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Related papers: Competing Ionization and Dissociation in the H$_2$…

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The recombination of an electron with an (initially) hydrogen-like ion is investigated. The effect of the electron-electron interaction is treated rigorously to the first order in the parameter 1/Z and within the screening-potential…

Atomic Physics · Physics 2015-05-19 Vladimir A. Yerokhin , Andrey Surzhykov

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and…

Quantum Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Thanh-Tung Nguyen Dang , Eric Charron

We demonstrate the applicability of extended Lagrangian Born-Oppenheimer quantum-based molecular dynamics (XL-BOMD) to model electron transfer reactions occurring on solid-liquid interfaces. Specifically, we consider the reduction of O$_2$…

We report on an energy-sensitive imaging detector for studying the fragmentation of polyatomic molecules in the dissociative recombination of fast molecular ions with electrons. The system is based on a large area (10 cm x 10 cm)…

We present a formalism for rigorous calculations of cross sections for inelastic and reactive collisions of ultracold atoms and molecules confined by laser fields in quasi-2D geometry. Our results show that the elastic-to-inelastic ratios…

Atomic Physics · Physics 2009-03-20 Z. Li , R. V. Krems

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

Atomic and Molecular Clusters · Physics 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

We present a study of non-sequential double recombination (NSDR) high harmonic generation (HHG) in a molecular-like system. Using a Coulomb-corrected three-step model we are able to classically describe the observed NSDR HHG cutoffs…

Atomic Physics · Physics 2017-07-12 Kenneth K. Hansen , Lars Bojer Madsen

The electron localization in the dissociation of the asymmetric charged molecular ion HeH$^{2+}$ exposed to an intense few-cycle laser pulse is studied by solving numerically the 3D time-dependent Schr\"odinger equation. By varying the…

Atomic Physics · Physics 2011-10-05 Kunlong Liu , Weiyi Hong , Peixiang Lu

The article presents an improved theoretical description of dissociative recombination of HCO$^+$ and DCO$^+$ ions with a low energy electron. In the previous theoretical study (Phys. Rev. A {\bf 74}, 032707) on HCO$^+$, the vibrational…

Chemical Physics · Physics 2009-11-13 Nicolas Douguet , Viatcheslav Kokoouline , Chris H. Greene

The dissociative ionization of $H_2^+$ in a linearly polarized, 400 nm laser pulse is simulated by solving a three-particle time-dependent Schr\"odinger equation in full dimensionality without using any data from quantum chemistry…

Atomic Physics · Physics 2021-01-26 Jinzhen Zhu

A statistical-type model is developed to describe the ion production and electron emission in collisions of (molecular) ions with atoms. The model is based on the Boltzmann population of the bound electronic energy levels of the quasi…

Atomic Physics · Physics 2016-08-19 Zoltán Juhász

Hybrid atom-ion systems are a rich and powerful platform for studying chemical reactions, as they feature both excellent control over the electronic state preparation and readout as well as a versatile tunability over the scattering energy,…

Context. Recent spectroscopic measurements have revealed absorption from higher rotational levels in C$_2$ than previous observations. These improvements are accompanied by the availability of updated radiative and collisional data. Aims.…

Astrophysics of Galaxies · Physics 2025-05-28 J. Le Bourlot , E. Roueff , S. R. Federman , A. M. Ritchey , D. L. Lambert

A variety of phenomena, which reveal itself in distant collisions of ultrarelativistic nuclei is discussed. One or both nuclei may be disintegrated in a single collision event by the long-range electromagnetic forces due to the impact of…

Nuclear Theory · Physics 2007-05-23 I. A. Pshenichnov

Theoretically self-consistent calculations for photoionization and (e + ion) recombination are described. An identical eigenfunction expansion for the ion is employed in coupled channel calculations for both processes, thus ensuring…

Astrophysics · Physics 2007-05-23 Sultana N. Nahar

The bound and resonance states along with corresponding autoionization widths for nitrogen sulphide (NS) molecule are determined using electron NS$^+$ cation scattering calculations. The calculations are performed for $^2{\Sigma}^+$,…

Instrumentation and Methods for Astrophysics · Physics 2024-05-01 F. Iacob , T. Meltzer , J. Zs. Mezei , I. F. Schneider , J. Tennyson

Context: The depletion of heavy elements in cold cores of interstellar molecular clouds can lead to a situation where deuterated forms of H_3^+ are the most useful spectroscopic probes of the physical conditions. Aims: The aim is to predict…

Astrophysics of Galaxies · Physics 2015-05-14 O. Sipilä , E. Hugo , J. Harju , O. Asvany , M. Juvela , S. Schlemmer

We study multiple ionization in proton collisions with water, methane, and ammonia molecules using an independent-atom model. Previous work on total (net) capture and ionization cross sections is extended to treat the multiple ionization…

Atomic Physics · Physics 2023-10-03 Hans Jürgen Lüdde , Marko Horbatsch , Tom Kirchner

Helium ionization plays an important role in the energy balance of the upper chromosphere and transition region. Helium spectral lines are also often used as diagnostics of these regions. We carry out 1D radiation-hydrodynamics simulations…

Solar and Stellar Astrophysics · Physics 2015-06-18 Thomas Peter Golding , Mats Carlsson , Jorrit Leenaarts

We present state-selective measurements on the NH$_2^{+}$ + H$^{+}$ and NH$^{+}$ + H$^{+}$ + H dissociation channels following single-photon double ionization at 61.5 eV of neutral NH$_{3}$, where the two photoelectrons and two cations are…

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