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Damage caused by freezing wet, porous materials is a widespread problem, but is hard to predict or control. Here, we show that polycrystallinity makes a great difference to the stress build-up process that underpins this damage. Unfrozen…

Soft Condensed Matter · Physics 2024-02-06 Dominic Gerber , Lawrence A. Wilen , Eric R. Dufresne , Robert W. Style

Most theoretical descriptions of stresses induced by freezing are rooted in the (generalized) Clapeyron equation, which predicts the pressure that a solid can exert as it cools below its melting temperature. This equation is central for…

Soft Condensed Matter · Physics 2023-08-09 Robert W. Style , Dominic Gerber , Alan W. Rempel , Eric R. Dufresne

The stress generation on pore walls due to the growth of a sodium chloride crystal in a confined aqueous solution is studied from evaporation experiments in microfluidic channels in conjunction with numerical computations of crystal growth.…

Fluid Dynamics · Physics 2018-06-25 A. Naillon , Pierre Joseph , M. Prat

What is pressure generated by ice crystals during ice-templating? This work addresses this crucial question by estimating the pressure exerted by oriented ice columns on a supramolecular probe composed of a lipid lamellar hydrogel during…

Soft Condensed Matter · Physics 2020-02-27 Niki Baccile , Thomas Zinn , Guillaume Laurent , Ghazi Messaoud , Viviana Cristiglio , Francisco Fernandes

Salt crystallization is a major cause of weathering of artworks, monuments and rocks. Damage will occur if crystals continue to grow in confinement, i.e. within the pore space of these materials generating mechanical stresses. We report on…

Materials Science · Physics 2016-01-26 Julie Desarnaud , Daniel Bonn , Noushine Shahidzadeh

Crystallization pressure drives deformation and damage in monuments, buildings and the Earth's crust. Even though the phenomenon has been known for 170 years there is no agreement between theoretical calculations of the maximum attainable…

Temperature increase in saturated porous materials under undrained conditions leads to thermal pressurization of the pore fluid due to the discrepancy between the thermal expansion coefficients of the pore fluid and of the solid matrix.…

Geophysics · Physics 2009-03-02 Siavash Ghabezloo , Jean Sulem

The pressure distribution is calculated underneath a skate which is pushed in the ice by the weight of a skater at rest. Due to the sharp edges of the skate the deformation is partly elastic and partly plastic. The ratio of the plastic and…

Classical Physics · Physics 2019-11-14 J. M. J. van Leeuwen

The mechanical properties of crystalline materials can be substantially modified under confinement. Such modified macroscopic properties are usually governed by the altered microstructures and internal stress fields. Here, we use a parallel…

Soft Condensed Matter · Physics 2016-10-25 Neil Y. C. Lin , Itai Cohen

A study of ice formation in stationary turbulent conditions is carried out in various limit regimes of crystal growth, supercooling and ice entrainment at the water surface. Analytical expressions for the temperature, salinity and ice…

Fluid Dynamics · Physics 2017-10-18 Francesca De Santi , Piero Olla

The presence of liquid water in frozen media impacts the strength of soils, the growth of frost heave, plant life and microbial activities, or the durability of infrastructures in cold regions. If the effect of confinement on freezing is…

Soft Condensed Matter · Physics 2019-07-25 Felix Ginot , Théo Lenavetier , Dmytro Dedovets , Sylvain Deville

We show that the long time tail of the shear stress autocorrelation, whose growth at large supercooling is responsible for the apparent divergence of the shear viscosity, is a direct result of a residual shear stress in the structures…

Soft Condensed Matter · Physics 2015-06-03 Sneha Abraham , Peter Harrowell

The friction of a stationary moving skate on smooth ice is investigated, in particular in relation to the formation of a thin layer of water between skate and ice. It is found that the combination of ploughing and sliding gives a friction…

Other Condensed Matter · Physics 2018-01-22 J. M. J. van Leeuwen

A drop of water that freezes from the outside-in presents an intriguing problem: the expansion of water upon freezing is incompatible with the self-confinement by a rigid ice shell. Using high-speed imaging we show that this conundrum is…

Fluid Dynamics · Physics 2017-04-05 Sander Wildeman , Sebastian Sterl , Chao Sun , Detlef Lohse

Heterogeneous ice growth exhibits a maximum in freezing rate arising from the competition between kinetics and the thermodynamic driving force between the solid and liquid states. Here, we use molecular dynamics simulations to elucidate the…

Soft Condensed Matter · Physics 2013-12-31 Razvan A. Nistor , Thomas E. Markland , B. J. Berne

Close to the triple point, the surface of ice is covered by a thin liquid layer (so-called quasi-liquid layer) which crucially impacts growth and melting rates. Experimental probes cannot observe the growth processes below this layer, and…

Chemical Physics · Physics 2021-01-22 David N. Sibley , Pablo Llombart , Eva G. Noya , Andrew J. Archer , Luis G. MacDowell

We describe observations of a novel hysteresis behavior in the growth of ice crystals under near-vacuum conditions. Above a threshold supersaturation, we find that the ice growth rate often exhibits a sudden increase that we attribute to an…

Materials Science · Physics 2008-09-30 Kenneth G. Libbrecht

The freezing of water is one of the major causes of mechanical damage in materials during wintertime; surprisingly this happens even in situations where water only partially saturates the material so that the ice has room to grow. Here we…

Soft Condensed Matter · Physics 2024-11-12 Menno Demmenie , Paul Kolpakov , Boaz van Casteren , Dirk Bakker , Daniel Bonn , Noushine Shahidzadeh

Convective flows coupled with solidification or melting in water bodies play a major role in shaping geophysical landscapes. Particularly in relation to the global climate warming scenario, it is essential to be able to accurately quantify…

Fluid Dynamics · Physics 2021-03-11 Ziqi Wang , Enrico Calzavarini , Chao Sun , Federico Toschi

It is widely known that freezing breaks soft, wet materials. However, the mechanism underlying this damage is still not clear. To understand this process, we freeze model, brittle hydrogel samples, while observing the growth of ice-filled…

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