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Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Strongly Correlated Electrons · Physics 2016-09-01 W. K. Zhu , J. -C. Tung , W. Tong , L. Ling , M. Starr , J. M. Wang , W. C. Yang , Y. Losovyj , H. D. Zhou , Y. Q. Wang , P. -H. Lee , Y. -K. Wang , Chi-Ken Lu , S. X. Zhang

The electronic structure and magnetism of Sr$_2$CeIrO$_6$, an Ir-based double perovskite system has been investigated using first-principles calculations. We found that a strong spin-orbit coupling dictate the electronic and magnetic…

Strongly Correlated Electrons · Physics 2013-01-29 S. K. Panda , I. Dasgupta

Spin-orbit coupling (SOC) plays a crucial role in magnetic and electronic properties of 5$d$ iridates. In this paper we have experimentally investigated the structural and physical properties of a series of Ir-based double perovskite…

Strongly Correlated Electrons · Physics 2019-10-02 Abhisek Bandyopadhyay , I. Carlomagno , L. Simonelli , M. Moretti Sala , A. Efimenko , C. Meneghini , Sugata Ray

The 3$d$-5$d$ based double perovskites offer an ideal playground to study the interplay between electron correlation ($U$) and spin-orbit coupling (SOC) effect, showing exotic physics. The Sr$_2$FeIrO$_6$ is an interesting member in this…

Strongly Correlated Electrons · Physics 2020-10-23 K. C. Kharkwal , Roumita Roy , Harish Kumar , A. K. Bera , S. M. Yusuf , A. K. Shukla , Kranti Kumar , Sudipta Kanungo , A. K. Pramanik

The double perovskite Ba$_{2}$NaOsO$_{6}$ (BNOO), an exotic example of a very high oxidation state (heptavalent) osmium $d^1$ compound and also uncommon by being a ferromagnetic Mott insulator without Jahn-Teller (JT) distortion, is modeled…

Strongly Correlated Electrons · Physics 2015-06-23 Shruba Gangopadhyay , Warren E. Pickett

The 5$d$ series semimetallic Dirac nodal-line perovskite SrIrO$_3$ presents a promising system to study the interplay between spin-orbit coupling and electron-electron interactions in the epitaxial thin film geometry. The competition…

Materials Science · Physics 2024-06-05 Wesley Surta , Saeed Almalki , Ya-Xun Lin , Tim Veal , Marita O'Sullivan

Using a combination of first-principles density functional theory (DFT) calculations and exact diagonalization studies of a first-principles derived model, we carry out a microscopic analysis of the magnetic properties of the half-metallic…

We investigate the antiferromagnetic insulating state of the recently discovered double perovskites Sr$_2$XOsO$_6$ (X$=$Sc, Mg) by using ab-initio calculations (based on Density Functional Theory and Dynamical Mean-Field Theory) to…

Strongly Correlated Electrons · Physics 2016-11-22 Gianluca Giovannetti

Understanding charge transfer at oxide interfaces is crucial for designing materials with emergent electronic and magnetic properties, especially in systems where strong electron correlations and spin-orbit coupling coexist.…

The subtle interplay between spin-orbit coupling, exchange interactions, and cation ordering can lead to exotic magnetic states in transition-metal ions. We report a comprehensive study of the Re-based (5$d^1$) ordered double perovskite…

Using the first-principles density functional approach, we investigate a material Pr$_2$MgIrO$_6$ (PMIO) of double perovskite structure synthesized recently. According to the calculations, PMIO is a magnetic Mott-Hubbard insulator…

Materials Science · Physics 2016-04-29 Madhav P. Ghimire , Long-Hua Wu , Xiao Hu

The 3$d$-5$d$ based double perovskites are of current interest as they provide model system to study the interplay between electronic correlation ($U$) and spin-orbit coupling (SOC). Here we report detailed structural, magnetic and…

Strongly Correlated Electrons · Physics 2017-10-30 K C Kharkwal , A K Pramanik

Here, we report on the structural, electronic, and magnetic properties of a polycrystalline sample of the LaCaCoIrO$_6$ double-perovskite investigated by means of synchrotron x-ray powder diffraction, x-ray absorption spectroscopy, and…

Strongly Correlated Electrons · Physics 2023-10-03 L. Bufaiçal , L. S. I. Veiga , J. R. L. Mardegan , T. Pohlmann , S. Francoual , S. S. Dhesi , M. B. Fontes , E. M. Bittar

This study is aimed at exploring the electronic, magnetic, and magneto-optical properties of double perovskites Ca$_2$FeIrO$_6$ and Ca$_2$CoIrO$_6$ {with monoclinic structure (space group P21/$c$) } in order to examine their potential…

Materials Science · Physics 2024-01-18 I. Touaibia , A. Bouguerra , W. Guenez , F. Chemam

We report electron spin resonance (ESR) spectroscopy results on the double perovskite Ba$_2$YIrO$_6$. On general grounds, this material is expected to be nonmagnetic due to the strong coupling of the spin and orbital momenta of Ir$^{5+}$…

Strongly Correlated Electrons · Physics 2018-06-12 S. Fuchs , T. Dey , G. Aslan-Cansever , A. Maljuk , S. Wurmehl , B. Büchner , V. Kataev

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

Materials Science · Physics 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

We study the effect of substrate induced strain on the structural, transport, optical and electronic properties of Sr$_2$CoNbO$_6$ double perovskite thin films. The reciprocal space mapping, $\phi$-scan and high-resolution…

Materials Science · Physics 2020-08-19 Ajay Kumar , Rishabh Shukla , Akhilesh Pandey , Sandeep Dalal , M. Miryala , K. Ueno , M. Murakami , R. S. Dhaka

Re-based double perovskites (DPs) exhibit a complex interplay of structural and metal-insulator transitions. Here we systematically study the ground state electronic and structural properties for a family of Re-based DPs $A_2B$ReO$_6$…

Strongly Correlated Electrons · Physics 2018-01-10 Alex Taekyung Lee , Chris A. Marianetti

We have implemented a systematic LSDA and LSDA+U study of the double perovskites $A_{2}$FeReO$_{6}$ (A=Ba,Sr,Ca) and Sr$_{2}$$M$MoO$_{6}$ (M=Cr,Mn,Fe,Co) for understanding of their intriguing electronic and magnetic properties. The results…

Materials Science · Physics 2009-11-07 Hua Wu

The electronic structure of the spintronic material Sr$_2$CrReO$_6$ is studied by means of full-potential linear muffin-tin orbital method. Scalar relativistic calculations predict Sr$_2$CrReO$_6$ to be half-metallic with a magnetic moment…

Materials Science · Physics 2009-11-10 G. Vaitheeswaran , V. Kanchana , A. Delin
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