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We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

We investigate theoretically the strong-field regime of light-matter interactions in the topological-insulator class of quantum materials. In particular, we focus on the process of non-perturbative high-order harmonic generation from the…

Mesoscale and Nanoscale Physics · Physics 2022-01-24 Denitsa Baykusheva , Alexis Chacón , Dasol Kim , Dong Eon Kim , David A. Reis , Shambhu Ghimire

Recently discovered photonic higher-order topological insulators enable unprecedented flexibility in the robust localization of light in structures of different dimensionality. While the potential of the two-dimensional systems is currently…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Valerii I. Kachin , Maxim A. Gorlach

Three-dimensional topological insulators represent a new quantum phase of matter with spin-polarized surface states that are protected from backscattering. The static electronic properties of these surface states have been comprehensively…

Mesoscale and Nanoscale Physics · Physics 2011-12-06 J. W. McIver , D. Hsieh , H. Steinberg , P. Jarillo-Herrero , N. Gedik

High-harmonic generation from solids can be utilized as probe of ultrafast dynamics, but thus far only over extended sample areas, since its spatial resolution is diffraction-limited. Here we propose spatial polarization gating, that is…

We report the observation of second harmonic generation with high conversion efficiency $\sim 0.005\%$ in the terahertz regime from thin films of the topological insulator Bi$_2$Se$_3$ that exhibit the linear photogalvanic effect, measured…

Strongly Correlated Electrons · Physics 2024-06-11 Jonathan Stensberg , Xingyue Han , Zhuoliang Ni , Xiong Yao , Xiaoyu Yuan , Debarghya Mallick , Akshat Gandhi , Seongshik Oh , Liang Wu

Topological insulators in three dimensions are nonmagnetic insulators that possess metallic surface states as a consequence of the nontrivial topology of electronic wavefunctions in the bulk of the material. They are the first known…

Strongly Correlated Electrons · Physics 2012-01-26 M. Zahid Hasan , Joel E. Moore

Topological insulators in the Bi2Se3 family have an energy gap in the bulk and a gapless surface state consisting of a single Dirac cone. Low frequency optical absorption due to the surface state is universally determined by the fine…

Materials Science · Physics 2015-03-17 Xiao Zhang , Jing Wang , Shou-Cheng Zhang

Topological materials are of interest to both fundamental science and advanced technologies, because topological states are robust with respect to perturbations and dissipation. Experimental detection of topological invariants is thus in…

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

We present an experimental evidence of \emph{topological} Hall-effect in an all-optical third-order nonlinear optical process via spatial symmetry-breaking in pseudo-spin textures created by a spatially-structured pump laser beam. The…

Optics · Physics 2025-10-03 Soumik Nandi , Arannya Ghosh , Ashok K Mohapatra , Ritwick Das

Topological insulators display unusual light-matter interactions due to the helical nature of surface electronic states. We study the near-field interaction of light propagating in an optical fiber with crystals of Sb2Te3, a 3D topological…

Materials Science · Physics 2018-10-16 Moti Fridman , Vlada Artel , Anna Peled , Shir Shahal , Ashwin Ramasubramaniam , Doron Naveh

Band topology has been studied as a design principle of realizing robust boundary modes. Here, by exploring non-Hermitian topology, we propose a three-dimensional topological laser that amplifies surface modes. The topological surface laser…

Mesoscale and Nanoscale Physics · Physics 2022-07-27 Kazuki Sone , Yuto Ashida , Takahiro Sagawa

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…

We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

We report high-resolution spin-resolved photoemission spectroscopy (Spin-ARPES) measurements on the parent compound Sb of the first discovered 3D topological insulator Bi{1-x}Sb{x} [D. Hsieh et al., Nature 452, 970 (2008) Submitted 2007].…

Mesoscale and Nanoscale Physics · Physics 2011-03-18 D. Hsieh , Y. Xia , L. Wray , D. Qian , J. H. Dil , F. Meier , L. Patthey , J. Osterwalder , G. Bihlmayer , Y. S. Hor , R. J. Cava , M. Z. Hasan

Topology-driven nonlinear light-matter effects open up new paradigms for both topological photonics and nonlinear optics. Here, we propose to achieve high-efficiency second-harmonic generation in a second-order photonic topological…

Optics · Physics 2021-12-02 Yafeng Chen , Zhihao Lan , Jensen Li , Jie Zhu

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

The recent realization of photonic topological insulators has brought the discovery of fundamentally new states of light and revolutionary applications such as non-reciprocal devices for photonic diodes and robust waveguides for light…

Optics · Physics 2019-08-05 Xiao-Dong Chen , Jian-Wen Dong

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

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