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We show that, because of the inevitable twist and lattice mismatch in heterobilayers of transition metal dichalcogenides, interlayer excitons have six-fold degenerate light cones anomalously located at finite velocities on the parabolic…

Mesoscale and Nanoscale Physics · Physics 2015-11-05 Hongyi Yu , Yong Wang , Qingjun Tong , Xiaodong Xu , Wang Yao

We present a comprehensive theoretical investigation of the photo-generated excitons in transition-metal dichalcogenide monolayers (TMD-ML's) by Laguerre-Gaussian beams, a celebrated kind of twisted lights (TL's) carrying quantized orbital…

Mesoscale and Nanoscale Physics · Physics 2022-03-07 Guan-Hao Peng , Oscar Javier Gomez Sanchez , Wei-Hua Li , Ping-Yuan Lo , Shun-Jen Cheng

Excitons, composite electron-hole quasiparticles, are known to play an important role in optoelectronic phenomena in many semiconducting materials. Recent experiments and theory indicate that the band-gap optics of the newly discovered…

Mesoscale and Nanoscale Physics · Physics 2015-09-02 Yuri N. Gartstein , Xiao Li , Chuanwei Zhang

The electron-hole exchange interaction is a fundamental mechanism that drives valley depolarization via intervalley exciton hopping in semiconductor multi-valley systems. Here, we report polarization-resolved photoluminescence spectroscopy…

Understanding the ultrafast coupling and relaxation mechanisms between valleys in transition metal dichalcogenide semiconductors is of crucial interest for future valleytronic devices. Recent ultrafast pump-probe experiments showed an…

In this letter, we address the chiral properties of valley exciton-polaritons in a monolayer of WS2 in the regime of strong light-matter coupling with a Tamm-Plasmon resonance. We observe that the valley polarization, which manifests in the…

Mesoscale and Nanoscale Physics · Physics 2017-12-13 N. Lundt , S. Stoll , P. Nagler , A. Nalitov , S. Klembt , S. Betzold , J. W. Goddard , E. Frieling , A. V. Kavokin , C. Schüller , T. Korn , S. Höfling , C. Schneider

Chiral light-matter interactions can enable polarization to control the direction of light emission in a photonic device. Most realizations of chiral light-matter interactions require external magnetic fields to break time-reversal symmetry…

Optics · Physics 2019-07-19 Zhili Yang , Shahriar Aghaeimeibodi , Edo Waks

The coupling between spin, charge, and lattice degrees of freedom plays an important role in a wide range of fundamental phenomena. Monolayer semiconducting transitional metal dichalcogenides have emerged as an outstanding platform for…

Chiral interaction between light and two-dimensional transition metal dichalcogenides (2D-TMDs) has recently drawn enormous scientific attention. The optical selection rules of these atomically thin semiconductors allow the attribution of a…

Optics · Physics 2021-06-08 Irina Komen , Sabrya E. van Heijst , Sonia Conesa-Boj , L. Kuipers

Single layers of transition metal dichalcogenides are two-dimensional direct bandgap semiconductors with degenerate, but inequivalent, `valleys' in the electronic structure that can be selectively excited by polarized light. Coherent…

Materials Science · Physics 2017-07-21 Yen-Jung Chen , Jeffrey D. Cain , Teodor K. Stanev , Vinayak P. Dravid , Nathaniel P. Stern

Monolayer transition metal dichalcogenides (TMDs) exhibit a remarkably strong Coulomb interaction that manifests in tightly bound excitons. Due to the complex electronic band structure exhibiting several spin-split valleys in the conduction…

Degenerate extrema in the energy dispersion of charge carriers in solids, also referred to as valleys, can be regarded as a binary quantum degree of freedom, which can potentially be used to implement valleytronic concepts in van der Waals…

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Exciton optical transitions in transition-metal dichalcogenides offer unique opportunities to study rich many-body physics. Recent experiments in monolayer WSe$_2$ and WS$_2$ have shown that while the low-temperature photoluminescence from…

Materials Science · Physics 2016-08-23 Hanan Dery

Local energy extrema of the bands in momentum space, or valleys, can endow electrons in solids with pseudo-spin in addition to real spin. In transition metal dichalcogenides this valley pseudo-spin, like real spin, is associated with a…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Grant Aivazian , Zhirui Gong , Aaron M Jones , Rui-Lin Chu , Jiaqiang Yan , David G Mandrus , Chuanwei Zhang , David Cobden , Wang Yao , Xiaodong Xu

Optical spectroscopy in high magnetic fields $B\leq65$ T is used to reveal the very different nature of carriers in monolayer and bulk transition metal dichalcogenides. In monolayer WSe$_{2}$, the exciton emission shifts linearly with the…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 A. A. Mitioglu , P. Plochocka , Á. Granados del Aguila , P. C. M. Christianen , G. Deligeorgis , S. Anghel , L. Kulyuk , D. K. Maude

We present photoluminescence measurements in monolayer WSe$_2$, which point to the importance of the interaction between charged particles and excitonic complexes. The theoretical analysis highlights the key role played by exchange…

Materials Science · Physics 2022-02-15 Min Yang , Lei Ren , Cedric Robert , Dinh Van Tuan , Laurent Lombez , Bernhard Urbaszek , Xavier Marie , Hanan Dery

A monolayer of a transition metal dichalcogenide (TMD) such as WSe$_2$ is a two-dimensional (2D) direct band-gap valley-semiconductor having an effective Honeycomb lattice structure with broken inversion symmetry. The inequivalent valleys…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Ajit Srivastava , Meinrad Sidler , Adrien V. Allain , Dominik S. Lembke , Andras Kis , Atac Imamoglu

We examine the full static non-linear optical response of uniaxially strained transition metal dichalcogenide monolayers doped with a finite carrier density in the conduction band, in the presence of disorder. We find that the customary…

Mesoscale and Nanoscale Physics · Physics 2022-05-23 Reza Asgari , Dimitrie Culcer

The variety of excitonic states in tungsten-based dichalcogenide monolayers stems from unique interplay between the spin and valley degrees of freedom. One of the exciton species is the indirect exciton (momentum or valley dark), which is…

Mesoscale and Nanoscale Physics · Physics 2022-08-23 Pengke Li , Cedric Robert , Dinh Van Tuan , Lei Ren , Xavier Marie , Hanan Dery