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Using temperature dependent Raman spectroscopy we address the question of how the transition from bulk to few atomic layers affects the charge density wave (CDW) phases in 1T-TaS2. We find that for crystals with thickness larger than approx…

Mesoscale and Nanoscale Physics · Physics 2019-10-30 Adina Luican-Mayer , Jeffrey R. Guest , Saw-Wai Hla

We employ low-frequency Raman spectroscopy to study the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition in 1T-TaS2 ultrathin flakes protected from oxidation. We identify new modes originating from C phase…

Electronic phases that lie outside the equilibrium ground state offer a route to explore competing configurations in correlated materials. In 1T-TaS2, ultrafast excitation accesses a metallic hidden phase that is distinct from the…

Strongly Correlated Electrons · Physics 2026-05-22 Turgut Yilmaz , Anil Rajapitamahuni , Suji Park , Houk Jang , Asish K. Kundu , Elio Vescovo

We present a state-of-the-art x-ray diffraction study of the charge density wave order in 1T-TaS2 as a function of temperature and pressure. Our results prove that the charge density wave, which we characterize in terms of wave vector,…

Strongly Correlated Electrons · Physics 2013-03-27 T. Ritschel , J. Trinckauf , G. Garbarino , M. Hanfland , M. v. Zimmermann , H. Berger , B. Buechner , J. Geck

We investigate mechanically exfoliated thin 1T-TaS$_2$ with scanning tunneling microscopy at room temperature. Sample preparation without air exposure enables access to intrinsic charge-density-wave (CDW) phases of thin 1T-TaS$_2$. At room…

Strongly Correlated Electrons · Physics 2023-02-09 Wooin Yang , Dowook Kim , Hyoung Kug Kim , Tae-Hwan Kim

We report on electrical gating of the charge-density-wave phases and current in h-BN capped three-terminal 1T-TaS$_2$ heterostructure devices. It is demonstrated that the application of a gate bias can shift the source-drain current-voltage…

Layered van der Waals materials are exciting as they often host multiple, competing electronic phases. This article reports experimental observation of the co-existence of insulating and metallic phases deep within the commensurate charge…

Mesoscale and Nanoscale Physics · Physics 2021-12-23 Sruthi S , Hemanta Kumar Kundu , Prasad Vishnubhotla , Aveek Bid

Transitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking…

Materials Science · Physics 2017-11-09 L. Le Guyader , T. Chase , A. Reid , R. K. Li , D. Svetin , X. Shen , T. Vecchione , X. J. Wang , D. Mihailovic , H. A. Dürr

Polymorphic phases and collective phenomena - such as charge density waves (CDWs) - in transition metal dichalcogenides (TMDs) dictate the physical and electronic properties of the material. Most TMDs naturally occur in a single given…

This article reports a comparative study of bulk and surface properties in the transition metal dichalcogenide 1T-TaS$_2$. When heating the sample, the surface displays an intermediate insulating phase that persists for $\sim 10$ K on top…

We study the electronic structure of bulk 1T-TaSe$_2$ in the charge density wave phase at low temperature. Our spatially and angle resolved photoemission (ARPES) data show insulating areas coexisting with metallic regions characterized by a…

Transport studies of atomically thin 1T-TaS2 have demonstrated the presence of intermediate resistance states across the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition, which can be further switched…

Materials Science · Physics 2020-09-29 Tarun Patel , Junichi Okamoto , Tina Dekker , Bowen Yang , Jingjing Gao , Xuan Luo , Wenjian Lu , Yuping Sun , Adam W. Tsen

The layered transition metal dichalcogenide, TaSe2, exhibits rich electronic phenomena across its polymorphs, 1T, 2H, and 3R, largely driven by differences in atomic coordination and c-axis stacking. In the 1T phase, octahedral coordination…

Superconductivity · Physics 2026-02-13 Kusal Dharmasiri , Maxim Avdeev , Despina Louca

We present first-principles calculations of the vibrational properties of the transition metal dichalcogenide 1T-TaS$_2$ for various thicknesses in the high-temperature (undistorted) phase and the low-temperature commensurate charge density…

Suppressing of an ordered state that competes with superconductivity is one route to enhance superconducting transition temperatures. Whereas the effect of suppressing magnetic states is still not fully understood, materials featuring…

For layered materials, the interlayer stacking is a critical degree of freedom tuning electronic properties, while its microscopic characterization faces great challenges. The transition-metal dichalcogenide 1T-TaS$_2$ represents a novel…

Materials Science · Physics 2025-08-01 Li Cheng , Linpeng Nie , Xuanyu Long , Li Liang , Dan Zhao , Jian Li , Zheng Liu , Tao Wu , Xianhui Chen , Xiaolong Zou

We report on depinning of nearly-commensurate charge-density waves in 1T-TaS2 thin-films at room temperature. A combination of the differential current-voltage measurements with the low-frequency noise spectroscopy provide unambiguous means…

Mesoscale and Nanoscale Physics · Physics 2024-06-19 A. Mohammadzadeh , A. Rehman , F. Kargar , S. Rumyantsev , J. M. Smulko , W. Knap , R. K. Lake , A. A. Balandin

Recently, many exotic electronic states, such as quantum spin liquid (QSL) and superconductivity (SC), have been extensively discovered and introduced in layered transition metal dichalcogenides 1T-TaS2 by controlling their complex…

Materials Science · Physics 2022-12-08 Geng Yanyan , Lei Le , Dong Haoyu , Guo Jianfeng , Mi Shuo , Li Yan , Huang Li , Pang Fei , Xu Rui , Zhou Weichang , Liu Zheng , Ji Wei , Cheng Zhihai

Electronic and topological properties of materials are derived from the interplay between crystalline symmetry and dimensionality. Simultaneously introducing 'forbidden' symmetries via quasiperiodic ordering with low-dimensionality into a…

Materials Science · Physics 2022-06-01 Jeffrey D. Cain , Amin Azizi , Matthias Conrad , Sinéad M. Griffin , Alex Zettl

The layered transition metal dichalcogenides host a rich collection of charge density wave (CDW) phases in which both the conduction electrons and the atomic structure display translational symmetry breaking. Manipulating these complex…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 A. W. Tsen , R. Hovden , D. Z. Wang , Y. D. Kim , J. Okamoto , K. A. Spoth , Y. Liu , W. J. Lu , Y. P. Sun , J. Hone , L. F. Kourkoutis , P. Kim , A. N. Pasupathy
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