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Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

The ionization dynamic of argon plasma irradiated by an intense laser is investigated to understand transient physics in dynamic systems. This study demonstrates that significant delayed ionization responses and stepwise ionization…

Plasma Physics · Physics 2026-01-22 M. S. Cho , A. L. Milder , W. Rozmus , H. P. Le , H. A. Scott , D. T. Bishel , D. Turnbull , S. B. Libby , M. E. Foord

Generation of laser-like narrow bandwidth emissions from nitrogen molecular ions generated in intense near- and mid-infrared femtosecond laser fields has aroused much interest because of the mysterious physics underlying such a phenomenon…

Optics · Physics 2018-02-28 Zhaoxiang Liu , Jinping Yao , Jinming Chen , Bo Xu , Wei Chu , Ya Cheng

Light-phase-sensitive techniques, such as coherent multidimensional spectroscopy, are well-established in a broad spectral range, already spanning from radio-frequencies in nuclear magnetic resonance spectroscopy to visible and ultraviolet…

A wide range of ultrafast phenomena in various atomic, molecular and condense matter systems is governed by electron dynamics. Therefore, the ability to image electronic motion in real space and real time would provide a deeper…

Atomic Physics · Physics 2018-02-27 Daria Popova-Gorelova

We present the results of an experimental and numerical investigation into temporally non-local coherent interactions between ultrashort pulses, mediated by Raman coherence, in gas-filled kagom\'{e}-style hollow-core photonic crystal fiber.…

Quantum coherence plays a fundamental role in the study and control of ultrafast dynamics in matter. In the case of photoionization, entanglement of the photoelectron with the ion is a well known source of decoherence when only one of the…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

Excited-state vibrational dynamics in molecules can be studied by an electronically off-resonant Raman process induced by a probe pulse with variable delay with respect to an actinic pulse. We establish the connection between several…

Chemical Physics · Physics 2013-09-27 Konstantin E. Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…

Atomic Physics · Physics 2019-05-15 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

The progress and the chronology in understanding the influence of electron correlations on the electronic structure of atoms and the dynamics of atomic processes are reviewed focusing on benchmark rare-gas atoms. The contributions and the…

We present coincidence measurements of two-photon double-ionization (TPDI) of argon driven by femtosecond pulses tunable around 26.5 eV photon energy, which are obtained from a high-harmonic generation source. The measured photoelectron…

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

Quantum Physics · Physics 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

We measure the photoelectron energy spectra from strong-field ionization of Kr in a two-color laser pulse consisting of a strong 400-nm field and a weak 800-nm field. The intensities of the main above-threshold ionization (ATI) and sideband…

Atomic Physics · Physics 2019-12-11 Yudi Feng , Min Li , Siqiang Luo , Kun Liu , Baojie Du , Yueming Zhou , Peixiang Lu

Resonances leave prominent signatures in atomic and molecular ionization triggered by the absorption of single or multiple photons. These signatures reveal various aspects of the ionization process, characterizing both the initial and final…

Atomic Physics · Physics 2026-03-03 Anatoli S. Kheifets

Photoelectron ionization spectra of an autoionization system with one discrete level interacting with a neighbor two-level atom are discussed. The formula for long-time ionization spectra is derived. According to this formula, the spectra…

Quantum Physics · Physics 2015-05-27 Jan Perina , Antonin Luks , Wieslaw Leonski , Vlasta Perinova

We propose a scheme to realize the storage and retrieval of light pulses in a fast-light medium via a mechanism of active Raman gain (ARG). The system under consideration is a four-level atomic gas interacting with three (pump, signal and…

Optics · Physics 2017-11-15 Datang Xu , Zhengyang Bai , Guoxiang Huang

We describe an experiment to measure the emitted real-time electric field from an ultrafast third-order nonlinear optical interaction in molecules, using a phase-tracked spectral interferometry scheme. By combining a software lock-in…

Optics · Physics 2025-03-11 Siddhant Pandey , Francis Walz , Niranjan Shivaram

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan