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Transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform to explore unique excitonic physics via properties of the constituent TMDs and external stimuli. Interlayer excitons (IXs) can form in TMD heterobilayers as…

Mesoscale and Nanoscale Physics · Physics 2023-11-02 Hanlin Fang , Qiaoling Lin , Yi Zhang , Joshua Thompson , Sanshui Xiao , Zhipei Sun , Ermin Malic , Saroj Dash , Witlef Wieczorek

Carbon-based bilayer van der Waals (vdW) materials are attracting much attention due to their predicted interesting physical properties. Here, we theoretically investigate electronic and optical properties of C$_3$B/C$_3$N vdW…

Materials Science · Physics 2023-09-07 Po-Hsin Shih , Thi-Nga Do , Godfrey Gumbs

Exciton-exciton interactions are key to understanding non-linear optical and transport phenomena in van der Waals heterobilayers, which emerged as versatile platforms to study correlated electronic states. We present a combined…

Self-trapped excitons (STEs), renowned for their unique radiative properties, have been harnessed in diverse photonic devices. Yet, a full comprehension and manipulation of STEs remain elusive. In this study, we present novel experimental…

The ability to assemble layers of two-dimensional (2D) materials to form permutations of van der Waals heterostructures provides significant opportunities in materials design and synthesis. Interlayer interactions provide a path to new…

Mesoscale and Nanoscale Physics · Physics 2023-01-09 Zachariah Hennighausen , Jisoo Moon , Kathleen M. McCreary , Connie H. Li , Olaf M. J. van `t Erve , Berend T. Jonker

Van der Waals (vdW) coupling is emerging as a powerful method to engineer and tailor physical properties of atomically thin two-dimensional (2D) materials. In graphene/graphene and graphene/boron-nitride structures it leads to interesting…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Kaihui Liu , Liming Zhang , Ting Cao , Chenhao Jin , Diana Qiu , Qin Zhou , Alex Zettl , Peidong Yang , Steve G. Louie , Feng Wang

Excitons in semiconductors, bound pairs of excited electrons and holes, can form the basis for new classes of quantum optoelectronic devices. A van der Waals heterostructure built from atomically thin semiconducting transition metal…

Little is known about the role of weak interlayer coupling in the second harmonic generation (SHG) effects of two-dimensional van der Waals (vdW) systems. In this article, taking homo-bilayer $MoS_2/MoS_2$ and hetero-bilayer $MoS_2/MoSe_2$…

Computational Physics · Physics 2022-02-02 Xiao Jiang , Lei Kang , Bing Huang

Homogeneous in-plane biaxial tensile strain strengthens the out-of-plane van der Waals interaction in \MoS\ bilayers (BLs) and can be used to fine-tune their terahertz (THz) oscillations. Using ultralow-frequency Raman spectroscopy on…

Materials Science · Physics 2026-02-13 S. Patel , Jose D. Mella , S. Puri , Salvador Barraza-Lopez , H. Nakamura

Van der Waals (vdW) heterobilayers formed by two-dimensional (2D) transition metal dichalcogenides (TMDCs) created a promising platform for various electronic and optical properties. ab initio band results indicate that the band offset of…

Materials Science · Physics 2020-09-04 Yuanyuan Wang , Fengping Li , Wei Wei , Baibiao Huang , Ying Dai

Moire superlattices in van der Waals (vdW) heterostructures could trap strongly bonded and long lived interlayer excitons. Assumed to be localized, these moire excitons could form ordered quantum dot arrays, paving the way for novel…

Computational Physics · Physics 2021-01-22 Hongli Guo , Xu Zhang , Gang Lu

Molecular-scale manipulation of electronic/ionic charge accumulation in materials is a preeminent challenge, particularly in electrochemical energy storage. Layered van der Waals (vdW) crystals exemplify a diverse family of materials that…

Indirect excitons (IXs) are bound pairs of electrons and holes confined in spatially separated layers. We present wide single quantum well (WSQW) heterostructures with high IX mobility, spectrally narrow IX emission, voltage-controllable IX…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 C. J. Dorow , M. W. Hasling , D. J. Choksy , J. R. Leonard , L. V. Butov , K. W. West , L. N. Pfeiffer

Analogous to conventional charge-based electronics, valleytronics aims at encoding data via the valley degree of freedom, enabling new routes for information processing. Long-lived interlayer excitons (IXs) in van der Waals heterostructures…

Applied Physics · Physics 2021-03-30 Tong Ye , Yongzhuo Li , Junze Li , Hongzhi Shen , Junwen Ren , Cun-Zheng Ning , Dehui Li

Twisted van der Waals heterostructures and the corresponding superlattices, moire superlattices, are remarkable new material platforms, in which electron interactions and excited-state properties can be engineered. Particularly, the band…

Mesoscale and Nanoscale Physics · Physics 2019-11-13 Xiaobo Lu , Xiaoqin Li , Li Yang

For quantum technologies based on single excitons and spins, the deterministic placement and control of a single exciton is a long-standing goal. MoSe2-WSe2 heterostructures host spatially indirect interlayer excitons (IXs) which exhibit…

Identifying two-dimensional heterostructures with exceptional electronic and optical properties remains an active area of research in advanced optoelectronics. Here, we present a comprehensive first-principles investigation of the…

Dipolar (or spatially indirect) excitons (IXs) in semiconductor double quantum well (DQW) subjected to an electric field are neutral species with a dipole moment oriented perpendicular to the DQW plane. Here, we theoretically study…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 C. Hubert , K. Cohen , A. Ghazaryan , M. Lemeshko , R. Rapaport , P. V. Santos

Observation of interlayer, charge-transfer (CT) excitons in van der Waals heterostructures (vdWHs) based on 2D-2D systems has been well investigated. While conceptually interesting, these charge transfer excitons are highly delocalized and…

Narrow lines in photoluminescence (PL) spectra of excitons are characteristic of low-dimensional semiconductors. These lines correspond to the emission of exciton states in local minima of a potential energy landscape formed by fluctuations…

Mesoscale and Nanoscale Physics · Physics 2026-04-17 Zhiwen Zhou , E. A. Szwed , W. J. Brunner , H. Henstridge , L. H. Fowler-Gerace , L. V. Butov