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We present a coupled cluster method (CCM) with optimized excitation operators. The efficiency comes from a parameterized form of excitation operators. The parameters are found by variational optimization procedure. The resultant number of…

Strongly Correlated Electrons · Physics 2014-12-09 Quanlin Jie

Three earlier relativistic coupled-cluster (RCC) calculations of dipole polarizability ($\alpha_d$) of the Cd atom are not in good agreement with the available experimental value of $49.65(1.65) \ e a_0^3$. Among these two are finite-field…

Atomic Physics · Physics 2018-08-15 B. K. Sahoo , Yan-mei Yu

The issue of orbital relaxation in computational core-hole spectroscopy, specifically x-ray absorption, has been a major problem for methods such as equation-of-motion coupled cluster with singles and doubles (EOM-CCSD). The…

Chemical Physics · Physics 2025-03-26 Megan Simons , Devin A. Matthews

Relativistic coupled-cluster (RCC) theory at the singles and doubles approximation has been implemented to estimate nuclear spin dependent (NSD) parity violating (PV) electric dipole (E1) transition amplitudes ($E1_{PV}^{NSD}$) among…

Atomic Physics · Physics 2024-08-19 A. Chakraborty , B. K. Sahoo

The {\it Principle of Maximum Conformality} (PMC), which generalizes the conventional Gell-Mann-Low method for scale-setting in perturbative QED to non-Abelian QCD, provides a rigorous method for achieving unambiguous scheme-independent,…

High Energy Physics - Phenomenology · Physics 2023-03-21 Xu-Dong Huang , Jiang Yan , Hong-Hao Ma , Leonardo Di Giustino , Jian-Ming Shen , Xing-Gang Wu , Stanley J. Brodsky

Tailored coupled cluster theory represents a computationally inexpensive way to describe static and dynamical electron correlation effects. In this work, we scrutinize the performance of various tailored coupled cluster methods externally…

Chemical Physics · Physics 2021-03-24 Aleksandra Leszczyk , Mihály Máté , Örs Legeza , Katharina Boguslawski

We present an extension of the pair coupled cluster doubles (p-CCD) method to quasiparticles and apply it to the attractive pairing Hamiltonian. Near the transition point where number symmetry gets spontaneously broken, the proposed…

Immense interest in quantum computing has prompted development of electronic structure methods that are suitable for quantum hardware. However, the slow pace at which quantum hardware progresses, forces researchers to implement their ideas…

Quantum Physics · Physics 2025-02-26 Ilya G. Ryabinkin , Seyyed Mehdi Hosseini Jenab , Scott N. Genin

We present the results of our calculations of the parity nonconserving electric dipole amplitudes ($E1_{PNC}$) for the $6s ~ ^2S_{1/2} - 5d ~ ^2D_{3/2;5/2}$ transitions of $^{133}$Cs employing a relativistic coupled-cluster (RCC) method.…

Atomic Physics · Physics 2017-11-22 B. K. Sahoo , B. P. Das

Wave functions based on electron-pair states provide inexpensive and reliable models to describe quantum many-body problems containing strongly-correlated electrons, given that broken-pair states have been appropriately accounted for by,…

Chemical Physics · Physics 2021-03-17 Artur Nowak , Ors Legeza , Katharina Boguslawski

We have developed a relativistic coupled-cluster theory to incorporate nuclear spin-dependent interaction Hamiltonians perturbatively. This theory is ideal to calculate parity violating nuclear spin-dependent electric dipole transition…

Atomic Physics · Physics 2011-06-09 B. K. Mani , D. Angom

Multicomponent systems are defined as chemical systems that require a quantum mechanical description of two or more different types of particles. Non-Born-Oppenheimer electron-nuclear interactions in molecules, electron-hole interactions in…

Chemical Physics · Physics 2015-10-21 Benjamin H. Ellis , Somil Aggarwal , Arindam Chakraborty

We have studied electron correlations in the doped two-dimensional (2D) Hubbard model by using the coupled-cluster method (CCM) to investigate whether or not the method can be applied to correct the independent particle approximations…

Strongly Correlated Electrons · Physics 2009-10-31 Yoshihiro Asai , Hideki Katagiri

We propose a method for measuring parity violation in neutral atoms. It is an adaptation of a seminal work by Fortson [Phys. Rev. Lett. {\bf 70}, 2383 (1993)], proposing a scheme for a single trapped ion. In our version, a large sample of…

Atomic Physics · Physics 2019-11-20 A. Kastberg , T. Aoki , B. K. Sahoo , Y. Sakemi , B. P. Das

We present a new high-order coupled cluster method (CCM) formalism for the ground states of lattice quantum spin systems for general spin quantum number, $s$. This new ``general-$s$'' formalism is found to be highly suitable for a…

Strongly Correlated Electrons · Physics 2010-05-07 D. J. J. Farnell , R. F. Bishop , K. A. Gernoth

We propose a new parton model and demonstrate that the model describes the relevant experimental data at high energies. The model is based on Pomeron calculus in 1+1 space-time dimensions, as suggested in Ref. [18] and on simple assumptions…

High Energy Physics - Phenomenology · Physics 2019-03-27 E. Gotsman , E. Levin , I. Potashnikova

Our previously developed Constrained-Pairing Mean-Field Theory (CPMFT) is shown to map onto an Unrestricted Hartree-Fock (UHF) type method if one imposes a corresponding pair constraint to the correlation problem that forces occupation…

Strongly Correlated Electrons · Physics 2015-05-19 Takashi Tsuchimochi , Thomas M. Henderson , Gustavo E. Scuseria , Andreas Savin

We show that the asymmetries in the nuclear resonance fluorescence processes with a circular polarized photon beam may be used as a tool for studying the parity non-conservation (PNC) in nuclei. The PNC asymmetry measurements both in…

Nuclear Theory · Physics 2009-11-11 A. I. Titov , M. Fujiwara , K. Kawase

It is conventional to choose a typical momentum transfer of the process as the renormalization scale and take an arbitrary range to estimate the uncertainty in the QCD prediction. However, predictions using this procedure depend on the…

High Energy Physics - Phenomenology · Physics 2012-07-24 Stanley J. Brodsky , Xing-Gang Wu

The generator coordinate method (GCM) casts the wavefunction as an integral over a weighted set of non-orthogonal single determinantal states. In principle this representation can be used like the configuration interaction (CI) or shell…

Nuclear Theory · Physics 2015-06-23 Jason L. Stuber