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Thin GaP films can be grown on an exact Si(001) substrate with nearly perfect lattice match. We perform all-optical pump-probe measurements to investigate the ultrafast electron-phonon coupling at the buried interface of GaP/Si.…

Ultrafast carrier and phonon dynamics at the buried heterointerface of GaP/Si(001) are investigated by means of two-color pump-probe reflectivity measurements. The carrier-induced reflectivity signal exhibits a resonant enhancement at…

Materials Science · Physics 2025-04-15 Gerson Mette , Kunie Ishioka , Steven Youngkin , Wolfgang Stolz , Kerstin Volz , Ulrich Höfer

We report on the optical generation and detection of ultrashort acoustic pulses that propagate in three-dimensional semiconductor crystals. Photoexcitaiton of lattice-matched GaP layers grown on Si(001) gives rise to a sharp spike in…

Semiconductor devices favor high carrier mobility for reduced Joule heating and high thermal conductivity for rapid heat dissipation. The ability to accurately characterize the motion of charge carriers and heat carriers is necessary to…

Mesoscale and Nanoscale Physics · Physics 2026-03-26 Qichen Song , Sorren Warkander , Samuel C. Huberman

Lattice-matched GaP layers without extended defects can be grown on Si(001) substrate via a two-step growth procedure, consisting of low-temperature nucleation followed by high-temperature overgrowth. A transient reflectivity experiment on…

We report on the intrinsic optical generation and detection of coherent acoustic phonons at (001)-oriented bulk Si and GaP without metallic phonon transducer structures. Photoexcitation by a 3.1-eV laser pulse generates a normal strain…

Materials Science · Physics 2017-07-31 Kunie Ishioka , Avinash Rustagi , Ulrich Hoefer , Hrvoje Petek , Christopher J. Stanton

We show that large amplitude, coherent acoustic phonon wavepackets can be generated and detected in In$_x$Ga$_{1-x}$N/GaN epilayers and heterostructures in femtosecond pump-probe differential reflectivity experiments. The amplitude of the…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Rongliang Liu , Chang Sub Kim , G. D. Sanders , C. J. Stanton , J. S. Yahng , Y. D. Jho , K. J. Yee , E. Oh , D. S. Kim

Gallium phosphide is an important indirect band gap material with variety of applications in optics ranging from LEDs to applications in GaP/Si based solar cells. We investigated GaP using ultrafast, pump-probe coherent acoustic phonon…

Materials Science · Physics 2019-04-15 Andrey Baydin , Rustam Gatamov , Halina Krzyzanowska , Christopher J. Stanton , Norman Tolk

We have performed ultrafast pump-probe spectroscopy studies on a series of InAs/GaSb-based short-period superlattice (SL) samples with periods ranging from 46 \AA to 71 \AA. We observe two types of oscillations in the differential…

Materials Science · Physics 2012-11-26 G. T. Noe , H. J. Haugan , G. J. Brown , G. D. Sanders , C. J. Stanton , J. Kono

The coherent modulation of electronic and vibrational nonlinearities in atoms and molecular gases by intense few-cycle pulses has been used for high-harmonic generation in the soft X-ray and attosecond regime, as well as for Raman frequency…

Materials Science · Physics 2013-09-16 Muneaki Hase , Masayuki Katsuragawa , Anca Monia Constantinescu , Hrvoje Petek

Intermediate frequency range (511 - 514 cm-1) Si phonons in Si-SiO2 nanocomposites are shown to have contribution from both core1 and surface/interface1 Si phonons, where, ratio of contribution of the two depends on the size of a Si…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Ekta Rani , Alka Ingale , A. Chaturvedi , M. P. Joshi , L. M. Kukreja

Gallium phosphide (GaP) is an indirect bandgap semiconductor used widely in solid-state lighting. Despite numerous intriguing optical properties---including large $\chi^{(2)}$ and $\chi^{(3)}$ coefficients, a high refractive index ($>3$),…

Here we perform a series of time-resolved experiments where a 100 fs pump pulse is tuned between 528 nm and 555 nm, across the second indirect gap of intrinsic silicon at ~540 nm which involves electrons in a higher-lying conduction band…

Optics · Physics 2017-01-24 Fabio Novelli , Jeffrey A Davis

Optical grating technique, where optical gratings are generated via light inference, has been widely used to measure charge carrier and phonon transport in semiconductors. In this paper, compared are three types of transient optical grating…

Materials Science · Physics 2018-05-07 Ke Chen , Xianghai Meng , Feng He , Yongjian Zhou , Jihoon Jeong , Nathanial Sheehan , Seth R Bank , Yaguo Wang

Optical dual-pulse pumping actively creates quantum-mechanical superposition of the electronic and phononic states in a bulk solid. We here made transient reflectivity measurements in an n-GaAs using a pair of relative-phase-locked…

Mesoscale and Nanoscale Physics · Physics 2019-05-22 Kazutaka G. Nakamura , Kensuke Yokota , Yuki Okuda , Rintaro Kase , Takashi Kitashima , Yu Mishima , Yutaka Shikano , Yosuke Kayanuma

Black phosphorus is emerging as a promising semiconductor for electronic and optoelectronic applications. To study fundamental carrier properties, we performed ultrafast femtosecond pump-probe spectroscopy on thin film black phosphorus…

Mesoscale and Nanoscale Physics · Physics 2017-03-13 Vasudevan Iyer , Peide Ye , Xianfan Xu

Coherent phonons (CP) generated by laser pulses on the femtosecond scale have been proposed as a means to achieve ultrafast, non-thermal switching in phase-change materials such as Ge$_{2}$Sb$_{2}$Te$_{5}$(GST). Here we use ultrafast…

A femtosecond pump-probe setup is described that is optimised for broadband transient reflectivity experiments on solid samples over a wide range of temperatures. By combining a temporal resolution of 45 fs and a broad detection range…

Instrumentation and Detectors · Physics 2016-08-12 Edoardo Baldini , Andreas Mann , Simone Borroni , Christopher Arrell , Frank van Mourik , Fabrizio Carbone

The transient second harmonic generation and linear optical reflectivity signals measured simultaneously in reflection from GaAs/GaSb/InAs and GaAs/GaSb heterostructures revealed a new mechanism for creating self-induced transparency in…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Y. D. Glinka , N. H. Tolk , J. K. Furdyna

The transient evolution of carriers in an intrinsic graphene under ultrafast excitation, which is caused by the collisionless interband transitions, is studied theoretically. The energy relaxation due to the quasielastic acoustic phonon…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 P. N. Romanets , F. T. Vasko
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