Related papers: What do the two times in two-time correlation func…
The paper describes a time-resolved photoemission (TRPES) apparatus equipped with a Yb-doped fiber laser system delivering 1.2-eV pump and 5.9-eV probe pulses at the repetition rate of 95 MHz. Time and energy resolutions are 11.3 meV and…
The angle-resolved photoemission (ARPES) technique has been developed rapidly over the last decay, accompanied by the improvement of energy and momentum resolutions. This technique has been established as the most powerful tool to…
Time-resolved X-ray Emission/Absorption Spectroscopy (Tr-XES/XAS) is an informative experimental tool sensitive to electronic dynamics in materials, widely exploited in diverse research fields. Typically, Tr-XES/XAS requires X-ray pulses…
Encoding information in the time-frequency domain is demonstrating its potential for quantum information processing. It offers a novel scheme for communications with large alphabets, computing with large quantum systems, and new approaches…
We demonstrate a new technique for characterizing two-photon quantum states based on joint temporal correlation measurements using time resolved single photon detection by femtosecond upconversion. We measure for the first time the joint…
We demonstrate quantum interference of three photons that are distinguishable in time, by resolving them in the conjugate parameter, frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the…
Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…
Angle-resolved photoemission spectroscopy (ARPES) is used to study the doping dependence of the lifetime and the mass renormalization of the low energy excitations in the high-Tc cuprate (Bi,Pb)_2Sr_2CaCu_2O_8 along the zone diagonal. We…
We develop a simulation procedure for angle-resolved photoemission spectroscopy (ARPES), where a photoelectron wave function is set to be an outgoing plane wave in a vacuum associated with the emitted photoelectron wave packet. ARPES…
A theory of correlations between N photons of given frequencies and detected at given time delays is presented. These correlation functions are usually too cumbersome to be computed explicitly. We show that they are obtained exactly through…
Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…
Suppose we measure the time-dependent spectrum of a single photon. That is, we first send the photon through a set of frequency filters (which we assume to have different filter frequencies but the same finite bandwidth $\Gamma$), and then…
We present a sensing scheme for estimating the frequency difference of two non-entangled photons. The technique consists of time-resolving sampling measurements at the output of a beam splitter. With this protocol, the frequency shift…
The bi-photon correlation time, a measure for the conditional uncertainty in the temporal arrival of two photons from a photon pair source, is a key performance identifier for many quantum spectroscopy applications, with shorter correlation…
A common challenge in quantum information processing with photons is the limited ability to manipulate and measure correlated states. An example is the inability to measure picosecond scale temporal correlations of a multi-photon state,…
We report a numerical calculation of the two-photon absorption coefficient of electrons in a binding potential using the real-time real-space higher-order difference method. By introducing random vector averaging for the intermediate state,…
X-ray spectroscopy has been a key method to determine ground and excited state properties of quantum materials with atomic specificity. Now, new x-ray facilities are opening the door to the study of pump-probe x-ray spectroscopy -…
The physics that governs quantum monitoring may involve other degrees of freedom than the ones initialised and controlled for probing. In this context we address the simultaneous estimation of phase and dephasing characterizing a dispersive…
We observed two-photon phase super-resolution in an unbalanced Michelson interferometer with classical Gaussian laser pulses. Our work is a time-reversed version of a two-photon interference experiment using an unbalanced Michelson…
Phase-sensitive pump-probe hyperspectral imaging is a precise technique for absolute two-beam measurements of the optical Kerr coefficient ($n_2$). The irradiance profile is characterized and background effects are rejected by rastering the…