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Aiming to combine density functional theory (DFT) and wavefunction theory, we study a mapping from the many-body interacting system to an effectively-interacting Kohn-Sham system instead of a non-interacting Kohn-Sham system. Because a…

Chemical Physics · Physics 2020-02-19 Shunsuke A. Sato , Angel Rubio

By using a Cahn-Hoffman $\boldsymbol{\xi}$-vector formulation, we propose a sharp-interface approach for solving solid-state dewetting problems in two dimensions. First, based on the thermodynamic variation and smooth vector-field…

Soft Condensed Matter · Physics 2019-03-27 Wei Jiang , Quan Zhao

We present unrestricted Hartree Fock method coupled with configuration interaction (CI) method (URHF-CI) suitable for the calculation of ground and excited states of large number of electrons localized by complex gate potentials in…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Ramin M. Abolfath , Pawel Hawrylak

We fully generalize a previously-developed computational geometry tool [1] to perform large-scale simulations of arbitrary two-dimensional faceted surfaces $z = h(x,y)$. Our method uses a three-component facet/edge/junction storage model,…

Mathematical Physics · Physics 2011-10-17 Scott A. Norris , Stephen J. Watson

Trajectory-based mixed quantum-classical approaches to coupled electron-nuclear dynamics suffer from well-studied problems such as the lack of (or incorrect account for) decoherence in the trajectory surface hopping method and the inability…

Quantum Physics · Physics 2016-02-29 Federica Agostini , Seung Kyu Min , Ali Abedi , E. K. U. Gross

We suggest a procedure for demonstrating quantum coherence and measuring decoherence times between different fluxoid states of a SQUID by using ``adiabatic inversion'', where one macroscopic fluxoid state is smoothly transferred into the…

Condensed Matter · Physics 2016-08-31 P. Silvestrini , L. Stodolsky

We demonstrate that, rather than resorting to high-cost dynamic correlation methods, qualitative failures in excited-state potential energy surface predictions can often be remedied at no additional cost by ensuring that optimal molecular…

Chemical Physics · Physics 2020-06-18 Lan Nguyen Tran , Eric Neuscamman

Mixed-quantum classical (MQC) methods for simulating the dynamics of molecules at metal surfaces have the potential to accurately and efficiently provide mechanistic insight into reactive processes. Here, we introduce simple two-dimensional…

Chemical Physics · Physics 2023-08-02 James Gardner , Scott Habershon , Reinhard J. Maurer

The exact nuclear time-dependent potential energy surface arises from the exact decomposition of electronic and nuclear motion, recently presented in [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys. Rev. Lett. 105, 123002 (2010)]. Such…

Chemical Physics · Physics 2015-06-16 Federica Agostini , Ali Abedi , Yasumitsu Suzuki , E. K. U. Gross

We unite two of the most widely used approaches for strongly damped, non-Markovian open quantum dynamics, the Hierarchical Equations of Motion (HEOM) and the pseudomode method by proving two statements: First, every physical bath…

Quantum Physics · Physics 2026-04-09 Kai Müller , Walter T. Strunz

This work addresses the problem of optimally steering the state covariance of a linear stochastic system from an initial to a target, subject to hybrid transitions. The nonlinear and discontinuous jump dynamics complicate the control design…

Optimization and Control · Mathematics 2024-10-18 Hongzhe Yu , Diana Frias Franco , Aaron M. Johnson , Yongxin Chen

A novel stochastic fluid model is proposed with non-ideal structure factor consistent with compressibility, and adjustable transport coefficients. This Stochastic Hard Sphere Dynamics (SHSD) algorithm is a modification of the Direct…

Statistical Mechanics · Physics 2009-11-13 Aleksandar Donev , Berni J. Alder , Alejandro L. Garcia

Approaches based on viscous hydrodynamics for the hot and dense stage and hadronic transport for the final dilute rescattering stage are successfully applied to the dynamic description of heavy ion reactions at high beam energies. One…

High Energy Physics - Phenomenology · Physics 2017-12-06 C. Schwarz , D. Oliinychenko , L. -G. Pang , S. Ryu , H. Petersen

We consider a strongly driven two-level (spin) system, with a periodic external field that induces a sequence of avoided level crossings. The spin system interacts with a bosonic reservoir which leads to decoherence. A Markovian dynamical…

Quantum Physics · Physics 2008-02-05 Peter Foldi , Mihaly G. Benedict , F. M. Peeters

Dynamical decoupling techniques constitute an integral part of many quantum sensing platforms, often leading to orders-of-magnitude improvements in coherence time and sensitivity. Most AC sensing sequences involve a periodic echo-like…

We present a new method that accurately approximates the shell-model ground-state by products of suitable states. The optimal factors are determined by a variational principle and result from the solution of rather low-dimensional…

Nuclear Theory · Physics 2007-05-23 T. Papenbrock , D. J. Dean

We propose to measure the importance of spin-orbit couplings (SOCs) in the nonadiabatic molecular quantum dynamics rigorously with quantum fidelity. To make the criterion practical, quantum fidelity is estimated efficiently with the…

Chemical Physics · Physics 2013-01-15 Tomas Zimmermann , Jiri Vanicek

Accurate exchange-correlation (XC) potentials are essential for density functional theory, yet reliable approximations remain challenging for strongly correlated systems. In this work, we present a quantum algorithmic framework to determine…

Strongly Correlated Electrons · Physics 2026-03-18 H. Arslan Hashim , Volodymyr M. Turkowski , Eduardo R. Mucciolo

We adapt and extend a formulation for soluble surfactant transport in multiphase flows recently presented by Muradoglu & Tryggvason (JCP 274 (2014) 737-757) to the context of the Level Contour Reconstruction Method (Shin et al. IJNMF 60…

Computational Engineering, Finance, and Science · Computer Science 2018-03-14 Seungwon Shin , Jalel Chergui , Damir Juric , Lyes Kahouadji , Omar K. Matar , Richard V. Craster

The factor graph framework is a convenient modeling technique for robotic state estimation where states are represented as nodes, and measurements are modeled as factors. When designing a sensor fusion framework for legged robots, one often…

Robotics · Computer Science 2019-05-22 Ross Hartley , Maani Ghaffari Jadidi , Lu Gan , Jiunn-Kai Huang , Jessy W. Grizzle , Ryan M. Eustice