Related papers: Imprinting chirality on atoms using synthetic chir…
It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…
We present a scheme to synthesize a three-dimensional laser field that produces a chiral electron momentum distribution upon strong-field ionization of atoms. Our approach employs two orthogonally propagating two-color laser beams. This…
We formulate a transparent measure that quantifies chirality in single electron ionization triggered in atoms, which are achiral systems. We do so in the context of Ar driven by a new type of optical fields that consists of two…
We introduce and theoretically analyze the concept of manipulating optical chirality via strong coupling of the optical modes of chiral nanostructures with excitonic transitions in molecular layers or semiconductors. With chirality being…
Synthetic chiral light enables ultrafast and highly efficient imaging of molecular chirality. Unlike standard circularly polarized light, the handedness of synthetic chiral light does not rely on the spatial structure of the light field: it…
We calculate the force of a near-resonant guided light field of an ultrathin optical fiber on a two-level atom. We show that, if the atomic dipole rotates in the meridional plane, the magnitude of the force of the guided light depends on…
Chirality is a pervasive form of symmetry that is intimately connected to the physical properties of solids, as well as the chemical and biological activity of molecular systems. However, its control with light is challenging, because…
Chiral systems exhibit unique properties traditionally linked to their asymmetric spatial arrangement. Recently, multiple laser pulses were shown to induce purely electronic chiral states without altering the nuclear configuration. Here, we…
In quantum optics, it is common to assume that atoms are point-like objects compared to the wavelength of the electromagnetic field they interact with. However, this dipole approximation is not always valid, e.g., if atoms couple to the…
We develop a family of chiral measures to quantify the chirality of a distribution and assign it a handedness. Our measures are built using the tensorial moments of the distribution, which naturally encode its spatial character, not only…
Light is one of the most powerful and precise tools allowing us to control, shape and create new phases of matter. In this task, the magnetic component of a light wave has so far played a unique role in defining the wave's helicity, but its…
A quantum sensing protocol is proposed for demonstrating the motion-induced chirality of circularly polarised Rydberg atoms. To this end, a cloud of Rydberg atoms is dressed by a bichromatic light field. This allows to exploit the…
Chiral molecules may exist in superpositions of left- and right-handed states. We show how the amplitudes of such superpositions may be teleported to the polarization degrees of freedom of a photon and thus measured. Two experimental…
Chirality, either of light or matter, has proved to be very practical in biosensing and nanophotonics. However, the fundamental understanding of its temporal dynamics still needs to be discovered. A realistic setup for this are the…
Chirality is a fundamental symmetry concept describing discrete states, i.e., left-handed, right-handed, or achiral, and existing at disparate scales and in many categories of scientific fields. Even though symmetry breaking is…
Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…
Chirality is a fundamental feature in all domains of nature, ranging from particle physics over electromagnetism to chemistry and biology. Chiral objects lack a mirror plane and inversion symmetry and therefore cannot be spatially aligned…
Ultrafast imaging of molecular chirality is a key step towards the dream of imaging and interpreting electronic dynamics in complex and biologically relevant molecules. Here, we propose a new ultrafast chiral phenomenon exploiting recent…
Chiral edge currents play an important role in characterizing topological matter. In atoms, they have been observed at such a low temperature that the atomic motion can be measured. Here we report the first experimental observation of…
Chiral excited electronic states of molecules have an intrinsic sense of handedness, or twist, and are the active component in energy efficient display technologies and in new photosynthetic routes to produce pharmaceuticals. Creating…