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Systematically controlling the superconducting transition temperature ($T_\text{c}$) in the bilayer Ruddlesden-Popper nickelate La$_3$Ni$_2$O$_7$ remains a significant challenge. Here, we address this by synthesizing high-quality…

The discovery of the superconductivity in the infinite-layer nickelates, as topotactically reduced from their respective perovskite percussors via co-annealing with CaH2, extends the understanding in superconductivity. Nevertheless, whether…

High-temperature unconventional superconductivity quite generically emerges from doping a strongly correlated parent compound, often (close to) an antiferromagnetic insulator. The recently developed dynamical vertex approximation is a…

Superconductivity · Physics 2024-06-04 Simone Di Cataldo , Paul Worm , Jan Tomczak , Liang Si , Karsten Held

The prediction of high $T_c$ superconductivity in layers of LaNiO$_3$ through orbital engineering has led to extensive research efforts over the last fifteen years. During this period, a plethora of thin films and heterostructures based…

Strongly Correlated Electrons · Physics 2022-05-10 J. Chakhalian , S. Middey

Although rare earth nickelates (ReNiO3) exhibit abundant electronic phases and widely adjustable metal to insulator electronic transition properties, their practical electronic applications are largely impeded by their intrinsic meta…

Materials Science · Physics 2021-11-29 Fengbo Yan , Zhishan Mi , Jinhao Chen , Haiyang Hu , Lei Gao , Jiaou Wang , Nuofu Chen , Yong Jiang , Lijie Qiao , Jikun Chen

The rare-earth nickelates possess a diverse set of collective phenomena including metal-to-insulator transitions, magnetic phase transitions, and, upon chemical reduction, superconductivity. Here, we demonstrate epitaxial stabilization of…

Revealing the momentum-resolved electronic structure of infinite-layer nickelates is essential for understanding this new class of unconventional superconductors, but has been hindered by the formidable challenges in improving the sample…

The mechanism of unconventional superconductivity in correlated materials remains a great challenge in condensed matter physics. The recent discovery of superconductivity in infinite-layer nickelates, as analog to high-Tc cuprates, has…

Motivated by the report of superconductivity in bilayer La$_3$Ni$_2$O$_7$ at high pressure, we examine the interacting electrons in this system. First-principles many-body theory is utilized to study the normal-state electronic properties.…

Strongly Correlated Electrons · Physics 2023-12-04 Frank Lechermann , Jannik Gondolf , Steffen Bötzel , Ilya M. Eremin

The layered square-planar nickelates, Nd$_{n+1}$Ni$_{n}$O$_{2n+2}$, are an appealing system to tune the electronic properties of square-planar nickelates via dimensionality; indeed, superconductivity was recently observed in…

Infinite layer nickelates have garnered significant attention due to their potential for high-temperature superconductivity. Despite extensive research, the interplay between oxygen stoichiometry and electronic properties in infinite layer…

The recent discovery of superconductivity in infinite-layer nickelates generates tremendous research endeavors, but the ground state of their parent compounds is still under debate. Here, we report experimental evidences for the dominant…

Since the discovery of cuprate, the origin of high-T$_c$ superconductivity has been an outstanding puzzle. Recently, high-T$_c$ superconductivity was observed in a bilayer nickelate La$_3$Ni$_2$O$_7$ under pressure, whose structure hosts…

Superconductivity · Physics 2025-05-09 Yuhao Gu , Congcong Le , Zhesen Yang , Xianxin Wu , Jiangping Hu

Recently Li et al (2019 Nature 572 624) discovered a new type of oxide superconductor Nd0.8Sr0.2NiO2 with T$_c$ = 14 K. To classify superconductivity in this infinite-layer nickelate experimental upper critical field, B$_{c2}$(T), and the…

Superconductivity · Physics 2020-05-05 E. F. Talantsev

The infinite-layer structure nickelate Ba$_2$NiO$_2$(AgSe)$_2$ (BNOAS) with $d^8$ Ni ions and a peculiar susceptibility $\chi(T)$ is studied with correlated density functional methods. The overriding feature of the calculations is violation…

Strongly Correlated Electrons · Physics 2020-08-14 Hyo-Sun Jin , W. E. Pickett , K. -W. Lee

We study a model for the metal-insulator (MI) transition in the rare-earth nickelates RNiO$_3$, based upon a negative charge transfer energy and coupling to a rock-salt like lattice distortion of the NiO$_6$ octahedra. Using exact…

Strongly Correlated Electrons · Physics 2014-03-12 Steve Johnston , Anamitra Mukherjee , Ilya Elfimov , Mona Berciu , George A. Sawatzky

The discovery of superconductivity under high pressure with $T_c$ exceeding 80 K in a bilayer nickelate La$_3$Ni$_2$O$_7$ has led to a strong desire to realize similar high $T_c$ phenomena at ambient pressure. As one possible path toward…

Superconductivity · Physics 2025-02-20 Masayuki Ochi , Hirofumi Sakakibara , Hidetomo Usui , Kazuhiko Kuroki

The discovery of superconductivity in the Ruddlesden-Popper (RP) nickelates has opened a new chapter in the search for high superconducting transition temperatures ($T_\mathrm{c}$) materials. A central and puzzling feature of this family is…

A hallmark of many unconventional superconductors is the presence of many-body interactions which give rise to broken symmetry states intertwined with superconductivity. Recent resonant soft x-ray scattering experiments report commensurate…

Motivated by the recent observation of superconductivity in the pressurized trilayer La$_4$Ni$_3$O$_{10}$ Ruddlesden-Popper (RP) nickelate, we explore its structural, electronic, and magnetic properties as a function of hydrostatic pressure…

Superconductivity · Physics 2024-07-19 Harrison LaBollita , Jesse Kapeghian , Michael R. Norman , Antia S. Botana