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We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

The active manipulation of nuclear spins with radio-frequency (RF) coils is at the heart of nuclear magnetic resonance (NMR) spectroscopy and spin-based quantum devices. Here, we present a microcoil transmitter system designed to generate…

Mesoscale and Nanoscale Physics · Physics 2021-03-10 K. Herb , J. Zopes , K. S. Cujia , C. L. Degen

Quantum sensing with solid-state spins offers the promise of high spatial resolution, bandwidth, and dynamic range at sensitivities comparable to more mature quantum sensing technologies, such as atomic vapor cells and superconducting…

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

Efficiently detecting and characterizing individual spins in solid-state hosts is an essential step to expand the fields of quantum sensing and quantum information processing. While selective detection and control of a few 13C nuclear spins…

Quantum Physics · Physics 2020-10-22 Hyunseok Oh , Jiwon Yun , M. H. Abobeih , Kyung-Hoon Jung , Kiho Kim , T. H. Taminiau , Dohun Kim

Studies of individual quantum systems, which have led to considerable progress in our understanding of quantum physics, have traditionally been associated with atomic gases. In the last decades however, the emphasis has shifted towards…

Materials Science · Physics 2020-11-26 J. -P. Tetienne , L. P. McGuinness , V. Jacques

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

We present a solid state magnetic field imaging technique using a two dimensional array of spins in diamond. The magnetic sensing spin array is made of nitrogen-vacancy (NV) centers created at shallow depths. Their optical response is used…

Magnetic resonance spectroscopy is universally regarded as one of the most important tools in chemical and bio-medical research. However, sensitivity limitations typically restrict imaging resolution to length scales greater than 10 \mu m.…

Sensing single nuclear spins is a central challenge in magnetic resonance based imaging techniques. Although different methods and especially diamond defect based sensing and imaging techniques in principle have shown sufficient…

Nanomagnetometry using the nitrogen-vacancy (NV) centre in diamond has attracted a great deal of interest because of the combined features of room temperature operation, nanoscale resolution and high sensitivity. One of the important goals…

Dynamic Nuclear Polarization (DNP) is a powerful suite of techniques that deliver multifold signal enhancements in NMR and MRI. The generated athermal spin states can also be exploited for quantum sensing and as probes for many-body…

In this work we investigated the time behavior of the polarization of bulk 13C nuclei in diamond above the thermal equilibrium. This nonthermal nuclear hyperpolarization is achieved by cross relaxation between two nitrogen related…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 Ralf Wunderlich , Jonas Kohlrautz , Bernd Abel , Jürgen Haase , Jan Meijer

Enhancing the polarization of nuclear spins surrounding the nitrogen-vacancy (NV) center in diamond has attracted widespread attention recently due to its various applications. Here we present an analytical theory and comprehensive…

Quantum Physics · Physics 2016-07-15 Ping Wang , Bao Liu , Wen Yang

Nuclear magnetic resonance (NMR) schemes can be applied to micron-, and nanometer-sized samples by the aid of quantum sensors such as nitrogen-vacancy (NV) color centers in diamond. These minute devices allow for magnetometry of nuclear…

Quantum Physics · Physics 2021-07-19 C. Munuera-Javaloy , R. Puebla , J. Casanova

NV-diamonds have attracted keen interest for nanoscale sensing and spin manipulation. In particular, the non-equilibrium electron spin polarization after optical excitation of single NV centers has successfully been transferred to nuclear…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 R. Rizzato , F. Bruckmaier , K. S. Liu , S. J. Glaser , D. B. Bucher

The sensing capability of a single optically bright electronic spin in diamond can be enhanced by making use of proximal dark nuclei as ancillary spins. Such systems, so far only realized in bulk diamond, provide orders of magnitude higher…

Quantum Physics · Physics 2017-10-04 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Quantum sensors based on nitrogen-vacancy centers in diamond have emerged as a promising detection modality for nuclear magnetic resonance (NMR) spectroscopy owing to their micron-scale detection volume and non-inductive based detection. A…

We use field-cycling-assisted dynamic nuclear polarization and continuous radio-frequency (RF) driving over a broad spectral range to demonstrate magnetic-field-dependent activation of nuclear spin transport from strongly-hyperfine-coupled…