-07-14 Drew Edelberg , Hemant Kumar , Vivek Shenoy , Héctor Ochoa , Abhay N. Pasupathy

Metallization of 1T-TaS2 is generally initiated at the domain boundary of charge density wave (CDW), at the expense of its long-range order. However, we demonstrate in this study that the metallization of 1T-TaS2 can be also realized…

The transition-metal dichalcogenide tantalum disulphide (1$T$-TaS$_2$) hosts a commensurate charge density wave (CCDW) at temperatures below 165~K where it also becomes insulating. The low temperature CCDW phase can be driven into a…

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