English
Related papers

Related papers: Photoelectron Circular Dichroism of a Model Anioni…

200 papers

We show that the photoelectron angular distributions produced by elliptical and cross-polarized two-color laser fields interacting with randomly oriented chiral molecules decompose into four irreducible representations of the $D_{2h}$ point…

Circular dichroism (CD) is in widespread use as a means of determining enantiomeric excess. We show how slow-light phenomena in dispersive structured media allow for a reduction in the required optical path length of an order of magnitude.…

Optics · Physics 2007-11-19 Jesper Pedersen , Niels Asger Mortensen

We introduce a matrix method and we derive a formula for phase retardation effects in plasmonic systems. We analyze the circular dichroic response (CD) of two orthogonal Au nanorods in detail and we show that, although, theoretically,…

Optics · Physics 2020-11-30 M. A. Kuntman , E. Kuntman

Chirality, a fundamental concept describing an object cannot superpose with its mirror image, is crucial in optics and photonics and leads to various exotic phenomena, such as circular dichroism, and optical activity. Recent findings reveal…

Optics · Physics 2025-01-13 Shijie Kang , Haitao Li , Jiayu Fan , Jiusi Yu , Boyang Qu , Peng Chen , Xiaoxiao Wu

The electron and ion properties observed in a photoionization inherit a symmetry properties of both a target and a radiation. Introducing a symmetry breaking in a photoionization process one can expect to observe a noticeable variation of…

Atomic Physics · Physics 2024-02-09 Maksim D. Kiselev , Elena V. Gryzlova , Alexei N. Grum-Grzhimailo

We discuss how tensorial observables, available in photoelectron angular distributions resulting from interaction between isotropic chiral samples and cross polarized $\omega$-$2\omega$ bichromatic fields, allow for chiral discrimination…

Atomic Physics · Physics 2022-06-28 Andres F. Ordonez , Olga Smirnova

The photoionization of a two-shell endohedral A@CN1@CN2 is considered. Formulas are presented for cross-sections and angular anisotropy parameters, both dipole and non-dipole. The effect of the fullerenes shell upon photoelectron from atom…

Atomic and Molecular Clusters · Physics 2013-05-29 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

Photoemission electron microscopy (PEEM) has evolved into an indispensable tool for structural and magnetic characterization of surfaces at the nanometer scale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a leading…

We employ ptychography, a phase-retrieval imaging technique, to show experimentally for the first time that a partially coherent high-energy matter (electron) wave emanating from an extended source can be decomposed into a set of mutually…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 S. Cao , P. Kok , P. Li , A. M. Maiden , J. M. Rodenburg

In the classical model of atomic polarizability, atomic charges are displaced by an applied electric field, assuming the electron cloud remains spherically symmetric but with its center shifted from the nucleus, thereby inducing an electric…

Classical Physics · Physics 2025-02-11 O. F. de Alcantara Bonfim

Molecular Circular dichroism (CD) spectroscopy faces significant limitations due to the inherent weakness of chiroptical light-matter interactions. In this view, resonant optical antennas constitute a promising solution to this problem…

Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…

We consider high energy electron scattering by hydrogen atoms in the presence of a laser field of moderate power and higher frequencies. If the field is a superposition of a linearly and a circularly polarized laser beam in a particular…

Atomic Physics · Physics 2013-03-07 Aurelia Cionga , Fritz Ehlotzky , Gabriela Zloh

Increasing the sensitivity of chiral spectroscopic techniques such as circular dichroism (CD) spectroscopy is a current aspiration in the research field of nanophotonics. Enhancing CD spectroscopy depends upon of two complementary…

We demonstrate that chiral response can be achieved in resonant metasurfaces with a monoclinic lattice symmetry (the so-called Bravais oblique lattices) where the mirror symmetry is broken by the lattice asymmetry and also by a substrate,…

Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation (SHG) response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole (E1) and…

Strongly Correlated Electrons · Physics 2019-12-11 S. W. Lovesey , G. van der Laan

Distinct selectivity to the spin angular momenta of photons have garnered significant attention in recent years, for their relevance in basic science and for imaging and sensing applications. While nonlocal metasurfaces with strong chiral…

Optics · Physics 2025-07-04 Minho Choi , Andrea Alù , Arka Majumdar

Controlling and channelling light emissions from unpolarized quantum dots into specific directions with chiral polarization remains a key challenge in modern photonics. Stacked metasurface designs offer a potential compact solution for…

Single-layer transition-metal dichalcogenides provide an unique intrinsic entanglement between the spin/valley/orbital degrees of freedom and the polarization of scattered photons. This scenario gives rise to the well-assessed optical…

Materials Science · Physics 2025-01-13 Habib Rostami , Federico Cilento , Emmanuele Cappelluti