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Symmetry informed diffraction patterns for magnetically ordered MnF2 illuminated by x-rays tuned in energy to a Mn atomic resonance depend on circular polarization in the primary beam. The change in intensity of a Bragg spot with a change…

Strongly Correlated Electrons · Physics 2025-11-19 Stephen W. Lovesey

Heterostructures of PbTiO$_3$/SrTiO$_3$ superlattices have shown the formation of "polar vortices", in which a continuous rotation of ferroelectric polarization spontaneously forms. Recently, Shafer {\it{et al.}} [Proc.\ Natl.\ Acad.\ Sci.\…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Stephen W. Lovesey , Gerrit van der Laan

For the oblique helicoidal structure of the chiral twist-bend nematic-forming mixture of CB7CB/CB6OCB/5CB doped by light-sensitive chiral compound based on azo-fragment, two consequent states of Bragg reflection of the light in the visible…

Soft Condensed Matter · Physics 2024-04-08 H. Bogatyryova , V. Chornous , L. Lisetski , I. Gvozdovskyy

A thorough tensor analysis of the Bragg-forbidden reflection (00.3)$_h$ in corundum systems having a global center of inversion, like V$_2$O$_3$ and $\alpha$-Fe$_2$O$_3$, shows that anomalous x-ray resonant diffraction can access chiral…

Strongly Correlated Electrons · Physics 2007-05-23 S. Di Matteo , Y. Joly , A. Bombardi , L. Paolasini , F. de Bergevin , C. R. Natoli

A theoretical study of Bragg diffraction by an enantiomorphic pair of structures should apply to patterns gathered on beta-Mn using resonance enhanced x-ray diffraction. The chiral polymorph of manganese, and structurally related compounds,…

Materials Science · Physics 2021-04-28 S. W. Lovesey

Possible ways of identification are discussed of an electronic order of higher multipoles such as octupoles and hexadecapoles. A particularly powerful method is resonant X-ray scattering (RXS) using quadrupolar resonance processes called…

Strongly Correlated Electrons · Physics 2009-11-11 Y. Kuramoto , H. Kusunose , A. Kiss

A new chiral phase of ferric ions in bismuth ferrite, the only material known to support multiferroic behaviour at room temperature, is inferred from extensive sets of data gathered by resonant x-ray Bragg diffraction. Values of all ferric…

Magnetic axial and polar (Dirac) nickel multipoles contribute to resonant x-ray Bragg amplitudes in a symmetry informed analysis of monoclinic Li2Ni3P4O14 presented for future diffraction experiments. Magnetic long-range order below a…

Strongly Correlated Electrons · Physics 2025-08-08 Stephen W. Lovesey

The Bragg diffraction of neutrons and x-rays are well-suited to the task of determining the distribution of magnetization in crystals. Applications of the two techniques proceed by contrasting observed intensities with intensities…

Strongly Correlated Electrons · Physics 2022-12-21 Stephen W. Lovesey

A recent experimental study of TbB4 at a low temperature using resonant x-ray Bragg diffraction implies a magnetic symmetry not found in any other rare-earth tetraboride. The evidence for this assertion is a change in the intensity of a…

Strongly Correlated Electrons · Physics 2024-06-26 R. D. Johnson , S. W. Lovesey

Optimally-chiral electromagnetic fields with maximized helicity density, recently introduced in [1], enable chirality characterization of optically small nanoparticles. Here, we demonstrate a technique to obtain optimally-chiral nearfields…

Applied Physics · Physics 2020-12-02 Mina Hanifeh , Mohammad Albooyeh , Filippo Capolino

Collinear and canted magnetic motifs in haematite were investigated by Kokubun et al. (2008) using x-ray Bragg diffraction magnified at the iron K-edge, and analyses of observations led to various potentially interesting conclusions. We…

Materials Science · Physics 2013-06-21 S. W. Lovesey , A. Rodriguez-Fernandez , J. A. Blanco

We use vortex photon fields with orbital and spin angular momentum to probe chiral fluctuations within liquid crystals. In the regime of iridescence with a well-defined pitch length of chirality, we find low energy Raman scattering that can…

Soft Condensed Matter · Physics 2023-08-21 Silvia Müllner , Florian Büscher , Angela Möller , Peter Lemmens

Structured x-rays carrying an orbital angular momentum break spatial inversion symmetry and have been proposed as a means to probe chirality. We theoretically investigate twisted non-resonant x-ray diffraction from chiral molecules and…

Optics · Physics 2026-03-02 Akilesh Venkatesh , Phay J. Ho , Jérémy R. Rouxel

The enantiomorphous (chiral) crystal class of the Sohncke-type insulator Pb(TiO)Cu4(PO4)4 permits the rotation of the plane of polarization of light (optical activity). Copper ions participate in antiferromagnetic order below a temperature…

Strongly Correlated Electrons · Physics 2024-01-17 S. W. Lovesey

Optical chiral properties of a resonant hybrid photonic crystal (RHPC) are computed taking into account spin-orbit effect due to light-hole excitons perfectly confined in 2D quantum wells. The trends of the optical activity, expressed as a…

Mesoscale and Nanoscale Physics · Physics 2023-12-25 A. D'Andrea

In this work we present an alternative way to look at electron diffraction in a transmission electron microscope. In stead of writing the scattering amplitude in Fourier space as a set of plane waves, we use the cylindrical Fourier…

Instrumentation and Detectors · Physics 2015-11-13 Roeland Juchtmans , Jo Verbeeck

The spatiotemporal response of crystals in x-ray Bragg diffraction resulting from excitation by an ultra-short, laterally confined x-ray pulse is studied theoretically. The theory presents an extension of the analysis in symmetric…

Optics · Physics 2012-10-22 Yuri Shvyd'ko , Ryan Lindberg

We study the resonance behaviour of the forbidden 600 and 222 x-ray Bragg peaks in Ge using LDA band structure methods. These Bragg peaks remain forbidden in the resonant dipole scattering approximation even taking into account the non…

Strongly Correlated Electrons · Physics 2009-11-07 I. S. Elfimov , N. A. Skorikov , V. I. Anisimov , G. A. Sawatzky

Free-electron laser hard X-ray light sources can provide high fluence, femtosecond pulses, enabling the time-resolved probing of structural dynamics and elementary relaxation processes in molecules. Traditional X-ray elastic scattering from…

Chemical Physics · Physics 2016-11-23 Kochise Bennett , Markus Kowalewski , Shaul Mukamel
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