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Compressing or cooling a fluid typically enhances its static interparticle correlations. However, there are notable exceptions. Isothermal compression can reduce the translational order of fluids that exhibit anomalous waterlike trends in…

Soft Condensed Matter · Physics 2008-04-11 William P. Krekelberg , Jeetain Mittal , Venkat Ganesan , Thomas M. Truskett

The interrelations between short range structural and elastic aspects in glasses and glass forming liquids pose important and yet unresolved questions. In this paper these relations are analyzed for mono-atomic glasses and stressed liquids…

Disordered Systems and Neural Networks · Physics 2009-10-31 Tamar Kustanovich , Zeev Olami

Amorphous materials such as metallic, polymeric, and colloidal glasses, exhibit complex preparation-dependent mechanical response to applied shear. We perform numerical simulations to investigate the mechanical response of binary…

Statistical Mechanics · Physics 2017-09-13 Meng Fan , Kai Zhang , Jan Schroers , Mark D. Shattuck , Corey S. O'Hern

We explore the structural signatures of excitations in amorphous materials with the atomic cluster expansion (ACE), a universal and complete linear basis of descriptors of the atomic environment. Body-orderd linear classifiers are…

Disordered Systems and Neural Networks · Physics 2024-10-07 Joerg Rottler , Christoph Ortner

The evolution of porous structure, potential energy and local density in binary glasses under oscillatory shear deformation is investigated using molecular dynamics simulations. The porous glasses were initially prepared via a rapid thermal…

Soft Condensed Matter · Physics 2022-10-25 Nikolai V. Priezjev , Maxim A. Makeev

Machine learning techniques have been used to quantify the relationship between local structural features and variations in local dynamical activity in disordered glass-forming materials. To date these methods have been applied to an array…

Soft Condensed Matter · Physics 2021-01-07 Indrajit Tah , Tristan A. Sharp , Andrea J. Liu , Daniel M. Sussman

Jammed soft disks exhibit avalanches of particle rearrangements under quasistatic shear. We follow the avalanches using steepest descent to decompose them into individual localized rearrangements. We characterize the local structural…

Soft Condensed Matter · Physics 2020-09-25 Ge Zhang , Sean Ridout , Andrea J. Liu

We study the yielding behaviour of a model glass under cyclic athermal quastistatic deformation computationally, and show that yielding is characterised by the discontinuous appearance of shear bands, whose width is about ten particle…

Disordered Systems and Neural Networks · Physics 2019-05-01 Anshul D. S. Parmar , Saurabh Kumar , Srikanth Sastry

The relation between elasticity and yielding is investigated in a model polymer solid by Molecular-Dynamics simulations. By changing the bending stiffness of the chain and the bond length, semicrystalline and disordered glassy polymers -…

Soft Condensed Matter · Physics 2018-11-20 Nicola Calonaci , Andrea Giuntoli , Sebastiano Bernini , Dino Leporini

We show numerically that a three-dimensional model for structural glass displays aging, rejuvenation and memory effects when submitted to a temperature cycle. These effects indicate that the free energy landscape of structural glasses may…

Soft Condensed Matter · Physics 2019-07-03 Camille Scalliet , Ludovic Berthier

Atomistic deformation simulations in the nominally elastic regime are performed for a model binary glass with strain rates as low as $10^{4}$/sec (corresponding to 0.01 shear strain per 1$\mu$sec). A robust elasticity is revealed that…

Soft Condensed Matter · Physics 2020-11-21 P. M. Derlet , R. Maass

We consider unsupervised learning methods for characterizing the disordered microscopic structure of supercooled liquids and glasses. Specifically, we perform dimensionality reduction of smooth structural descriptors that describe radial…

Statistical Mechanics · Physics 2022-11-24 Daniele Coslovich , Robert L. Jack , Joris Paret

Plastic rearrangements play a crucial role in the characterization of soft-glassy materials, such as emulsions and foams. Based on numerical simulations of soft-glassy systems, we study the dynamics of plastic rearrangements at the…

Soft Condensed Matter · Physics 2014-10-27 R. Benzi , M. Sbragaglia , A. Scagliarini , P. Perlekar , M. Bernaschi , S. Succi , F. Toschi

Amorphous solids relax via slow molecular rearrangement induced by thermal fluctuations or applied stress. Although microscopic structural signatures predicting these structural relaxations have long been sought, a physically motivated…

Soft Condensed Matter · Physics 2024-08-12 Ratimanasee Sahu , Mohit Sharma , Peter Schall , Sarika Maitra Bhattacharyya , Vijayakumar Chikkadi

When stressed sufficiently, solid materials yield and deform plastically via reorganization of microscopic constituents. Indeed, it is possible to alter the micro-structure of materials by judicious application of stress, an empirical pro-…

Soft Condensed Matter · Physics 2021-08-09 K. L. Galloway , Xiaoguang Ma , Nathan C. Keim , Douglas J. Jerolmack , Arjun G. Yodh , Paulo E. Arratia

We explore the relationship between a machine-learned structural quantity (softness) and excess entropy in simulations of supercooled liquids. Excess entropy is known to scale well the dynamical properties of liquids, but this…

Soft Condensed Matter · Physics 2023-06-07 Ian R. Graham , Paulo E. Arratia , Robert A. Riggleman

We discuss aging and localization in a simple "Eshelby" mesoscopic model of amorphous plasticity. Plastic deformation is assumed to occur through a series of local reorganizations. Using a discretization of the mechanical fields on a…

Soft Condensed Matter · Physics 2011-12-06 Damien Vandembroucq , Stéphane Roux

Complex crystal structures are composed of multiple local environments, and how this type of order emerges spontaneously during crystal growth has yet to be fully understood. We study crystal growth across various structures and along…

Soft Condensed Matter · Physics 2024-06-03 Maya M. Martirossyan , Matthew Spellings , Hillary Pan , Julia Dshemuchadse

Plastic deformation in metallic glasses at room temperature leads to the development of shear bands due to shear localization. In many experiments, shear bands have shown local density variations along their path, with a distinct imbalance…

Disordered Systems and Neural Networks · Physics 2024-07-22 Harald Rösner , Arabinda Bera , Alessio Zaccone

The fundamental instability responsible for the shear localization which results in shear bands in amorphous solids remains unknown despite enormous amount of research, both experimental and theoretical. As this is the main mechanism for…

Soft Condensed Matter · Physics 2015-06-05 Ratul Dasgupta , H. George E. Hentschel , Itamar Procaccia