Related papers: Structural Origin of Boson Peak in Glasses
The boson peak appears in all amorphous solids and is an excess of vibrational states at low frequencies compared to the phonon spectrum of the corresponding crystal. Until recently, the consensus was that it originated from "defects" in…
A hallmark of glasses is an excess of low-frequency, nonphononic vibrations, in addition to phonons. It is associated with the intrinsically nonequilibrium and disordered nature of glasses, and is generically manifested as a THz peak -- the…
The boson peak (BP) is a universal feature in the Raman and inelastic scattering spectra of both disordered and crystalline materials. The current paradigm presents the boson peak as the result of a Ioffe-Regel crossover between ballistic…
The Boson peak is believed to be the key to the fundamental understanding of the anomalous thermodynamic properties of glasses, notably the anomalous peak in the heat capacity at low temperatures; it is believed to be due to an excess of…
We propose that the boson peak originates from the (quasi-) localized vibrational modes associated with long-lived locally favored structures, which are intrinsic to a liquid state and are randomly distributed in a sea of normal-liquid…
The inelastic scattering intensities of glasses and amorphous materials has a maximum at a low frequency, the so called Boson peak. Under applied hydrostatic pressure, $P$, the Boson peak frequency, $\omega_{\rm b}$, is shifted upwards. We…
Using the example of a two-dimensional macroscopic model glass in which the interparticle forces can be precisely measured, we obtain strong hints for resolving a controversy concerning the origin of the anomalous enhancement of the…
Vibrational spectra of proteins and topologically disordered solids display a common anomaly at low frequencies, known as Boson peak. We show that such feature in globular proteins can be deciphered in terms of an energy landscape picture,…
Despite extensive theoretical \cite{GanterPRL1998, ElliotPRL2001,SchirmacherPRL2007, TanakaNatureM2008, MonacoPNAS2009, MarruzzoSCIRP2013} and experimental studies \cite{ChumakovPRL2011, ChumakovPRL2014, KayaScience2010,KChenPRL2010,…
We present a novel analytical model for glasses, starting from the first principle that the disorder in a glass mimics the disorder in a fluid. The origin of the boson peak is attributed to the intrinsically noncommutative geometry of the…
The vibrational anomalies of glasses, in particular the boson peak, are addressed from the standpoint of heterogeneous elasticity, namely the spatial fluctuations of elastic constants caused by the structural disorder of the amorphous…
The vibrational spectra of solids, both ordered and amorphous, in the low-energy regime, control the thermal and transport properties of materials, from heat capacity to heat conduction, electron-phonon couplings, conventional…
Glasses are amorphous solids, in the sense that they display elastic behaviour. In crystals, elasticity is associated with phonons, quantized sound-wave excitations. Phonon-like excitations exist also in glasses at very high frequencies…
The high-frequency excitations in glasses and supercooled liquids belong to the great mysteries of the physics of condensed matter. While the fast process, located at GHz-THz, can be interpreted as encaged molecular motion, the occurrence…
In glasses, atomic disorder combined with atomic connectivity makes understanding of the nature of the vibrations much more complex than in crystals or molecules. With a simple model, however, it is possible to show how disorder generates…
The emergence of excess vibrational modes over the Debye prediction, typically manifested as the well-known boson peak in the plot of vibrational density of states scaled by the Debye prediction, has become a hallmark of various amorphous…
The dynamics of a soft sphere model glass, studied by molecular dynamics, is investigated. The vibrational density of states divided by $\omega^2$ shows a pronounced boson peak. Its shape is in agreement with the universal form derived for…
A hallmark of structural glasses and other disordered solids is the emergence of excess low-frequency vibrations, on top of the Debye spectrum $D_{\rm Debye}(\omega)$ of phonons ($\omega$ denotes the vibrational frequency), which exist in…
It is well known that amorphous solids display a phonon spectrum where the Debye $\sim \omega^2$ law at low frequency melds into an anomalous excess-mode peak (the boson peak) before entering a quasi-localized regime at higher frequencies…
We show that the same physical mechanism is fundamental for two seemingly different phenomena such as the formation of two-level systems in glasses and the Boson peak in the reduced density of low-frequency vibrational states g(w)/w^2. This…