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Particle plasmons in metal nanoparticles have primarily been investigated through the use of local optical response approximations. However, as nanoparticle size approaches the average distance of electrons to the metal surface, mesoscopic…

Optics · Physics 2023-06-28 Weixiang Ye

We analyze the impact of nonlocality on the waveguide modes of metallo-dielectric multilayers and optical patch antennas, the latter formed from metal strips closely spaced above a metallic plane. We model both the nonlocal effects…

Optics · Physics 2015-06-12 Antoine Moreau , Cristian Ciracì , David R. Smith

Non-local effects in the optical response of noble metals are shown to produce significant blueshift and near-field quenching of plasmons in nanoparticle dimers, nanoshells, and thin metal waveguides. Compared with a local description…

Other Condensed Matter · Physics 2012-11-13 F. Javier Garcia de Abajo

Surface plasmons on metals can concentrate light into sub-nanometric volumes and on these near atomic length scales the electronic response at the metal interface is smeared out over a Thomas-Fermi screening length. This nonlocality is a…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Yu Luo , A. I. Fernandez-Dominguez , Aeneas Wiener , S. A. Maier , J. B. Pendry

We report theoretical evidence that bulk nonlinear materials weakly interacting with highly localized plasmonic modes in ultra-sub-wavelength metallic nanostructures can lead to nonlinear effects at the single plasmon level in the visible…

Mesoscale and Nanoscale Physics · Physics 2017-04-27 Filippo Alpeggiani , Stefania D'Agostino , Daniele Sanvitto , Dario Gerace

We provide theoretical and numerical tools to quantitatively study the impact of nonlocality arising from free electrons in metals on the optical properties of metallo-dielectric multilayers. Though effects due to nonlocality are in general…

In this paper we analyze the effects of nonlocality on the optical properties of a system consisting of a thin metallic film separated from a graphene sheet by a hexagonal boron nitride (hBN) layer. We show that nonlocal effects in the…

Recent experiments have shown that spatial dispersion may have a conspicuous impact on the response of plasmonic structures. This suggests that in some cases the Drude model should be replaced by more advanced descriptions that take spatial…

The nonclassical modification of plasmon-assisted fluorescence enhancement is theoretically explored by placing two-level dipole emitters at the narrow gaps encountered in canonical plasmonic architectures, namely dimers and trimers of…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Christos Tserkezis , N. Asger Mortensen , Martijn Wubs

Geometrical singularities in plasmonic metasurfaces have recently been proposed for the enhancement of light-matter interactions, owing to their broadband light-harvesting properties and extreme plasmon confinement. However, the large…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Fan Yang , Emanuele Galiffi , Paloma Arroyo Huidobro , John Pendry

Nonlocal effects have been shown to be responsible for a variety of non-trivial optical effects in small-size plasmonic nanoparticles, beyond classical electrodynamics. However, it is not clear whether optical mode descriptions can be…

We develop a consistent quantum description of surface plasmons interacting with quantum emitters and external electromagnetic field. Within the framework of macroscopic electrodynamics in dispersive and absorptive medium, we derive, in the…

Mesoscale and Nanoscale Physics · Physics 2021-01-21 Tigran V. Shahbazyan

The effect of nonlocality on the optical response of metals lies at the forefront of research in nanoscale physics and, in particular, quantum plasmonics. In alkali metals, nonlocality manifests predominantly as electron density spill-out…

Mesoscale and Nanoscale Physics · Physics 2025-03-06 Ida Juliane Bundgaard , Christian Nicolaisen Hansen , P. Elli Stamatopoulou , Christos Tserkezis

The plasmon response of metallic nanostructures is anticipated to exhibit nonlocal dynamics of the electron gas when exploring the true nanoscale. We extend the local-response approximation (based on Ohm's law) to account for a general…

Mesoscale and Nanoscale Physics · Physics 2014-03-04 N. Asger Mortensen

Inspired by recent measurements on individual metallic nanospheres that can not be explained with traditional classical electrodynamics, we theoretically investigate the effects of nonlocal response by metallic nanospheres in three distinct…

Mesoscale and Nanoscale Physics · Physics 2014-03-07 Thomas Christensen , Wei Yan , Søren Raza , Antti-Pekka Jauho , N. Asger Mortensen , Martijn Wubs

High spatial and energy resolution EELS can be employed for detailed characterization of both localized and propagating surface plasmon excitations supported by metal nanostructures, giving insight into fundamental physical phenomena…

In tiny metallic nanostructures, quantum confinement and nonlocal response change the collective plasmonic behavior with important consequences for e.g. field-enhancement and extinction cross sections. We report on our most recent…

Optics · Physics 2012-09-07 N. A. Mortensen , G. Toscano , S. Raza , N. Stenger , W. Yan , A. -P. Jauho , S. Xiao , M. Wubs

Herein, we investigate the optical properties of quantum plasmonic metasurfaces composed of metallic nano-objects with subnanometer gaps according to the time-dependent density functional theory, a fully quantum mechanical approach. When…

Optics · Physics 2019-06-17 Takashi Takeuchi , Masashi Noda , Kazuhiro Yabana

We analyze electromagnetic modes in multi-layered nano-composites and demonstrate that the response of a majority of realistic layered structures is strongly affected by the non-local effects originating from strong field oscillations…

A rigorous account of quantum nonlocal effects is paramount for understanding the optical response of metal nanostructures and for designing plasmonic devices at the nanoscale. Here, we present a scheme for retrieving the quantum surface…

Mesoscale and Nanoscale Physics · Physics 2023-09-06 P. A. D. Gonçalves , F. Javier García de Abajo
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