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For large-scale deployment and use of polymer electrolyte fuel cells, high-performance electrocatalysts with low platinum consumption are desirable. One promising strategy to meet this demand is to explore alternative materials that retain…

Materials Science · Physics 2025-09-01 Kevin Allen , Christopher Lane , Emilia Morosan , Jian-Xin Zhu

The physical properties of La$_4$Ni$_3$O$_{10}$ with a 2D-like Ruddlesden-Popper-type crystal structure are extraordinarily dependent on temperature and chemical substitution. By introducing Al$^{3+}$ atoms ($x$) randomly at the Ni-sites,…

Ferrite nanoparticles serve as potent heterogeneous Fenton-like catalysts, producing reactive oxygen species (ROS) for decomposing organic pollutants. We investigated the impact of temperature and copper content on the catalytic activity of…

We present the results of an ab initio study of magnetic properties of Fe, Co and Ni surfaces. In particular, we discuss their electronic structure and magnetic exchange interactions (Jij), as obtained by means of a combination of density…

Computational Physics · Physics 2015-10-14 S. Keshavarz , Y. O. Kvashnin , I. Di Marco , A. Delin , M. I. Katsnelson , A. I. Lichtenstein , O. Eriksson

We investigated the effects of paramagnetic (PM) fluctuations on the thermochemistry of the MnO(100) surface in the oxygen evolution reaction (OER) using the "noncollinear magnetic sampling method \textit{plus} $U$" (NCMSM$+U$). Various…

Materials Science · Physics 2023-07-19 Sangmoon Yoon , Kyoungsuk Jin , Sangmin Lee , Ki Tae Nam , Miyoung Kim , Young-Kyun Kwon

Photocatalytic water splitting has greatly stimulated as an ideal technique for producing hydrogen (H$_{2}$) fuel by employing two renewable sources, i.e., water and solar energy. Here, we have adopted a facile hydrothermal approach for the…

Chemical Physics · Physics 2022-01-04 Fahmida Sharmin , Dayal Chandra Roy , M. A. Basith

Reducible oxides are widely used catalyst supports that can increase oxidation reaction rates by transferring their lattice oxygen at the metal-support interface. The interfacial oxidation process is typically described in terms of a…

Materials Science · Physics 2021-04-05 Joshua L. Vincent , Peter A. Crozier

The effect of silica-promotion on the reduction of iron oxides in hydrogen was investigated using in situ X-ray diffraction and aberration-corrected transmission electron microscopy to understand the mechanism of reduction and the identity…

Materials Science · Physics 2021-05-13 M. J. Coombes , E. J. Olivier , E. Prestat , S. J. Haigh , E. du Plessis , J. H. Neethling

Using first-principles density functional theory (DFT), we studied the issue of water incorporation in iron bearing wadsleyite (Mg$_2$SiO$_4$)mineral at transition zone pressures and temperature under varying conditions of vacancy…

Geophysics · Physics 2018-12-12 Tilak Das , Swastika Chatterjee , Tanusri Saha-Dasgupta

This paper presents synthesis methods and multifunctional properties of porous Co3O4 nanoplatelets and nanowires. Surprisingly, significantly superior Li-ion battery performance compared to other cathode materials is exhibited in the same…

Materials Science · Physics 2012-07-16 R. Zeng , J. Q. Wang , G. D. Du , W. X. Li , Z. X. Chen , S. Li , Z. P. Guo , S. X. Dou

Recently, the development of efficient and non-noble metal electrocatalysts with excellent durability for the hydrogen evolution reaction (HER) has attracted increasing attention. The exotic and robust metallic surface states of topological…

Chemical Physics · Physics 2019-09-27 Qing Qu , Bin Liu , Jing Liang , Ding Pan , Iam Keong Sou

Using a combination of first principles molecular dynamics simulations (FPMD) and electronic structure calculations, we characterize the atomistic structure and vibrational properties of a photocatalytic surface of In$_2$O$_3$, a promising…

Materials Science · Physics 2025-03-12 Matthew Bousquet , Jiawei Zhan , Chunxin Luo , Alex B. Martinson , Francois Gygi , Giulia Galli

BiVO$_4$ is a promising photocatalyst for efficient water oxidation, with surface reactivity determined by the structure of active catalytic sites. Surface oxidation in the presence of oxygen vacancies induces electron localization,…

Understanding how the local environment of a single-atom catalyst affects stability and reactivity remains a significant challenge. We present an in-depth study of Cu1, Ag1, Au1, Ni1, Pd1, Pt1, Rh1, and Ir1 species on Fe3O4(001); a model…

Layered double-hydroxides (LDHs) are superior to the conventional (Transition Metal Oxides) TMOs as their lamellar morphology accommodates higher active sites contributing to the facile electron transfer towards the material degradation…

We report here on a novel and facile techniques for the synthesis nanocomposite based on stable bimetallic catalyst containing iridium and gold nanoparticles electrodeposited on chemically reduced graphene oxide (rGO) sheet admixed with…

X-ray absorption spectroscopy (XAS) as well as x-ray magnetic circular dichroism (XMCD) and magnetization of hybrid pyrochlore Eu2-xFexTi2O7 were investigated, where the rare earth Eu (4f) was replaced with transition metal Fe (3d) to…

Electrochemical CO2 reduction (CO2R) offers a promising approach to decarbonize chemical manufacturing through production of carbon-neutral fuels. However, insufficient performance and instability of membrane electrode assembly (MEA)…

Five bimetallic electrocatalysts (ECs) including a carbon nitride (CN) support are synthesised through the pyrolysis of a solid precursor obtained through sol-gel and gel-plastic processes. The resulting ECs are characterised through…

Chemical Physics · Physics 2018-05-23 Stefano Diodati , Enrico Negro , Keti Vezzu' Vito Di Noto , Silvia Gross

Hydrogen has emerged as a promising energy source, holding the key to achieve low-carbon and sustainable mobility. However, its applications are still limited by modest conversion efficiency in the electrocatalytic oxygen reduction reaction…