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Related papers: Theoretical Challenges in Polaritonic Chemistry

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Polaritonic crystals - periodic structures where the hybrid light-matter waves called polaritons can form Bloch states - promise a deeply subdiffractional nanolight manipulation and enhanced light-matter interaction. In particular,…

Topological polaritons characterized by light-matter interactions have become a pivotal platform in exploring new topological phases of matter. Recent theoretical advances unveiled a novel mechanism for tuning topological phases of…

Polaritons, arising from the strong coupling between excitons and photons within microcavities, hold promise for optoelectronic and all-optical devices. They have found applications in various domains, including low-threshold lasers and…

Dynamic manipulation of arbitrary light polarization is of fundamental importance for versatile optical functionalities, yet realizing such full-Poincar\'e-sphere control within compact nanophotonic architectures remains a formidable…

Plasmonic nanocavities form very robust sub-nanometer gaps between nanometallic structures and confine light in deep subwavelength volumes to enable unprecedented control on light-matter interactions. However, spherical nanoparticles…

Conventional approaches to probing ultrafast molecular dynamics rely on the use of synchronized laser pulses with a well-defined time delay. Typically, a pump pulse excites a wavepacket in the molecule. A subsequent probe pulse can then…

Mesoscale and Nanoscale Physics · Physics 2020-03-27 R. E. F. Silva , Javier del Pino , Francisco J. García-Vidal , Johannes Feist

We consider a semiconductor polymer chain coupled to a single electromagnetic mode in a cavity. The excitations of the chain have a mixed exciton-photon character and are described as polaritons. Polaritons are coupled to the lattice by the…

Mesoscale and Nanoscale Physics · Physics 2007-06-13 M. V. Katkov , Y. V. Pershin , C. Piermarocchi

Polarization of photons plays a key role in quantum optics and light-matter interactions, however, it is difficult to control in nanosystems since the eigenstate of a nanophotonic cavity is usually fixed and linearly polarized. Here we…

When mid-infrared light interacts with nanoscale polar dielectric structures optical phonon propagation cannot be ignored, leading to a rich nonlocal phenomenology which we have only recently started to uncover. In properly crafted…

Mesoscale and Nanoscale Physics · Physics 2021-08-10 Christopher R. Gubbin , Simone De Liberato

Resonant interaction between excitonic transitions of molecules and localized electromagnetic field allows the formation of hybrid light-matter polaritonic states. This hybridization of the light and the matter states has been shown to be…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 Dmitriy Dovzhenko , Maksim Lednev , Konstantin Mochalov , Ivan Vaskan , Yury Rakovich , Igor Nabiev

Systems with strong light-matter interaction opens up new avenues for studying topological phases of matter. Examples include exciton-polaritons, mixed light-matter quasiparticles, where the topology of the polaritonic band structure arises…

Optics · Physics 2023-02-08 Li He , Jingda Wu , Jicheng Jin , Eugene J. Mele , Bo Zhen

We revisited the intersubband polaritonics - the branch of mesoscopic physics having a huge potential for optoelectronic applications in the infrared and terahertz domains - and found that, contrary to the general opinion, the Coulomb…

Materials Science · Physics 2013-03-05 Oleksandr Kyriienko , Ivan A. Shelykh

Cavity-polaritons in semiconductor photonic structures have emerged as a test bed for exploring non-equilibrium dynamics of quantum fluids in an integrated solid-state device setting. Several recent experiments demonstrated the potential of…

Mesoscale and Nanoscale Physics · Physics 2013-12-04 Benjamin Besga , Cyril Vaneph , Jakob Reichel , Jerome Esteve , Andreas Reinhard , Javier Miguel-Sanchez , Atac Imamoglu , Thomas Volz

The ability to actively tune the properties of a nanocavity is crucial for future applications in photonics and quantum information. Two important man-made classes of materials have emerged to mold the flow of electromagnetic waves.…

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…

Harnessing strong light-matter interactions to control chemical reactions in confined electromagnetic fields offers a promising route toward deepening our understanding of chemical dynamics at the collective quantum-mechanical level, with…

Chemical Physics · Physics 2026-01-21 Yaling Ke

We present a new methodology to calculate the strong light-matter coupling between photonic modes in microcavities and large molecular aggregates that consist of hundreds of molecular fragments. To this end, we combine our fragment…

Chemical Physics · Physics 2024-07-30 Richard Einsele , Luca Nils Philipp , Roland Mitrić

Polariton chemistry may provide a new means to control molecular reactivity, permitting remote, reversible modification of reaction energetics, kinetics, and product yields. A considerable body of experimental and theoretical work has…

Chemical Physics · Physics 2023-10-26 Ashley P. Fidler , Liying Chen , Alexander M. McKillop , Marissa L. Weichman

We introduce crystal polaritons, hybrid excitations formed when the collective excitations of a periodic quantum-emitter array strongly couple to the resonant Bloch modes of a metasurface. This realizes a cavity-QED platform in which…

Polaritons - hybrid light-matter states formed in cavity - strongly change the properties of the underlying matter. In optical or plasmonic nanocavities, polaritons decay by radiative emission of the cavity, which is accessible…

Chemical Physics · Physics 2022-10-19 Csaba Fábri , Gábor J. Halász , Lorenz S. Cederbaum , Ágnes Vibók