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A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying AC Stark shifts, induced by far off-resonant, focused laser…

Atomic Physics · Physics 2015-06-16 M. Shi , P. F. Herskind , M. Drewsen , I. L. Chuang

We present a technique for generating light in an arbitrary polarization state. The technique is based on interference of two orthogonally polarized light beams, whose amplitudes and phases are controlled with a Mach-Zehnder inteferometer…

Applied Physics · Physics 2018-10-22 P. Wlodarczyk , S. Pustelny , D. Budker

Optical pump-probe techniques are used to generate and measure electron spin polarization in a gallium arsenide epilayer in which the electron spin coherence time exceeds the mode-locked laser repetition period. Resonant spin amplification…

Mesoscale and Nanoscale Physics · Physics 2020-09-14 Michael Macmahon , Joseph R. Iafrate , Michael J. Dominguez , Vanessa Sih

Optical pump-probe time- and magnetic-field-resolved Kerr rotation measurements provide a window into the mechanisms that generate dynamic nuclear polarization in bulk gallium arsenide. Previously, we have reported an unexpected dependence…

Mesoscale and Nanoscale Physics · Physics 2020-05-13 Michael J. Dominguez , Joseph R. Iafrate , Vanessa Sih

Optically Pumped Magnetometers use light to drive an atomic vapor into a Non-Equilibrium Steady State for sensing. This kind of state is achieved when spin-exchange collisions, together with optical pumping, dominate the relaxation…

Quantum Physics · Physics 2026-04-13 A. F. Sousa , C. H. S. Vieira , H. M. Florez

We have studied relative-intensity fluctuations for a variable set of orthogonal elliptic polarization components of a linearly polarized laser beam traversing a resonant $^{87}$Rb vapor cell. Significant polarization squeezing at the…

Quantum Physics · Physics 2015-05-28 S. Barreiro , P. Valente , H. Failache , A. Lezama

We theoretically investigate dynamic nuclear spin polarization in a self-assembled quantum dot pumped optically by two laser beams. With the assumption that a noncollinear interaction between the hole spin and nuclear spins leads to nuclear…

Mesoscale and Nanoscale Physics · Physics 2013-06-07 Xiao-Feng Shi

Population of levels of the hyperfine and fine split ground state of an atom is affected by radiative transitions induced by anisotropic radiation flux. Such aligned atoms precess in the external magnetic field and this affects properties…

Astrophysics · Physics 2007-05-23 Huirong Yan , A. Lazarian

In the optical pumping systems based on the pump-probe arrangement, the spin polarization of the atoms is generally monitored utilizing the probe laser beam, in which way an extra perturbation must be introduced and thus affects the normal…

Atomic Physics · Physics 2017-02-09 Jiancheng Fang , Rujie Li , Lihong Duan , Wenfeng Fan , Liwei Jiang

We report on further investigation of nuclear hyperpolarization of helium-3 in magnetized plasma at a magnetic field of 3.66 T and at different experimental conditions in a dual cell of relatively large volume, compared to those reported in…

Atomic Physics · Physics 2022-08-16 Alexander Makarchenko , Vyacheslav Kuzmin , Kajum Safiullin , Murat Tagirov

We report a measurement of the nuclear polarization of laser-cooled, optically-pumped $^{37}\mathrm{K}$ atoms which will allow us to precisely measure angular correlation parameters in the beta-decay of the same atoms. These results will be…

We propose schemes to produce highly nuclear-spin polarized small molecules in an intense and cold molecular beam via microwave or infrared rotational excitation, followed by hyperfine-induced quantum beats. Repumping schemes can be used to…

Chemical Physics · Physics 2026-03-20 C. S. Kannis , T. P. Rakitzis

We demonstrate a novel experimental technique for quantum-state tomography of the collective density matrix. It is based on measurements of the polarization of light, traversing the atomic vapor. To assess the technique's robustness against…

Quantum Physics · Physics 2025-08-29 Marek Kopciuch , Magdalena Smolis , Adam Miranowicz , Szymon Pustelny

Photoassociation of ultracold atoms is shown to lead to alignment of the product molecules along the excitation laser polarization axis. We theoretically investigate pulsed photoassociation of $^{87}Rb$ atoms into a specific weakly-bound…

Quantum Physics · Physics 2017-11-15 S. Kallush , J. L. Carini , P. L. Gould , R. Kosloff

The interaction between light and vapors in the presence of magnetic fields is fundamental to many quantum technologies and applications. Recently, the ability to geometrically confine atoms into periodic structures has enabled the creation…

Applied Physics · Physics 2025-05-20 Ori Nefesh , Heleni Krelman , Kfir Levi , Liron Stern

Circularly polarized light plays a key role in many applications including spectroscopy, microscopy, and control of atomic systems. Particularly in the latter, high polarization purity is often required. Integrated technologies for atomic…

Optics · Physics 2022-09-20 Leonardo Massai , Tom Schatteburg , Jonathan P. Home , Karan K. Mehta

We present a novel approach to precisely synthesize arbitrary polarization states of light with a high modulation bandwidth. Our approach consists of superimposing two laser light fields with the same wavelength, but with opposite circular…

Atomic magnetometry is one of the most sensitive field-measurement techniques for biological, geo-surveying, and navigation applications. An essential process in atomic magnetometry is measurement of optical polarization rotation of a…

Optics · Physics 2023-04-19 Xuting Yang , Meryem Benelajla , Jennifer T. Choy

We demonstrate the polarization of electron orbital angular momentum (OAM) in neutral atoms by integrating the Zeeman effect with attosecond transient absorption spectroscopy (ATAS). Using density matrix simulations, we show that in a…

Atomic Physics · Physics 2025-07-04 Hongtao Hu , Sebastian Mai , Peng Peng , Andrius Baltuška , Xinhua Xie

We show that it is possible to generate continuous-wave fields and pulses of polarization squeezed light by sending classical, linearly polarized laser light twice through an atomic sample which causes an optical Faraday rotation of the…

Quantum Physics · Physics 2011-10-13 Jacob F. Sherson , Klaus Molmer