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The development of extreme ultraviolet sources is critical for advancing angleresolved photoemission spectroscopy (ARPES), a powerful technique for probing the electronic structure of materials. Here, we report the construction of a…

Developing a widely tunable vacuum ultraviolet (VUV) source with sub-100 femtoseconds (fs) pulse duration is critical for ultrafast pump-probe techniques such as time- and angle-resolved photoemission spectroscopy (TrARPES). While a tunable…

Mesoscale and Nanoscale Physics · Physics 2023-02-02 Haoyuan Zhong , Changhua Bao , Tianyun Lin , Shaohua Zhou , Shuyun Zhou

We describe different approximations associated with employing a constant matrix element for the coupling of light to multiband electrons in the context of time-resolved angle-resolved photoemission spectroscopy (TR-ARPES). In particular,…

Strongly Correlated Electrons · Physics 2016-10-11 J. K. Freericks , H. R. Krishnamurthy

Angle-resolved photoemission spectroscopy (ARPES) is a powerful probe of electron correlations in two-dimensional layered materials. In this Letter we demonstrate that ARPES can be used to probe the onset of exciton condensation in…

Strongly Correlated Electrons · Physics 2013-02-25 Stefan Rist , A. A. Varlamov , A. H. MacDonald , Rosario Fazio , Marco Polini

Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium…

Strongly Correlated Electrons · Physics 2016-10-04 Christopher L. Smallwood , Robert A. Kaindl , Alessandra Lanzara

The paper describes a time-resolved photoemission (TRPES) apparatus equipped with a Yb-doped fiber laser system delivering 1.2-eV pump and 5.9-eV probe pulses at the repetition rate of 95 MHz. Time and energy resolutions are 11.3 meV and…

Instrumentation and Detectors · Physics 2016-12-13 Y. Ishida , T. Otsu , A. Ozawa , K. Yaji , S. Tani , S. Shin , Y. Kobayashi

A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond…

A synchrotron radiation beamline in the photon energy range of 18 - 240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation…

A notable role in understanding of microscopic electronic properties of high temperature superconductors (HTSC) belongs to angle resolved photoemission spectroscopy (ARPES). This technique supplies a direct window into reciprocal space of…

Superconductivity · Physics 2007-05-23 A. A. Kordyuk , S. V. Borisenko

In this article we review our angle- and time-resolved photoemission studies (ARPES and trARPES) on various ferropnictides.

The spectral energy gap is an important signature that defines states of quantum matter: insulators, density waves, and superconductors have very different gap structures. The momentum resolved nature of angle-resolved photoemission…

Superconductivity · Physics 2015-03-03 Makoto Hashimoto , Inna M. Vishik , Rui-Hua He , Thomas P. Devereaux , Zhi-Xun Shen

We developed a table-top vacuum ultraviolet (VUV) laser with $113.778$nm wavelength (10.897eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond…

Motivated by recent experimental progress we revisit the theory of pump-probe time- and angle-resolved photoemission spectroscopy (trARPES), which is one of the most powerful techniques to trace transient pump-driven modifications of the…

Mesoscale and Nanoscale Physics · Physics 2022-01-14 Michael Schüler , Michael A. Sentef

Angle Resolved Photoemission Spectroscopy (ARPES) probes the momentum-space electronic structure of materials, and provides invaluable information about the high-temperature superconducting cuprates. Likewise, the cuprate real-space,…

Superconductivity · Physics 2009-10-27 I. M. Vishik , B. Moritz , E. A. Nowadnick , W. S. Lee , K. Tanaka , T. Sasagawa , T. Fujii , T. P. Devereaux , Z. X. Shen

Recent improvements to spatial resolution in angle-resolved photo-emission spectroscopy (ARPES) have made it common to perform measurements with a very brief dwell time, for the purpose of mapping the spectral function over large surface…

We present an experimental set-up developed to perform optical spectroscopy experiments (Raman scattering and photoluminescence measurements) with a micrometer spatial resolution, in an extreme environment of low temperature, high magnetic…

We develop a simulation procedure for angle-resolved photoemission spectroscopy (ARPES), where a photoelectron wave function is set to be an outgoing plane wave in a vacuum associated with the emitted photoelectron wave packet. ARPES…

We introduce an efficient first-principles framework for simulating angle-resolved photoemission spectroscopy (ARPES) based on the direct computation of photoelectron states as solutions of the Kohn-Sham equation with scattering boundary…

Materials Science · Physics 2026-02-02 Gian Parusa , Sotirios Fragkos , Samuel Beaulieu , Michael Schüler

The electronic band structure, describing the motion and interactions of electrons in materials, dictates the electrical, optical, and thermodynamic properties of solids. Angle-resolved photoemission spectroscopy (ARPES) provides a direct…

Relevant metrological scenarios involve the simultaneous estimation of multiple parameters. The fundamental ingredient to achieve quantum-enhanced performances is based on the use of appropriately tailored quantum probes. However, reaching…