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We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire…

Materials Science · Physics 2025-02-11 Takeshi Suzuki , Yigui Zhong , Kecheng Liu , Teruto Kanai , Jiro Itatani , Kozo Okazaki

The angle-resolved photoemission spectroscopy (ARPES) is one powerful experimental technique to study the electronic structure of materials. As many electron materials show unusual many-body correlations, the technique to detect directly…

Superconductivity · Physics 2020-05-12 Yuehua Su , Chao Zhang

We present angular-resolved correlation measurements between photons after propagation through a three-dimensional disordered medium. The multiple scattering process induces photon correlations that are directly measured for light sources…

Optics · Physics 2011-06-30 Stephan Smolka , Otto L. Muskens , Ad Lagendijk , Peter Lodahl

The pursuit of a comprehensive understanding of the dynamical nature of intertwined orders in quantum matter has fueled the development of several new experimental techniques, including time- and angle-resolved photoemission spectroscopy…

Superconductivity · Physics 2021-07-21 Marta Zonno , Fabio Boschini , Andrea Damascelli

This treatise reviews latest results obtained from angle-resolved photoemission spectroscopy (ARPES) on cuprate superconductors, with a special focus on the electron-phonon interaction. What has emerged is rich information about the…

Strongly Correlated Electrons · Physics 2009-09-29 X. J. Zhou , T. Cuk , T. Devereaux , N. Nagaosa , Z. -X. Shen

Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium…

Strongly Correlated Electrons · Physics 2016-10-04 Christopher L. Smallwood , Robert A. Kaindl , Alessandra Lanzara

Interaction of light with media often occurs with a femtosecond response time. Its measurement by conventional techniques requires the use of femtosecond lasers and sophisticated time-gated optical detection1-3. Here we demonstrate that by…

Two-color side-view probing of light-matter interaction from minute focal volume of a tightly focused fs-laser pump pulse reveals charge dynamics with high 0.9 micrometers optical resolution and approximately ~20 fs temporal resolution in…

A theoretical frame for two-photon photoemission is derived from the general theory of pump-probe photoemission, assuming that not only the probe but also the pump pulse is sufficiently weak. This allows us to use a perturbative approach to…

Mesoscale and Nanoscale Physics · Physics 2016-09-21 J. Braun , R. Rausch , M. Potthoff , H. Ebert

The interaction of light with a material's electronic system creates an out-of-equilibrium (non-thermal) distribution of optically excited electrons. Non-equilibrium dynamics relaxes this distribution on an ultrafast timescale to a hot…

Strongly Correlated Electrons · Physics 2014-03-05 Søren Ulstrup , Jens Christian Johannsen , Marco Grioni , Philip Hofmann

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

Time Resolved Correlation (TRC) is a recently introduced light scattering technique that allows to detect and quantify dynamic heterogeneities. The technique is based on the analysis of the temporal evolution of the speckle pattern…

Soft Condensed Matter · Physics 2007-05-23 Agnes Duri , Hugo Bissig , Veronique Trappe , Luca Cipelletti

Recent angle-resolved photoemission (ARPES) studies of the high Tc superconductors are reviewed. Amongst the topics discussed are: the spectral function interpretation of ARPES data and sum rules; studies of the momentum distribution and…

Superconductivity · Physics 2008-02-03 Mohit Randeria , Juan-Carlos Campuzano

A two-photon emission of a medium with periodically time-dependent refractive index is considered. The emission results from the zero-point fluctuations of the medium. Usually this emission is very weak. However, it can be strongly enhanced…

Quantum Physics · Physics 2007-05-23 V. Hizhnyakov

We describe different approximations associated with employing a constant matrix element for the coupling of light to multiband electrons in the context of time-resolved angle-resolved photoemission spectroscopy (TR-ARPES). In particular,…

Strongly Correlated Electrons · Physics 2016-10-11 J. K. Freericks , H. R. Krishnamurthy

Angle-resolved photoemission spectroscopy (ARPES) is one of the most direct methods of studying the electronic structure of solids. By measuring the kinetic energy and angular distribution of the electrons photoemitted from a sample…

Strongly Correlated Electrons · Physics 2013-03-07 Riccardo Comin , Andrea Damascelli

Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…

We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Jochen Küpper , Robin Santra

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

Causality implies that by measuring an absorption spectrum, the time-dependent linear response function can be retrieved. Recent experiments suggest a link between the shape of spectral lines observed in absorption spectroscopy with the…