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Push-Pull functional compounds consisting of dicyanorhodanine derivatives have attracted a lot of interest because their optical, electronic, and charge transport properties make them useful as building blocks for organic photovoltaic…

Electron transfer (ET) in molecular donor-acceptor dye systems is crucial for charge transport in organic semiconductors. Classically, ET rates should decrease with increasing donor-acceptor distance while the microscopic mechanism is more…

Linear and nonlinear optical lineshapes reveal details of excitonic structure in semiconductor polymers. We implement absorption, photoluminescence, and transient absorption spectroscopies in DPP-DTT, an electron push-pull copolymer, to…

Tuning the ambipolar behavior in charge carrier transport via defect-engineering is crucial for achieving high mobility transistors for nonlinear logic circuits. Here, we present the electric-field tunable electron and hole transport in a…

The charge transfer integral, site energy and the stacking angle fluctuations are used to study the hole and electron transport in recently synthesized dialkyl substituted thienothiophene caped benzobisthiazole (BDHTT-BBT) and…

Soft Condensed Matter · Physics 2017-05-17 K. Navamani , K. Senthilkumar

We present an investigation of the microscopic interplay between excitons and charge carriers by means of combined photoluminescence (PL) and charge carrier transport measurements on organic thin film transistors (OTFT). For this purpose,…

Materials Science · Physics 2015-06-15 N. H. Hansen , C. Wunderlich , A. K. Topczak , J. Pflaum

Diketopyrrolopyrroles are a popular class of electron-withdrawing unit in optoelectronic materials. When combined with electron donating side-chain functional groups such as thiophenes, they form a very broad class of donor-acceptor…

Using density-functional theory with the hybrid functional B3LYP, we investigate the electronic properties of polymers with diketo-pyrrolo-pyrrole (DPP) unit. We note that some of the polymers studied have LUCO energy similar to the…

Materials Science · Physics 2009-11-03 Simon Lévesque , Paolo E. Trevisanutto , Jean Frédéric Laprade , Michel Cote

Near-room-temperature electronic transport of annealing induced semiconducting crystallites embedded within its amorphous counterpart is treated within the effective-medium approach. As such, the mixtures transport coefficients become…

Mesoscale and Nanoscale Physics · Physics 2019-04-23 David Emin

The electronic transport of electrons and holes through stacks of $\alpha$,$\ome ga$-dicyano-$\beta$,$\beta$'-dibutyl- quaterthiophene (DCNDBQT) as part of a nov el organic ferroic field-effect transistor (OFFET) is investigated. The novel…

Materials Science · Physics 2015-05-14 T. Kunze , S. Gemming , V. Pankoke , K. Morawetz , R. Luschtinetz , G. Seifert

Chiral perovskites are emerging semiconducting materials with broken symmetry that can selectively absorb and emit circularly polarized light. However, most of the chiral perovskites are typically low-dimensional structures with limited…

Controlling the nonlinear optical (NLO) response properties at the molecular level is a key to develop strong NLO active materials for technological applications. In this paper, we report quantum chemical investigation of NLO response…

Chemical Physics · Physics 2017-02-24 Ramprasad Misra

The anisotropic charge carrier mobilities of two phenancene series compounds such as dibenzo[a,c]picene (DBP) and tribenzo[a,c,k]tetraphene (TBT) is investigated based on the first-principle calculations and Marcus-Hush theory. The…

Chemical Physics · Physics 2019-10-28 Smruti R. Sahoo , Rudranarayan Khatua , Suryakanti Debata , Sagar Sharma , Sridha Sahu

Charge transfer complexes are materials with a wide range of interesting optical and electronic properties. They have seen a great deal of research over the past decade, both in device development as well as research to elucidate the…

Materials Science · Physics 2024-06-04 Satwik Ramanjanappa , Edward R Van Keuren

The exciton transport in the prototypical organic semiconductor Di-Indeno-Perylene (DIP) has been investigated by means of photoluminescence (PL) quenching and interpreted by an advanced exciton diffusion model including interference…

Materials Science · Physics 2012-07-05 A. K. Topczak , T. Roller , B. Engels , W. Brütting , J. Pfaum

We theoretically study the electronic transport in the monolayer of dithiolated phenylene vinylene oligomeres coupled to the (111) surfaces of gold electrodes. We use non-equilibrium Green functions (NEGF) and density functional theory(DFT)…

Materials Science · Physics 2009-11-10 Z. Crljen , A. Grigoriev , G. Wendin , K. Stokbro

The systematic trends in structural and electronic properties of perylene diimide (PDI) derived dye molecules have been investigated by DFT calculations based on projector augmented wave (PAW) method including gradient corrected…

Materials Science · Physics 2008-01-15 E. Mete , D. Uner , M. Cakmak , O. Gulseren , S. Ellialtioglu

The family of hybrid organic-inorganic lead-halide perovskites are the subject of intense interest for optoelectronic applications, from light-emitting diodes to photovoltaics to X-ray detectors. Due to the inert nature of most organic…

There is a resurgence of interest in the electronic structure of perylene for its applications in molecular devices such as organic photovoltaics and organic light emitting diodes. In this study, we have obtained the low-lying singlet…

Strongly Correlated Electrons · Physics 2018-11-21 Geetanjali Giri , Suryoday Prodhan , Y. Anusooya Pati , S. Ramasesha

This study systematically investigates the regulation mechanisms of backbone topology (tri-/tetracyclic arenes), substitution positions, and functional groups on charge transport properties through molecular design of…

Chemical Physics · Physics 2025-05-28 Zhipeng Tong , Xiaoqi Sun , Guiya Qin , Jinpu Bai , Qi Zhao , Aimin Ren , Jingfu Guo
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