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In order to explore the effects of high levels of electron correlation on the real-time coupled cluster formalism and algorithmic behavior, we introduce a time-dependent implementation of the CC3 singles, doubles and approximate triples…

Chemical Physics · Physics 2025-01-23 Zhe Wang , Håkon Emil Kristiansen , Thomas Bondo Pedersen , T. Daniel Crawford

We perform a systematic exact diagonalization study of spin-orbit coupling effects for stationary few-electron states confined in quasi two-dimensional double quantum dots. We describe the spin-orbit-interaction induced coupling between…

Mesoscale and Nanoscale Physics · Physics 2010-06-17 M. P. Nowak , B. Szafran

Two-electron charged self-assembled quantum dot molecules exhibit a decoherence-avoiding singlet-triplet qubit subspace and an efficient spin-photon interface. Here, we demonstrate that the cycling transitions originating from auxiliary…

Mesoscale and Nanoscale Physics · Physics 2015-09-15 Y. L. Delley , M. Kroner , S. Faelt , W. Wegscheider , A. İmamoğlu

Unitary Coupled Cluster (UCC) theory is a promising variational method for electronic structure calculations, especially for strongly correlated systems and quantum computers. However, its practical application is limited by the steep…

Chemical Physics · Physics 2026-02-05 Prateek Vaish , Brenda Rubenstein

The Coupled Cluster (CC) method is used to compute the electronic correlation energy in atoms and molecules and often leads to highly accurate results. However, due to its single-reference nature, standard CC in its projected form fails to…

Bethe-Salpeter equation is applied to $p$-$p$ elastic scattering. The observables of spin are calculated in the framework of the M matrix using the two-body interaction potential. The parameter of the pseudovector coupling constant is…

Nuclear Theory · Physics 2015-08-27 Susumu Kinpara

We develop a systematic approach to deriving addition theorems for, and some other bilocal sums of, spin spherical harmonics. In this first part we establish some necessary technical results. We discuss the factorization of orbital and spin…

Mathematical Physics · Physics 2013-06-13 Antonio O. Bouzas

We present a formulation and implementation of second-order quasidegenerate N-electron valence perturbation theory (QDNEVPT2) that provides a balanced and accurate description of spin-orbit coupling and dynamic correlation effects in…

Chemical Physics · Physics 2024-06-19 Rajat Majumder , Alexander Yu. Sokolov

A microscopic description of nuclei is important to understand the nuclear shell-model from fundamental principles. This is difficult to achieve for more than the lightest nuclei without an effective approximation scheme. The purpose of…

Nuclear Theory · Physics 2013-08-19 Gustav R. Jansen

This paper examines the properties of the self-energy operator in lattice-matched semiconductor heterostructures, focusing on nonanalytic behavior at small values of the crystal momentum, which gives rise to long-range Coulomb potentials. A…

Materials Science · Physics 2007-05-23 Bradley A. Foreman

We demonstrate that a series of procedures for increasing the efficiency of transition matrix calculations can be realized by integrating the standard single-spin flip transition matrix method with global cluster flipping techniques. Our…

Statistical Mechanics · Physics 2019-03-19 David Yevick , Yong Hwan Lee

A new approximate scheme, DSUB$m$, is described for the coupled cluster method. We then apply it to two well-studied (spin-1/2 Heisenberg antiferromagnet) spin-lattice models, namely: the $XXZ$ and the $XY$ models on the square lattice in…

Strongly Correlated Electrons · Physics 2017-08-24 R. F. Bishop , P. H. Y. Li , J. Schulenburg

We present a control-theoretic analysis of the system consisting of a two-level atom coupled with a quantum harmonic oscillator. We show that by applying external fields with just two resonant frequencies, any desired unitary operator can…

Quantum Physics · Physics 2009-11-13 Haidong Yuan , Seth Lloyd

We compute the leading and sub-leading spin effects through the second post-Newtonian order (2PN) in spherical harmonic modes of gravitational waveforms from inspiralling compact binaries in non-circular orbits with non-precessing…

General Relativity and Quantum Cosmology · Physics 2023-08-07 Kaushik Paul , Chandra Kant Mishra

We study the effect of spin-orbit coupling on quantum gates produced by pulsing the exchange interaction between two single electron quantum dots. Spin-orbit coupling enters as a small spin precession when electrons tunnel between dots. For…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 D. Stepanenko , N. E. Bonesteel , D. P. DiVincenzo , G. Burkard , Daniel Loss

The global coupling of few-level quantum systems ("spins") to a discrete set of bosonic modes is a key ingredient for many applications in quantum science, including large-scale entanglement generation, quantum simulation of the dynamics of…

Quantum Gases · Physics 2016-12-07 Michael L. Wall , Arghavan Safavi-Naini , Ana Maria Rey

In this contribution we present calculations performed for interacting electron systems within a non-perturbative formulation of the cluster theory. Extrapolation of the model to describe the time dependence of the interacting systems is…

Atomic Physics · Physics 2009-11-13 M. Tomaselli , T. Kuehl , D. Ursescu , S. Fritzsche

Simulating molecules using the Variational Quantum Eigensolver method is one of the promising applications for NISQ-era quantum computers. Designing an efficient ansatz to represent the electronic wave function is crucial in such…

Chemical Physics · Physics 2022-05-09 Dmitry A. Fedorov , Yuri Alexeev , Stephen K. Gray , Matthew Otten

We investigate the fractionalized Skyrmion excitations induced by spin-orbit coupling in rotating and rapidly quenched spin-1 Bose-Einstein condensates. Our results show that the fractionalized Skyrmion excitation depends on the combination…

Quantum Gases · Physics 2015-06-04 Chao-Fei Liu , Wu-Ming Liu

Focusing on the efficient probe and manipulation of single-particle spin states, we investigate the coupled spin and orbital dynamics of a spin 1/2 particle in a harmonic potential subject to ultrastrong spin-orbit interaction and external…

Mesoscale and Nanoscale Physics · Physics 2014-01-21 C. Echeverria-Arrondo , E. Ya. Sherman