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Compartmentalizing reagents within small droplets is promising for highly efficient conversion and simplified procedures in many biphasic chemical reactions. In this work, surface nanodroplets (i.e., less than 100 nm in their maximal…
A new method based on the combination of small-anglescattering, reverse Monte Carlo simulations, and an aggregate recognition algorithm is proposed to characterize the structure of nanoparticle suspensions in solvents and polymer…
Effective mixing is essential for biochemical reactions. In droplet-based microfluidics, immediate mixing of substances upon contact in the droplet formation stage can greatly enhance the uniformity of chemical reactions. Furthermore, it…
Hypothesis: Immiscible liquids are commonly used to achieve unique functions in many applications, where the breakup of compound droplets in airflow is an important process. Due to the existence of the liquid-liquid interface, compound…
A systematically designed study has been conducted to understand and clearly demarcate the degree of contribution by the constituting elements to the surface tension of nanocolloids. The effects of elements such as surfactants, particles…
The ordering of nanoparticles into predetermined configurations is of importance to the design of advanced technologies. In this work, we moderate the surface anchoring against the bulk elasticity of liquid crystals to dynamically shape…
This review focuses on a microparticle-producing technique widely used for its efficacy in controlling physicochemical properties: droplet-based microfluidics. The review describes the various strategies applied under this technique, and…
In this work, we investigate crystallization from droplets formed on micro-patterned surfaces. By solvent exchange in a micro-chamber, a ternary solution consisting of a model compound beta-alanine, water, and isopropanol, was displaced by…
Surface structure affects the growth, shape and properties of nanoparticles. In wet chemical syntheses, metal additives and surfactants are used to modify surfaces and guide nanocrystal growth. To understand this process, it is critical to…
Hypothesis: Interfacial instabilities cause undesirable droplet breakage during impact. Such breakage affects many applications, such as printing, spraying, etc. Particle coating over a droplet can significantly change the impact process…
This work describes a new microfluidic device developed for rapid screening of solubility diagrams. In several parallel channels, hundreds of nanoliter-volume droplets of a given solution are first stored with a gradual variation in the…
The behavior of cross-linking polymer solutions as they transition from liquid-like to solid-like material in flow determines success or failure in several applications. Dilute polymer solutions flow easily, while concentrated polymers or…
When a water droplet is deposited within a sparsely miscible liquid medium such as certain oils, the droplet surprisingly vanishes, even in a confined geometry. Such a phenomenon has crucial consequences for multiphase flows in which…
Micro and nanodroplets have many important applications such as in drug delivery, liquid-liquid extraction, nanomaterial synthesis and cosmetics. A commonly used method to generate a large number of micro or nanodroplets in one simple step…
Solvent exchange is a simple method to produce surface nanodroplets on a substrate for a wide range of applications by displacing a solution of good solvent, poor solvent and oil (Solution A) by a poor solvent (Solution B). In this work, we…
(Abbreviated) In this paper we report on the development of a multiscale method for simulating complex liquid-liquid systems such as water in contact with oil containing asphaltenes. We consider simulations where water drops covered with…
Block copolymers often create droplets when placed on a substrate. Such nanostructured droplets can be arranged into regular microstructured arrays, thereby forming hierarchically organized materials that can be used in microelectronics,…
Droplet breakup is important in many natural and industrial processes, but the current classification of breakup regimes, especially the intermediate breakup regime, is ambiguous. In this study, the transitions of breakup regimes for…
We present a new methodology for efficient and high-quality patterning of biological reagents for surface-based biological assays. The method relies on hydrodynamically confined nanoliter volumes of reagents to interact with the substrate…
Cutting onions often leads to tear-inducing aerosol release in kitchen, yet the underlying mechanics of droplet generation remain poorly understood. In this work, we combine custom-developed high-speed particle tracking velocimetry (PTV)…