Related papers: Laser-coolable AcOH$^+$ ion for $\mathcal{CP}$-vio…
We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to $20(3)~\mu\text{K}$ in free space and loaded into an optical dipole trap. We…
The observed baryon asymmetry of the universe (BAU) cannot be explained by the known sources of charge-parity (CP)-violation in the Standard Model (SM). A non-zero permanent electric-dipole-moment (EDM) for fundamental particles, nuclei or…
The energy levels and transition rates of promising laser-cooling candidate thorium anion Th^- have been experimentally obtained in the current work. Three new excited states between the bound-bound electric dipole (E1) transition of Th^-…
Molecular ions formed in cold hybrid ion-atom experiments may find interesting applications ranging from precision measurements to controlled chemical reactions. Here, we investigate electronic structure of the Sr$_2^+$ molecular ion, which…
The discovery of the atomic electric dipole moment (EDM) would reveal the simultaneous violation of parity (P) and time-reversal (T) invariance. The EDM can be induced by T-odd forces between the nucleus and atomic electrons. As the nuclear…
We present a comprehensive study of the electronic transitions in neutral cadmium (Cd I) with a focus on forbidden transitions, motivated by recent advances in laser technology and the growing relevance of cadmium in quantum gas research,…
Searches for the permanent electric dipole moments (EDMs) of molecules, atoms, nucleons and nuclei provide powerful probes of CP violation both within and beyond the Standard Model (BSM). The interpretation of experimental EDM limits…
The prospect of laser cooling of polyatomic molecules has opened a new avenue in the search for the electric dipole moment of the electron (eEDM). An upper bound on the eEDM would probe new physics arising from beyond the Standard Model of…
Atomic clocks based on an Al$^+$ ion sympathetically cooled by a laser-cooled alkaline-earth ion have achieved unprecedented accuracy. Here, we investigate theoretically interactions and charge transfer dynamics of an Al$^+$ ion immersed in…
The electronic structure of the ICl+ molecular ion is investigated by using high-level multireference configuration interaction (MRCI) method. To improve computational accuracy, Davidson corrections, spin-orbit coupling (SOC), and…
If axion simultaneously has the scalar couplings to the nucleons and pseudo-scalar couplings to the electrons, it may mediate a $\mathcal{P}$, $\mathcal{T}$-violating interaction between the electronic shell and nuclei in the molecules. The…
We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…
Multiply charged actinide molecules provide a unique platform to study fundamental physics and the chemical bond under extreme conditions. Beyond the inherently large relativistic effects associated with a high proton number $Z$, an…
We demonstrate that electron electric dipole moment experiments with molecules in paramagnetic state are sensitive to $P,T$-violating nuclear forces and other $CP$-violating parameters in the hadronic sector. These experiments, in…
Laser cooling methods for trapped ions are most commonly studied at low energies, i.e., in the Lamb-Dicke regime. However, ions in experiments are often excited to higher energies for which the Lamb-Dicke approximation breaks down. Here we…
The electric dipole moment of the electron (eEDM) is a signature of CP-violating physics beyond the Standard Model. We describe an ongoing experiment to measure or set improved limits to the eEDM, using a cold beam of thorium monoxide (ThO)…
In the presence of P,T-violating interactions, the exchange of axion-like particles between electrons and nucleons in atoms and molecules induces electric dipole moments (EDMs) of atoms and molecules. We perform calculations of such…
We currently live in the age of the CKM paradigm. The $3\times 3$ matrix that links $(d,\ s,\ b)$ quarks to $(u,\ c,\ t)$ in the charged current weak interaction, being complex and nominally with 18 parameters, can be accounted for by just…
Using the ab initio computed Potential Energy Surface (PES) for the electronic interaction of the MgH$^+$ ($^1\Sigma$) ion with the He($^1$S) atom, we calculate the relevant state-changing rotationally inelastic collision cross sections…
Triatomic molecule RaOH combines the advantages of laser-coolability and the spectrum with close opposite-parity doublets. This makes it a promising candidate for experimental study of the $\mathcal{P}$,$\mathcal{T}$-violation. Previous…