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The correlated electronic structure of the submonolayer surface systems Sn/Si(111) and Sn/Ge(111) is investigated by density-functional theory (DFT) and its combination with explicit many-body methods. Namely, the dynamical mean-field…

Materials Science · Physics 2015-03-13 Sergej Schuwalow , Daniel Grieger , Frank Lechermann

The 7x7 reconstruction of Si(111) surface is widely understood by the dimer-adatom-stacking-fault model (DAS), but the predicted metallicity of DAS contradicts experimental signs of insulation. It is still challenge to predict DAS-like…

Mesoscale and Nanoscale Physics · Physics 2025-06-19 Yuke Song , ShiFang Li , PeiZe Lin , Jin Li , Tao Ouyang , Chao Tang , Chaoyu He

We examine theoretically the signatures of magnetic adatoms in graphene probed by scanning tunneling spectroscopy (STS). When the adatom hybridizes equally with the two graphene sublattices, the broadening of the local adatom level is…

Strongly Correlated Electrons · Physics 2009-11-11 Bruno Uchoa , Ling Yang , S. -W. Tsai , N. M. R. Peres , A. H. Castro Neto

Integrating nanoscale opto-electronic functions is vital for applications such as optical emitters, detectors, and quantum information. Lanthanide atoms show great potential in this endeavor due to their intrinsic transitions. Here, we…

Applied Physics · Physics 2024-01-02 Eric Duverger , Damien Riedel

The energetics and structures of physisorbed and chemisorbed alkanethiols on Au(111) have been systematically investigated up to 10 carbon atoms using van der Waals (vdW) corrected density functional theory (DFT) calculations. The role of…

Chemical Physics · Physics 2018-03-07 Ersen Mete , Merve Yortanlı , Mehmet Fatih Danışman

Recent scanning tunneling spectroscopy (STM) experiments display images with star and ellipsoidal like features resulting from unique geometrical arrangements of a few adsorbed hydrogen atoms on graphite. Based on first-principles STM…

Our ability to understand and tailor metal-organic interfaces is mandatory to functionalize organic complexes for next generation electronic and spintronic devices. For magnetic data storage applications, metal-carrying organic molecules,…

Materials Science · Physics 2019-03-14 J. Seidel , L. L. Kelly , M. Franke , G. van Straaten , C. Kumpf , M. Cinchetti , M. Aeschlimann , B. Stadtmüller

We investigated the adsorption of iodine on silver (111) in ultra-high vacuum. Using low-temperature scanning tunneling microscopy (LT-STM) measurements we catalog the complex surface structures on the local scale. We identified three…

Materials Science · Physics 2022-04-13 Michael Dreyer , Joseph Murray , Robert E. Butera

Theoretical and experimental investigation of the electronic and magnetic structure of transition metal atoms on an insulating interface with a metallic substrate at low temperatures is quite challenging. In this paper, we show a density…

Advanced materials often consist of multiple elements which are arranged in a complicated structure. Quantitative scanning transmission electron microscopy is useful to determine the composition and thickness of nanostructures at the atomic…

Applied Physics · Physics 2024-05-17 Zezhong Zhang , Ivan Lobato , Annick De Backer , Sandra Van Aert , Peter Nellist

LEED experiments show that Li adsorbed at Cu(100) surfaces at room temperature induces a (2x1) missing row substrate reconstruction while adsorption at lower temperatures, T=180 K, results in an unreconstructed Cu(100)+c(2x2)--Li overlayer…

mtrl-th · Physics 2009-10-30 S. Quassowski , K. Hermann

Ammonium tetrathiomolybdate (ATM) spontaneously self assembles on Au electrodes forming a hydrophilic, air stable, pH (3-11) tolerant multilayer that is stable over a reasonably large potential window. The ATM functionalized Au electrodes…

Materials Science · Physics 2014-09-11 Sudipta Chatterjee , Kushal Sengupta , Abhishek Dey

Superconductors with non-trivial band topology are emerging as one of the best avenues to study quantum anomalies and experimental realization of Majorana Fermions. This article reports the successful crystal growth of superconducting SnAs,…

Superconductivity · Physics 2021-10-27 M. M. Sharma , N. K. Karn , Prince Sharma , Ganesh Gurjar , S. Patnaik , V. P. S. Awana

In this paper, we report first principles calculations based on density functional theory to reveal the effects of selected adatoms (Li, Na, K, Be, Mg, Ca, B, C, N, O, Al, Si, P, Ga, Ge, As, Se and S) adsorption on GaX ( where X=S, Se)…

Mesoscale and Nanoscale Physics · Physics 2017-11-29 H. D. Ozaydin , Y. Kadioglu , F. Ersan , O. Üzengi Aktürk , E. Aktürk

We carried out simulations of crystal truncation rod (CTR) scatterings, i.e., one of the surface X-ray diffraction techniques with atomic resolution, from a monolayer He film adsorbed on graphite. Our simulations reveal that the 00L rod…

We investigate the static and dynamic behaviors of a Br adlayer electrochemically deposited onto single-crystal Ag(100) using an off-lattice model of the adlayer. Unlike previous studies using a lattice-gas model, the off-lattice model…

Materials Science · Physics 2015-06-24 S. J. Mitchell , Sanwu Wang , P. A. Rikvold

Molecular electronics on silicon has distinct advantages over its metallic counterpart. We describe a theoretical formalism for transport through semiconductor-molecule heterostructures, combining a semi-empirical treatment of the bulk…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 T. Rakshit , G-C. Liang , A. W. Ghosh , S. Datta

We have observed an aggregation of carbon or carbon derivatives on platinum and natively oxidized silicon surfaces during STM measurements in ultra-high vacuum on solvent-cleaned samples previously structured by e-beam lithography. We have…

Mesoscale and Nanoscale Physics · Physics 2012-08-28 Dominik Stöffler , Hilbert von Löhneysen , Regina Hoffmann

We investigate the adsorption of cobalt phthalocyanine (CoPc) molecules on a thin layer of cobalt oxide grown on Ir(100). To that end we compare the results of low-temperature scanning tunneling microscopy (STM) with those of ab-initio…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Tobias Schmitt , Pascal Ferstl , Lutz Hammer , M. Alexander Schneider , Josef Redinger

We present a joint experimental and theoretical determination of structures of Ag adatoms on the Ge(111) surface using low energy electron diffraction, low energy electron microscopy, scanning tunneling microscopy, and density functional…

Materials Science · Physics 2019-09-25 Shree Ram Acharya , Cory H. Mullet , Jason A. Giacomo , Duy Le , Shirley Chiang , Talat S. Rahman