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We have developed a Green-Kubo relation that enables accurate calculations of friction at solid-liquid interfaces directly from equilibrium molecular dynamics (MD) simulations and that provides a pathway to bypass the time-scale limitations…

Statistical Mechanics · Physics 2016-08-08 Kai Huang , Izabela Szlufarska

We introduce a novel approach to model heat transport in solids, based on the Green-Kubo theory of linear response. It naturally bridges the Boltzmann kinetic approach in crystals and the Allen-Feldman model in glasses, leveraging…

Materials Science · Physics 2019-09-11 Leyla Isaeva , Giuseppe Barbalinardo , Davide Donadio , Stefano Baroni

The interfacial thermal resistance determines condensation-evaporation processes and thermal transport across material-fluid interfaces. Despite its importance in transport processes, the interfacial structure responsible for the thermal…

Soft Condensed Matter · Physics 2017-08-02 Jordan Muscatello , Enrique Chacón , Pedro Tarazona , Fernando Bresme

The thermal conductivity of classical multi-component fluids is seemingly affected by the intrinsic arbitrariness in the definition of the atomic energies and it is ill-conditioned numerically, when evaluated from the Green-Kubo theory of…

Statistical Mechanics · Physics 2019-09-30 Riccardo Bertossa , Federico Grasselli , Loris Ercole , Stefano Baroni

The properties of the interface between solid and melt are key to solidification and melting, as the interfacial free energy introduces a kinetic barrier to phase transitions. This makes solidification happen below the melting temperature,…

Statistical Mechanics · Physics 2015-12-02 Bingqing Cheng , Gareth A. Tribello , Michele Ceriotti

Understandings heat transfer across a solid/liquid interface is important to develop new pathways to improve thermal management in various energy applications. One of the important questions that arises in this context is the impact of…

Boundary conditions for the solid-liquid interface of the solidifying pure melt have been derived. In the derivation the model of Gibbs interface is used. The boundary conditions include both the state quantities of bulk phases are taken at…

Materials Science · Physics 2016-11-02 Gennady Buchbinder , Peter Galenko

Using equilibrium and nonequilibrium molecular dynamics simulations, we determine the Kapitza resistance (or thermal contact resistance) at a model liquid solid interface. The Kapitza resistance (or the associated Kapitza length) can reach…

Materials Science · Physics 2009-11-07 Jean-Louis Barrat , François Chiaruttini

Given the unique optical properties of LiF, it is often used as an observation window in high-temperature and pressure experiments; and, hence, estimates of its transmission properties are necessary to interpret observations. Since direct…

Materials Science · Physics 2016-07-27 R. E. Jones , D. K. Ward

The Green-Kubo theory of thermal transport has long be considered incompatible with modern simulation methods based on electronic-structure theory, because it is based on such concepts as energy density and current, which are ill-defined at…

Statistical Mechanics · Physics 2018-08-20 Stefano Baroni , Riccardo Bertossa , Loris Ercole , Federico Grasselli , Aris Marcolongo

We obtain an exact Green-Kubo type linear response result for the heat current in an open system. The result is derived for classical Hamiltonian systems coupled to heat baths. Both lattice models and fluid systems are studied and several…

Statistical Mechanics · Physics 2009-11-13 Anupam Kundu , Abhishek Dhar , Onuttom Narayan

The problem presented involves the development of a new analytical model for the general fluid-solid temperature jump. To the best of our knowledge, there are no analytical models that provide the accurate predictions of the temperature…

Soft Condensed Matter · Physics 2016-12-26 Jian-Jun Shu , Ji Bin Melvin Teo , Weng Kong Chan

In the past few years, the theory of thermal transport in amorphous solids has been substantially extended beyond the Allen-Feldman model. The resulting formulation, based on the Green-Kubo linear response or the Wigner-transport equation,…

Materials Science · Physics 2023-09-08 Alfredo Fiorentino , Paolo Pegolo , Stefano Baroni

In this paper new characterization equipment for thermal interface materials is presented. Thermal management of electronic products relies on the effec-tive dissipation of heat. This can be achieved by the optimization of the system design…

Materials Science · Physics 2007-09-13 R. Schacht , D. May , B. Wunderle , O. Wittler , A. Gollhardt , B. Michel , H. Reichl

We report a numerical study of thermo-osmotic slip, i.e. the particle flux induced by a thermal gradient along a solid-fluid interface. To facilitate comparison with theory, we consider a model of an ideal but viscous gas. We compare three…

Statistical Mechanics · Physics 2019-10-23 Karel Proesmans , Daan Frenkel

In this paper we describe a spatial decomposition of the thermal conductivity, what we name "site-projected thermal conductivity", a gauge of the thermal conduction activity at each site. The method is based on the Green-Kubo formula and…

Materials Science · Physics 2025-09-16 C. Ugwumadu , A. Gautam , Y. G. Lee , D. A. Drabold

Four results associated with the diffuse-interface model (DIM) for contact lines are reported in this paper. First, a boundary condition is derived, which states that the fluid near a solid wall must have a certain density $\rho_{0}$…

Fluid Dynamics · Physics 2021-09-27 E. S. Benilov

Molecular dynamics simulations are used to simulate the thermal properties of a model fluid containing nanoparticles (nanofluid). By modelling transient absorption experiments, we show that they provide a reliable determination of…

Materials Science · Physics 2015-06-25 Mihail Vladkov , J. -L. Barrat

This work is aimed at the study and analysis of the heat transport on a metal bar of length $L$ with a solid-solid interface. The process is assumed to be developed along one direction, across two homogeneous and isotropic materials.…

Analysis of PDEs · Mathematics 2021-10-28 Diana Rubio , Domingo A. Tarzia , Guillermo F. Umbricht

The existed theories and methods for calculating interfacial thermal conductance of solid-solid interface lead to diverse values that deviate from experimental measurements. In this letter, We propose a model to estimate the ITC at high…

Materials Science · Physics 2020-11-20 Jinxin Zhong , Zhiguo Wang , Xiaobo Li , Jun Liu , Jun Zhou
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