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Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…

Mesoscale and Nanoscale Physics · Physics 2026-04-10 Elia Turco , Fupeng Wu , Annika Bernhardt , Nils Krane , Ji Ma , Roman Fasel , Michal Juriček , Xinliang Feng , Pascal Ruffieux

Problems of strongly interacting electrons can be greatly simplified by reducing them to effective quantum spin models. The initial step is renormalization of the Hamiltonian into a lower energy subspace. The positive and negative U Hubbard…

Strongly Correlated Electrons · Physics 2007-05-23 A. Auerbach

We study the behavior of the magnetization and the magnetic susceptibility of molecular magnets with complex bridging structure. Our computations are based on a post-Hartree-Fock method accounting for the intricate network of interatomic…

Strongly Correlated Electrons · Physics 2020-03-30 M. Georgiev , H. Chamati

We propose Symplectic Recurrent Neural Networks (SRNNs) as learning algorithms that capture the dynamics of physical systems from observed trajectories. An SRNN models the Hamiltonian function of the system by a neural network and…

Machine Learning · Computer Science 2020-04-28 Zhengdao Chen , Jianyu Zhang , Martin Arjovsky , Léon Bottou

The rapid growth of research in exploiting machine learning to predict chaotic systems has revived a recent interest in Hamiltonian Neural Networks (HNNs) with physical constraints defined by the Hamilton's equations of motion, which…

Machine Learning · Computer Science 2021-06-02 Chen-Di Han , Bryan Glaz , Mulugeta Haile , Ying-Cheng Lai

Recent advances in the field of strongly correlated electron systems allow to access the entanglement properties of interacting fermionic models, by means of Monte Carlo simulations. We briefly review the techniques used in this context to…

Statistical Mechanics · Physics 2019-04-12 Francesco Parisen Toldin , Fakher F. Assaad

We propose a quantum algorithm for inferring the molecular nuclear spin Hamiltonian from time-resolved measurements of spin-spin correlators, which can be obtained via nuclear magnetic resonance (NMR). We focus on learning the anisotropic…

A dynamics of the precession of coupled atomic moments in the tight-binding (TB) approximation is presented. By implementing an angular penalty functional in the energy that captures the magnetic effective fields self-consistently, the…

Materials Science · Physics 2021-07-07 Ramon Cardias , Cyrille Barreteau , Pascal Thibaudeau , Chu Chun Fu

Machine learning promises to deliver powerful new approaches to neutron scattering from magnetic materials. Large scale simulations provide the means to realise this with approaches including spin-wave, Landau Lifshitz, and Monte Carlo…

Computational Physics · Physics 2020-11-12 Anjana M. Samarakoon , D. Alan Tennant

We consider properties of a two-dimensional electron system in a random magnetic field. It is assumed that the magnetic field not only influences orbital electron motion but also acts on the electron spin. For calculations, we suggest a new…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Kazutaka Takahashi , K. B. Efetov

Artificial Intelligence (AI) has become an exceptionally powerful tool for analyzing scientific data. In particular, attention-based architectures have demonstrated a remarkable capability to capture complex correlations and to furnish…

Strongly Correlated Electrons · Physics 2025-11-03 Changkai Zhang , Jan von Delft

Investigations of molecular magnets are driven both by prospective applications in future storage technology or quantum computing as well as by fundamental questions. Nowadays numerical simulation techniques and computer capabilities make…

Strongly Correlated Electrons · Physics 2009-10-08 J. Schnack

Molecular quantum magnets adsorbed on surfaces exhibit rich spin and orbital excitations that can be probed by scanning tunneling microscopy with inelastic electron tunneling spectroscopy (STM-IETS). However, the quantitative extraction of…

Mesoscale and Nanoscale Physics · Physics 2026-01-28 Greta Lupi , Adolfo O. Fumega , Mohammad Amini , Robert Drost , Peter Liljeroth , Jose L. Lado

Two-dimensional noncollinear magnetic states, such as spin-spiral magnets, offer an excellent platform for investigating fundamental phenomena, with potential for advancing stray-field-free spintronics. However, detection and…

Mesoscale and Nanoscale Physics · Physics 2026-04-06 Fedor Nigmatulin , Greta Lupi , Jose L. Lado , Zhipei Sun

We derive an effective spin Hamiltonian for the one-dimensional half-filled Alternating Hubbard model in the limit of strong on-site repulsion. We show that the effective Hamiltonian is a spin $S=1/2$ Heisenberg chain with asymmetric…

Strongly Correlated Electrons · Physics 2007-05-23 Paata Kakashvili , George I. Japaridze

Quantum materials research requires co-design of theory with experiments and involves demanding simulations and the analysis of vast quantities of data, usually including pattern recognition and clustering. Artificial intelligence is a…

Other Condensed Matter · Physics 2021-11-01 A. M. Samarakoon , D. Alan Tennant , Feng Ye , Qiang Zhang , S. A. Grigera

Simulating the evolution of the gravitational N-body problem becomes extremely computationally expensive as N increases since the problem complexity scales quadratically with the number of bodies. We study the use of Artificial Neural…

Earth and Planetary Astrophysics · Physics 2023-11-01 Veronica Saz Ulibarrena , Philipp Horn , Simon Portegies Zwart , Elena Sellentin , Barry Koren , Maxwell X. Cai

In this article, we use artificial intelligence algorithms to show how to enhance the resolution of the elementary particle track fitting in inhomogeneous dense detectors, such as plastic scintillators. We use deep learning to replace more…

Data Analysis, Statistics and Probability · Physics 2023-06-21 Saúl Alonso-Monsalve , Davide Sgalaberna , Xingyu Zhao , Clark McGrew , André Rubbia

We present a multi-scale computational approach that combines atomistic spin models with the cluster multipole (CMP) method. The CMP method enables a systematic and accurate generation of complex non-collinear magnetic structures using…

Materials Science · Physics 2025-03-06 Juba Bouaziz , Takuya Nomoto , Ryotaro Arita

An extended atomistic spin model allowing for studies of the finite temperature magnetic properties of alloys is proposed. The model is obtained by extending the Heisenberg Hamiltonian via a parameterization from a first principles basis,…

Computational Physics · Physics 2017-06-07 Fan Pan , Jonathan Chico , Anna Delin , Anders Bergman , Lars Bergqvist
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