Related papers: Visualizing coherent molecular rotation in a gaseo…
We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…
A general method for rotational microwave spectroscopy and control of polar molecular ions via direct microwave addressing is considered. Our method makes use of spatially varying AC Stark shifts, induced by far off-resonant, focused laser…
We investigate beam pointing dynamics in filamentation in gases driven by high repetition rate femtosecond laser pulses. Upon suddenly exposing a gas to a kilohertz train of filamenting pulses, the filament is steered from its original…
A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…
Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…
We have investigated the angle-resolved ATI spectrum of oriented molecules in the IR+XUV co-rotating circular laser fields. According to the different roles of IR and XUV laser in the ionization process, we purposefully adjust the photon…
The performance of organic optoelectronic devices is critically dependent on how molecules orient within organic thin films. Yet, standard characterization techniques only reveal the first and second moments of the molecular orientation…
We consider the propagation of slow light with an orbital angular momentum (OAM) in a moving atomic medium. We have derived a general equation of motion and applied it in analysing propagation of slow light with an OAM in a rotating medium,…
Ultracold polar molecules are an ideal platform for studying many-body physics with long-range dipolar interactions. Experiments in this field have progressed enormously, and several groups are pursuing advanced apparatus for manipulation…
We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…
We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…
Properly polarized and correctly timed femtosecond laser pulses have been demonstrated to create rotational states with a preferred sense of rotation. We show that due to conservation of angular momentum, collisional relaxation of these…
We show that a 450 fs nonresonant, moderately intense, linearly polarized laser pulse can induce field-free molecular axis alignment of methyliodide molecules dissolved in a helium nanodroplet. Time-resolved measurements reveal rotational…
Since its invention in 1999, optical centrifuge has become a powerful tool for controlling molecular rotation and studying molecular dynamics and molecular properties at extreme levels of rotational excitation. The technique has been…
Understanding the quantum dynamics of strongly coupled molecule-cavity systems remains a significant challenge in molecular polaritonics. This work develops a comprehensive self-consistent model simulating electromagnetic interactions of…
Coherent control of chaotic molecular systems, using laser-assisted alignment of sulphur dioxide (SO$_2$) molecules in the presence of a static electric field as an example, is considered. Conditions for which the classical version of this…
The alternative to dynamic alignment explanation of experimental results on spatial-asymmetric dissociation of molecules in a laser field is proposed. The concept of geometrical alignment is sufficient for explanation of these results. In…
In recent years it became possible to align molecules in free space using ultrashort laser pulses. Here we explore two schemes for controlling molecule-surface scattering process, which are based on the laser-induced molecular alignment. In…
CS$_2$ is identified as a molecule for which distinction can be made between dynamic and geometric alignment induced by intense laser fields. Measured anisotropic angular distributions of fragment ions arise from (i) dynamic alignment of…
We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…