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Current-induced electron spin polarization is shown to produce nuclear hyperpolarization through dynamic nuclear polarization. Saturated fields of several millitesla are generated upon the application of electric field over a timescale of a…

Mesoscale and Nanoscale Physics · Physics 2014-10-31 C. J. Trowbridge , B. M. Norman , Y. K. Kato , D. D. Awschalom , V. Sih

We demonstrate continuous Pound-Drever-Hall (PDH) nondestructive monitoring of the electron spin polarization of an atomic vapor in a microfabricated vapor cell within an optical resonator. The two-chamber silicon and glass cell contains…

The nature of the nano-scale environment presents a major challenge for solid-state implementation of spin-based qubits. In this work, a single electron spin in an optically pumped nanometer-sized III-V semiconductor quantum dot is used to…

We use microwave-induced dynamic nuclear polarization (DNP) of the substitutional nitrogen defects (P1 centers) in diamond to hyperpolarize bulk $^{13}$C nuclei in both single crystal and powder samples at room temperature at 3.34 T. The…

The SpinQuest experiment at Fermilab employs a dynamically polarized solid ammonia target to probe the spin structure of the proton, requiring stable, optimized microwave-driven Dynamic Nuclear Polarization (DNP) under high radiation…

Instrumentation and Detectors · Physics 2026-04-28 Vibodha Bandara , Jordan D. Roberts , Dustin Keller

Under ambient conditions, spin impurities in solid-state systems are found in thermally-mixed states and are optically "dark", i.e., the spin states cannot be optically controlled. Nitrogen-vacancy (NV) centers in diamond are an exception…

Quantum Physics · Physics 2012-11-13 Chinmay Belthangady , N. Bar-Gill , L. M. Pham , K. Arai , D. Le Sage , P. Cappellaro , R. L. Walsworth

For the polarization of neutrons with an energy level of \textcolor{black}{$>0.1$ eV}, we developed a novel polarized proton spin filter based on dynamic nuclear polarization using photo-excited triplet electron spins. The spin filter…

Instrumentation and Detectors · Physics 2020-07-21 Shusuke Takada , Kenichiro Tateishi , Yasuo Wakabayashi , Yoshimasa Ikeda , Tamaki Yoshioka , Yoshie Otake , Tomohiro Uesaka

Recently, Pang et al reported a novel polarization transfer scheme applicable to three-spin systems, whereby a rotating-frame NMR analogue of the cross effect could transfer polarization between; e.g., two 13Cs and an 15N in a single…

Quantum Physics · Physics 2026-04-21 Sundaresan Jayanthi , Adonis Lupulescu , Julia Grinshtein , Lucio Frydman

Dynamic nuclear polarization (DNP) is a method of enhancing NMR signals via the transfer of polarization from electron spins to nuclear spins using on-resonance microwave (MW) irradiation. In most cases, monochromatic continuous-wave (MCW)…

Chemical Physics · Physics 2022-11-17 Daphna Shimon , Kelly A. Cantwell , Linta Joseph , Chandrasekhar Ramanathan

The representation of information within the spins of electrons and nuclei has been powerful in the ongoing development of quantum computers. Although nuclear spins are advantageous as quantum bits (qubits) due to their long coherence…

Enrichment of nuclear spin isomers of molecules by infrared radiation resonant to molecular rovibrational transition is considered. Special attention is given to the enrichment by light-induced crossing of far separated ortho and para…

Chemical Physics · Physics 2007-05-23 Pavel Chapovsky

A sensitivity increase of two orders of magnitude in proton (1H) and carbon (13C) spins via dynamic nuclear polarization (DNP) has been accomplished recently using a compact benchtop DNP polarizer operating at 1 T and 77 K. However the DNP…

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

A theoretical study of spin dynamics in non-relativistic particle beams with interacting angular momenta traversing static, spatially varying magnetic fields is presented. The computational framework evaluates sinusoidal magnetic field…

Adiabatic fast passage (AFP) is a rapid method for reversing nuclear polarization and manipulating spin populations in polarized solid targets, avoiding the long repolarization times associated with dynamic nuclear polarization (DNP). We…

Atomic Physics · Physics 2026-05-26 M. F. Hossain , K. Nakano , N. G. Vismith , D. Keller

Magnetic noise of atomic nuclear spins is a major problem for solid state spin qubits. Highly-polarized nuclei would not only overcome this obstacle, but also make nuclear spins a useful quantum information resource. However, achieving…

The generation, manipulation and detection of spin-polarized electrons in nanostructures define the main challenges of spin-based electronics[1]. Amongst the different approaches for spin generation and manipulation, spin-orbit coupling,…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Sergio O. Valenzuela , M. Tinkham

By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 1000 at a fixed…

A quantum-mechanical many-particle system may exhibit non-local behavior in that measurements performed on one of the particles can affect a second one that is far apart. These so-called entangled states are crucial for the implementation…

Other Condensed Matter · Physics 2009-11-10 J. M. Bao , A. V. Bragas , J. K. Furdyna , R. Merlin

We propose a general technique to produce cold spin-polarized molecules, in which rotationally excited states are first populated by coherent microwave excitation, and then allowed to spin-flip and relax via collisional quenching, which…

Chemical Physics · Physics 2024-11-13 Rebekah Hermsmeier , Timur V. Tscherbul
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