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We present a comprehensive optical study of the excitonic Zeeman effects in transition metal dichalcogenide monolayers, which are discussed comparatively for selected materials: MoSe$_2$, WSe$_2$ and WS$_2$. We introduce a simple…

Mesoscale and Nanoscale Physics · Physics 2018-03-02 M. Koperski , M. R. Molas , A. Arora , K. Nogajewski , M. Bartos , J. Wyzula , D. Vaclavkova , P. Kossacki , M. Potemski

A direct band gap, remarkable light-matter coupling as well as strong spin-orbit and Coulomb interaction establish two-dimensional (2D) crystals of transition metal dichalcogenides (TMDs) as an emerging material class for fundamental…

The optical properties of molecular crystals are largely determined by the excitonic coupling of neighboring molecules. This coupling is extremely sensitive to the arrangement of adjacent molecular units, as their electronic interaction is…

Excitons in monolayer transition metal dichalcogenide are endowed with intrinsic valley-orbit coupling between their center-of-mass motion and valley pseudospin. When trapped in a confinement potential, e.g., generated by strain field, we…

Mesoscale and Nanoscale Physics · Physics 2023-05-11 Di Zhang , Sha Deng , Dawei Zhai , Wang Yao , Qizhong Zhu

Single layers of transition metal dichalcogenides (TMDs) are direct gap semiconductors with nondegenerate valley indices. An intriguing possibility for these materials is the use of their valley index as an alternate state variable. Several…

We study theoretically the electron dynamics of transition metal dichalcogenide quantum dots in the field of an ultrashort and ultrafast circularly polarized optical pulse. The quantum dots have the shape of a disk and their electron…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Aranyo Mitra , Ahmal Jawad Zafar , Vadym Apalkov

Monolayers of transition metal dichalcogenides present an intriguing platform to investigate the interplay of excitonic complexes in two dimensional semiconductors. Here, we use optical spectroscopy to study light-matter coupling and…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Jonas Zipfel , Koloman Wagner , Jonas D. Ziegler , Takashi Taniguchi , Kenji Watanabe , Marina A. Semina , Alexey Chernikov

Motivated by the triumph and limitation of graphene for electronic applications, atomically thin layers of group VI transition metal dichalcogenides are attracting extensive interest as a class of graphene-like semiconductors with a desired…

Mesoscale and Nanoscale Physics · Physics 2013-04-17 Hualing Zeng , Gui-Bin Liu , Junfeng Dai , Yajun Yan , Bairen Zhu , Ruicong He , Lu Xie , Shijie Xu , Xianhui Chen , Wang Yao , Xiaodong Cui

Moir\'e superlattices created by stacking atomic layers of transition metal dichalcogenide semiconductors have emerged as a class of fascinating artificial photonic and electronic materials. An appealing attribute of these structures is the…

Mesoscale and Nanoscale Physics · Physics 2025-03-11 Yueh-Chun Wu , Matthew DeCapua , ZhongChen Xu , Takashi Taniguchi , Kenji Watanabe , YouGuo Shi , Jun Yan

Monolayer transition metal dichalcogenides (TMDCs) constitute the core group of materials in the emerging semiconductor technology of valleytronics. While the coupled spin-valley physics of pristine TMDC materials and their heterstructures…

Mesoscale and Nanoscale Physics · Physics 2023-11-14 Chumki Nayak , Suvadip Masanta , Sukanya Ghosh , Shubhadip Moulick , Atindra Nath Pal , Indrani Bose , Achintya Singha

Monolayer semiconducting transition metal dichalcogenides possess broken inversion symmetry and strong spin-orbit coupling, which leads to unique spin-valley locking effect. In 2H stacked pristine multilayers, the spin-valley locking yields…

Mesoscale and Nanoscale Physics · Physics 2023-06-07 Yinong Zhang , Chengxin Xiao , Dmitry Ovchinnikov , Jiayi Zhu , Xi Wang , Takashi Taniguchi , Kenji Watanabe , Jiaqiang Yan , Wang Yao , Xiaodong Xu

The spectral signatures associated with different negatively charged exciton complexes (trions) in a WS$_2$ monolayer encapsulated in hBN, are analyzed from low temperature and polarization resolved reflectance contrast (RC) and…

We analyze magnetic phases of monolayers of transition metal dichalcogenides that are two-valley materials with electron-electron interactions. The exchange inter-valley scattering makes two-valley systems less stable to the spin…

Strongly Correlated Electrons · Physics 2019-07-31 Dmitry Miserev , Jelena Klinovaja , Daniel Loss

The coupled spin-valley physics in transition metal dichalcogenides (TMDs) endows exciton states with valley degrees of freedom, making them promising for valleytronic applications in TMDs monolayers and/or their heterostructures. Although…

Applied Physics · Physics 2022-12-07 Yingying Chen , Zeyi Liu , Junchao Hu , Junze Li , Wendian Yao , Dehui Li

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual…

Tungsten-based monolayer transition metal dichalcogenides host a long-lived dark exciton, an electron-hole pair in a spin-triplet configuration. The long lifetime and unique spin properties of the dark exciton provide exciting opportunities…

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

Excitonic semiconductors such as transition metal dichalcogenides (TMDCs) are attractive for next-generation photovoltaics (PVs) with low cost, light weight, and low material consumption. In WS2 and other TMDCs, the simultaneous large…

Optics · Physics 2024-10-22 Adam D. Alfieri , Tobia Ruth , Cheryl Lim , Jason Lynch , Deep Jariwala

We study theoretically the Coulomb interaction between excitons in transition metal dichalcogenide (TMD) monolayers. We calculate direct and exchange interaction for both ground and excited states of excitons. The screening of the Coulomb…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 V. Shahnazaryan , I. Iorsh , I. A. Shelykh , O. Kyriienko

Monolayer transition-metal dichalcogenides possess a pair of degenerate helical valleys in the band structure that exhibit fascinating optical valley polarization. Optical valley polarization, however, is limited by carrier lifetimes of…

Materials Science · Physics 2015-09-16 Jingshan Qi , Xiao Li , Qian Niu , Ji Feng
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