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Raman spectroscopy is a widely-used non-destructive material characterization method, which provides information about the vibrational modes of the material and therefore of its atomic structure and chemical composition. Interpretation of…

Computational Physics · Physics 2023-02-09 Mohammad Bagheri , Hannu-Pekka Komsa

Machine learning methods have found many applications in Raman spectroscopy, especially for the identification of chemical species. However, almost all of these methods require non-trivial preprocessing such as baseline correction and/or…

Machine Learning · Computer Science 2018-02-07 Jinchao Liu , Margarita Osadchy , Lorna Ashton , Michael Foster , Christopher J. Solomon , Stuart J. Gibson

Open Set Recognition (OSR) requires models not only to accurately classify known classes but also to effectively reject unknown samples. However, when unknown samples are semantically similar to known classes, inter-class overlap in the…

Computer Vision and Pattern Recognition · Computer Science 2025-11-19 Dongdong Zhao , Ranxin Fang , Changtian Song , Zhihui Liu , Jianwen Xiang

We demonstrate novel instrumentation for spontaneous Raman spectroscopy in biofluids, enabling development of a portable, automated, reliable diagnostics technique requiring minimal operator expertise to quantify disease markers. Label-free…

Biological Physics · Physics 2021-05-27 Emily E. Storey , Duxuan Wu , Amr S. Helmy

Rapid and reliable detection and identification of unknown chemical substances is critical to homeland security. It is challenging to identify chemical components from a wide range of explosives. There are two key steps involved. One is a…

Numerical Analysis · Mathematics 2011-10-10 Y. Sun , J. Xin

Time-resolved spectral techniques play an important analysis tool in many contexts, from physical chemistry to biomedicine. Customarily, the label-free detection of analytes is manually performed by experts through the aid of classic…

Machine Learning · Computer Science 2020-11-17 Stefano Rini , Hirotsugu Hiramatsu

The primary assumption of conventional supervised learning or classification is that the test samples are drawn from the same distribution as the training samples, which is called closed set learning or classification. In many practical…

Computer Vision and Pattern Recognition · Computer Science 2022-08-23 Sepideh Esmaeilpour , Lei Shu , Bing Liu

Open-Set Classification (OSC) intends to adapt closed-set classification models to real-world scenarios, where the classifier must correctly label samples of known classes while rejecting previously unseen unknown samples. Only recently,…

Computer Vision and Pattern Recognition · Computer Science 2022-10-19 Andres Palechor , Annesha Bhoumik , Manuel Günther

The limitations of existing Synthetic Aperture Radar (SAR) Automatic Target Recognition (ATR) methods lie in their confinement by the closed-environment assumption, hindering their effective and robust handling of unknown target categories…

Computer Vision and Pattern Recognition · Computer Science 2024-12-09 Xiayang Xiao , Zhuoxuan Li , Ruyi Zhang , Jiacheng Chen , Haipeng Wang

Open set recognition (OSR), aiming to simultaneously classify the seen classes and identify the unseen classes as 'unknown', is essential for reliable machine learning.The key challenge of OSR is how to reduce the empirical classification…

Computer Vision and Pattern Recognition · Computer Science 2021-09-08 Guangyao Chen , Peixi Peng , Xiangqian Wang , Yonghong Tian

To assist in the development of machine learning methods for automated classification of spectroscopic data, we have generated a universal synthetic dataset that can be used for model validation. This dataset contains artificial spectra…

Machine Learning · Computer Science 2022-06-15 Jan Schuetzke , Nathan J. Szymanski , Markus Reischl

Histopathology, the current gold standard for cancer diagnosis, involves the manual examination of tissue samples after chemical staining, a time-consuming process requiring expert analysis. Raman spectroscopy is an alternative, stain-free…

In open-set recognition (OSR), classifiers should be able to reject unknown-class samples while maintaining high closed-set classification accuracy. To effectively solve the OSR problem, previous studies attempted to limit latent feature…

Computer Vision and Pattern Recognition · Computer Science 2022-07-22 Wonwoo Cho , Jaegul Choo

Active Learning (AL) aims to enhance the performance of deep models by selecting the most informative samples for annotation from a pool of unlabeled data. Despite impressive performance in closed-set settings, most AL methods fail in…

Computer Vision and Pattern Recognition · Computer Science 2023-12-22 Bardia Safaei , Vibashan VS , Celso M. de Melo , Vishal M. Patel

Scattering obscures information carried by wave by producing a speckle pattern, posing a common challenge across various fields, including microscopy and astronomy. Traditional methods for extracting information from speckles often rely on…

Detecting both known and unknown objects is a fundamental skill for robot manipulation in unstructured environments. Open-set object detection (OSOD) is a promising direction to handle the problem consisting of two subtasks: objects and…

Computer Vision and Pattern Recognition · Computer Science 2023-12-05 Zhongxiang Zhou , Yifei Yang , Yue Wang , Rong Xiong

Mass spectrometry is a widely used method to study molecules and processes in medicine, life sciences, chemistry, catalysis, and industrial product quality control, among many other applications. One of the main features of some mass…

Chemical Physics · Physics 2024-07-02 Daniil A. Boiko , Valentine P. Ananikov

As the Internet is growing rapidly these years, the variant of malicious software, which often referred to as malware, has become one of the major and serious threats to Internet users. The dramatic increase of malware has led to a research…

Machine Learning · Computer Science 2020-04-10 Jingyun Jia

Confocal Raman microscopy, a highly specific and label-free technique for the microscale study of thick samples, often presents difficulties due to weak Raman signals. Inhomogeneous samples introduce wavefront aberrations that further…

Coherent Raman scattering provides highly sensitive vibrational analysis through nonlinear light-matter interactions. However, its application to metal interfaces has remained challenging because the intrinsically large non-resonant…