Related papers: An Integrated Quantum Material Testbed with Multi-…
We used angle-resolved photoemission spectroscopy (ARPES) and density functional theory calculations to study the electronic structure of Ba(Fe1-x-yCoxMny)2As2 for x=0.06 and 0<=y <=0.07. From ARPES we derive that the substitution of Fe by…
The existence of coherent quasiparticles near the Fermi energy in the low temperature state of high-temperature superconductors has been well established by angle-resolved photoemission spectroscopy (ARPES). This technique directly probes…
Various technical developments extended the potential of angle-resolved photoemission (ARPES) tremendously during the last twenty years. In particular improved momentum, energy and spin resolution as well as the use of photon energies from…
The development of high-performance quantum technologies relies on the ability to prepare the quantum states of solid-state emitters with high fidelity while cleanly separating the emitted photons from the driving field. Here, we present a…
There is an enormous interest in renormalization of quasi-particle (qp) dispersion relation of cuprate superconductors both below and above the critical temperature $T_c$ because it enables determination of the fluctuation spectrum to which…
Structuring light emission from single-photon emitters in multiple degrees of freedom is of a great importance for quantum information processing towards higher dimensions. However, traditional control of emission from quantum light sources…
Angle resolved photoemission spectroscopy (ARPES) has been performed on quasi-one dimensional Li0.9Mo6O17 using photon energy 500 eV. Measured band dispersions are in agreement with those from both low photon energy measurements and band…
We present the development of a time- and angle-resolved photoemission spectroscopy based on a Yb-based femtosecond laser and a hemispherical electron analyzer. The energy of the pump photon is tunable between 1.4 and 1.9 eV, and the pulse…
Ultrafast spectroscopy of molecular systems is fundamentally constrained by the Fourier uncertainty principle: high temporal resolution smears out electronic state signatures, while high spectral resolution obscures dynamic information.…
Optical pumping of solids creates a non-equilibrium electronic structure where electrons and photons combine to form quasiparticles of dressed electronic states. The resulting shift of electronic levels is known as the optical Stark effect,…
The Electron Multiplying Charge Coupled Devices (EMCCD), owing to their high quantum efficiency and spatial resolution, are widely used to study typical quantum optical phenomena and related applications. Researchers have already developed…
Free electrons provide a powerful tool to probe material properties at atomic-scale spatial resolution. Recent advances in ultrafast electron microscopy enable the manipulation of free electron wavefunctions using laser pulses. It would be…
Synchrotron based photoemission electron microscopy with energy filter combines real space imaging with microprobe diffraction ($\mu$-ARPES), giving access to the local electronic structure of laterally inhomogeneous materials. We present…
Explosive increase of interest in quantum computing has resulted in various proposals for generation of quantum bits or qubits, the basic quantum computing unit. The superconducting qubits of Josephson Junction are the most widely accepted…
At Argonne National Laboratory, we are developing hard X-ray (2 to 20 keV) Transition Edge Sensor (TES) arrays for beamline science. The significantly improved energy resolution provided by superconducting detectors compared to…
Squeezed light enables quantum-enhanced phase estimation, with crucial applications in both fundamental physics and emerging technologies. To fully exploit the advantage provided by this approach, estimation protocols must remain optimal…
Strongly correlated topological surface states are promising platforms for next-generation quantum applications, but they remain elusive in real materials. The correlated Kondo insulator SmB$_6$ is one of the most promising candidates, with…
Electronic structure of crystalline materials is their fundamental characteristic which is the basis of almost all their physical and chemical properties. Angle-resolved photoemission spectroscopy (ARPES) is the main experimental tool to…
Recent renewed interest in the mixed valent insulator SmB6 comes from topological theory predictions and surface transport measurements of possible in-gap surface states whose existence is most directly probed by angle-resolved…
Optical quantum computing, as well as quantum communication and sensing technology based on quantum correlations are in preparation. These require photodiodes for the detection of about 10^16 photons per second with close to perfect quantum…