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In order to promote the development of the next generation of nano-spintronic devices, it is of great significance to tune the freedom of valley in two-dimensional (2D) materials. Here, we propose a mechanism for manipulating the valley and…

Materials Science · Physics 2024-09-11 Hanbo Sun , Yewei Ren , Chao Wu , Pengqiang Dong , Weixi Zhang , Yin-Zhong Wu , Ping Li

The selective control of specific momentum valleys lies at the core of valleytronics, a field that has thus far focused primarily on the $\mathbf{K}$ and $\mathbf{K'}$ valleys in transition metal dichalcogenides (TMDs). However, direct…

Strongly Correlated Electrons · Physics 2026-05-05 Youngjae Kim

Although single-layer transition-metal dichalcogenides with novel valley functionalities are promising candidate to realize valleytronic devices, the essential understanding of valley depolarization mechanisms is still incomplete. Based on…

Mesoscale and Nanoscale Physics · Physics 2020-12-18 Tae-Young Jeong , Soungmin Bae , Seong-Yeon Lee , Suyong Jung , Yong-Hoon Kim , Ki-Ju Yee

Valleytronics is rapidly emerging as an exciting area of basic and applied research. In two dimensional systems, valley polarisation can dramatically modify physical properties through electron-electron interactions as demonstrated by such…

We identify a valley-polarized Chern insulator in the van der Waals heterostructure, Pt$_{2}$HgSe$_{3}$/CrI$_3$, for potential applications with interplay between electric, magnetic, optical, and mechanical effects. The interlayer proximity…

Materials Science · Physics 2021-09-29 Zheng Liu , Yulei Han , Yafei Ren , Qian Niu , Zhenhua Qiao

Transition-metal dichalcogenides monolayers exhibit strong exciton resonances that enable intense light-matter interactions at room temperature (RT). However, the sensitivity of these materials to the surrounding environment and their…

Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

Atomically thin transition metal dichalcogenides possess valley dependent functionalities that are usually available only at crogenic temperatures, constrained by various valley depolarization scatterings. The formation of exciton…

Transition metal dichalcogenides (TMD) monolayers, holding potential as good sunlight absorbers, are promising materials for next-generation optoelectronic devices. They may enable ultrathin photovoltaic(PV) devices thanks to their…

Materials Science · Physics 2022-11-28 C. Attaccalite , M. S. Prete , M. Palummo , O. Pulci

In single-layer WSe$_2$, a paradigmatic semiconducting transition metal dichalcogenide, a circularly polarized laser field can selectively excite electronic transitions in one of the inequivalent $K^{\pm}$ valleys. Such selective valley…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Alejandro Molina-Sánchez , Davide Sangalli , Ludger Wirtz , Andrea Marini

Van der Waals materials enable the construction of atomically sharp interfaces between compounds with distinct crystal and electronic properties. This is dramatically exploited in moir\'e systems, where a lattice mismatch or twist between…

Application of transition metal dichalcogenides (TMDC) in photonic, optoelectronic or valleytronic devices requires the growth of continuous monolayers, heterostructures and alloys of different materials in a single process. We present a…

The valley degree of freedom is a sought-after quantum number in monolayer transition-metal dichalcogenides. Similar to optical spin orientation in semiconductors, the helicity of absorbed photons can be relayed to the valley (pseudospin)…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 Min Yang , Cedric Robert , Zhengguang Lu , Dinh Van Tuan , Dmitry Smirnov , Xavier Marie , Hanan Dery

Understanding the electronic transport properties of layered, van der Waals transition metal halides (TMHs) and chalcogenides is a highly active research topic today. Of particular interest is the evolution of those properties with changing…

Valleytronics is one of the breaking-through to the technology of electronics, which provides a new degree of freedom to manipulate the properties of electrons. Combining DFT calculations, optical absorption analysis and the linear…

Materials Science · Physics 2017-08-16 Tiantian Zhang , Sijie Zhang , Gang Xu , Nanlin Wang , Zhong Fang

We report experimental observation of 2s exciton radiative emission from monolayer tungsten diselenide, enabled by hexagonal boron nitride protected high-quality samples. The 2s luminescence is highly robust and persists up to 150K,…

Mesoscale and Nanoscale Physics · Physics 2018-01-31 Shao-Yu Chen , Thomas Goldstein , Jiayue Tong , Takashi Taniguchi , Kenji Watanabe , Jun Yan

Electrons in monolayer transition metal dichalcogenides (TMDs) possess both the valley and spin degree of freedom. These internal quantum degrees of freedom have provided an ideal laboratory for exploring both new physical phenomena and…

Mesoscale and Nanoscale Physics · Physics 2017-02-21 Zefang Wang , Jie Shan , kin Fai Mak

Van der Waals (vdW) polytypes of broken inversion and mirror symmetries were recently shown to exhibit switchable electric polarization even at the ultimate two-layer thin limit. Their out-of-plane polarization was found to accumulate in a…

The two-fold valley degeneracy in two-dimensional (2D) semiconducting transition metal dichalcogenides (TMDCs) (Mo,W)(S,Se)2 is suitable for "valleytronics", the storage and manupulation of information utilizing the valley degree of…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Shao-Yu Chen , Changxi Zheng , Michael S. Fuhrer , Jun Yan

Monolayer transition metal dichalcogenides have emerged as prominent candidates to explore the complex interplay between the spin and the valleys degrees of freedom. The strong spin-orbit interaction and broken inversion symmetry within…