Related papers: Broadband complementary vibrational spectroscopy w…
A virtual vibrational spectrometer, based on efficient software exploring unrestricted Hartree-Fock approximation, has been proposed to perform computational spectroscopy of radicals. The computational device allows obtaining spectra of IR…
A combined approach that uses the vibrational self-consistent field (VSCF) and vibrational configuration interaction (VCI) method together with the semiclassical instanton theory was developed to study vibrational tunneling spectra of…
We introduce a new cascaded four-wave mixing technique which scales up the bandwidth of frequency combs generated by phase modulation of a continuous wave laser while simultaneously enhancing the spectral flatness. As a result we…
Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…
Cavity ring-down (CRD) spectroscopy represents a direct absorption technique of sample absorption measurement. Instead of measuring the amount of the absorbed light, this technique determines the rate at which light intensity decays inside…
We present a novel approach to realize microresonator-comb-based high resolution spectroscopy that combines a fiber-laser cavity with a microresonator. Although the spectral resolution of a chip-based comb source is typically limited by the…
Spectral imaging and detection of mid-infrared (mid-IR) wavelengths are emerging as an enabling technology of great technical and scientific interest; primarily because important chemical compounds display unique and strong mid-IR spectral…
A novel characterization method to measure the pulse duration of ultrafast near-IR pulses is introduced, which uses simple tabletop optics, is relatively inexpensive, and is expected to work in a broad wavelength range. Our diagnostic tool…
Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…
Raman spectroscopy is an appealing technique that probes molecular vibrations in a wide variety of materials with virtually no sample preparation. However, accurate and reliable Raman measurements are still a challenge and require more…
We demonstrate the implementation of a fiber-integrated spectrograph utilizing chromatic group velocity dispersion (GVD) in a single mode fiber. By means of GVD we stretch an ultrafast pulse in time in order to spectrally resolve single…
The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…
Vibrational sum frequency generation (SFG) spectroscopy is a powerful technique for investigating molecular structures, orientations, and dynamics at surfaces. However, its spatial resolution is fundamentally restricted to the micrometer…
Miniaturized spectrometers employing chip solutions are essential for a wide range of applications, such as wearable health monitoring, biochemical sensing, and portable optical coherence tomography. However, the development of integrated…
Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne…
We evaluate the spectral performance of a novel continuous-wave room-temperature distributed feedback quantum cascade laser operating at the long wavelength of 17 $\mu$m. By demonstrating broadband laser absorption spectroscopy of the…
Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…
Diffuse correlation spectroscopy (DCS) is a powerful tool for assessing microvascular hemodynamic in deep tissues. Recent advances in sensors, lasers, and deep learning have further boosted the development of new DCS methods. However,…
Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…
The measurement of the isotopic composition of cosmic rays (CRs) provides essential insights the understanding of the origin and propagation of these particles, namely the CR source spectra, the propagation processes and the galactic halo…