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Genetic algorithms, as implemented in optimal control strategies, are currently successfully exploited in a wide range of problems in molecular physics. In this context, laser control of molecular alignment and orientation remains a very…

Chemical Physics · Physics 2007-05-23 O. Atabek , C. M. Dion

A new class of cost functionals for optimal control of quantum systems which produces controls which are sparse in frequency and smooth in time is proposed. This is achieved by penalizing a suitable time-frequency representation of the…

Optimization and Control · Mathematics 2016-07-15 Gero Friesecke , Felix Henneke , Karl Kunisch

The paper aims at the development of an apparatus for analysis and construction of near optimal solutions of singularly perturbed (SP) optimal controls problems (that is, problems of optimal control of SP systems) considered on the infinite…

Optimization and Control · Mathematics 2014-08-20 Vladimir Gaitsgory , Sergei Rossomakhine

A generic formulation for the optimal control of a single wave-energy converter (WEC) is proposed. The formulation involves hard and soft constraints on the motion of the WEC to promote reduced damage and fatigue to the device during…

Optimization and Control · Mathematics 2020-12-16 Mertcan Yetkin , Sudharsan Kalidoss , Frank E. Curtis , Lawrence V. Snyder , Arindam Banerjee

Fastness and robustness are both critical in the implementation of high-fidelity gates for quantum computation, but in practice, a trade-off has to be made between them. In this paper, we investigate the underlying robust time-optimal…

Quantum Physics · Physics 2023-09-12 Xi Cao , Jiangyu Cui , Man Hong Yung , Re-Bing Wu

We present some approaches to the computation of ultra-fast laser pulses capable of selectively breaking molecular bonds. The calculations are based on a mixed quantum-classical description: The electrons are treated quantum mechanically…

Atomic and Molecular Clusters · Physics 2015-05-27 Kevin Krieger , Alberto Castro , E. K. U. Gross

Lasers are becoming a more and more important tool in cutting and shaping materials. Improving precision and effectivity is an ongoing demand in science and industry. One possibility are double pulses. Here we study laser ablation of…

Materials Science · Physics 2015-06-19 Johannes Roth , Armin Krauß , Jan Lotze , Hans-Rainer Trebin

In this paper we consider an optimal control problem governed by a time-dependent variational inequality arising in quasistatic plasticity with linear kinematic hardening. We address certain continuity properties of the forward operator,…

Optimization and Control · Mathematics 2012-09-06 Gerd Wachsmuth

Controlling molecular reactivity by shaped laser pulses is a long-standing goal in chemistry. Here we suggest a direct optimal control approach which combines external pulse optimization with other control parameters arising in the upcoming…

Quantum Physics · Physics 2024-01-03 A. R. Ramos Ramos , E. W. Fischer , P. Saalfrank , O. Kühn

Optical techniques for spatiotemporal control can produce laser pulses with custom amplitude, phase, or polarization structure. In nonlinear optics and plasma physics, the use of structured pulses typically follows a forward design…

On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…

Quantum Physics · Physics 2024-09-05 Reon Ishii , Tomotaro Namba , Hiroyuki Katsuki , Kenji Ohmori , Yukiyoshi Ohtsuki

Highly polarized, multi-kiloampere-current electron bunches from compact laser-plasma accelerators are desired for numerous applications. Current proposals to produce these beams suffer from intrinsic limitations to the reproducibility,…

Accelerator Physics · Physics 2023-10-05 Simon Bohlen , Zheng Gong , Michael J. Quin , Matteo Tamburini , Kristjan Põder

We consider the optimal control problem of minimizing some quadratic functional over all possible solutions of an internally controlled multi-dimensional heat equation with a periodic terminal state constraint. This problem has a unique…

Optimization and Control · Mathematics 2015-09-22 Emmanuel Trélat , Lijuan Wang , Yubiao Zhang

Method-of-lines discretizations are demanding test problems for stiff integration methods. However, for PDE problems with known analytic solution the presence of space discretization errors or the need to use codes to compute reference…

Numerical Analysis · Mathematics 2023-05-24 Jens Lang , Bernhard A. Schmitt

This paper is concerned with an optimal control problem subject to the $H^1$-critical defocusing semilinear wave equation on a smooth and bounded domain in three spatial dimensions. Due to the criticality of the nonlinearity in the wave…

Optimization and Control · Mathematics 2019-07-08 Karl Kunisch , Hannes Meinlschmidt

The control of quantum dynamics via specially tailored laser pulses is a long-standing goal in physics and chemistry. Partly, this dream has come true, as sophisticated pulse shaping experiments allow to coherently control product ratios of…

Quantum Physics · Physics 2007-07-16 J. Werschnik , E. K. U. Gross

Coherent control of a system involves steering an interaction to a final coherent state by controlling the phase of an applied field. Plasmas support coherent wave structures that can be generated by intense laser fields. Here, we…

Plasma Physics · Physics 2015-06-02 Z. -H. He , B. Hou , V. Lebailly , J. A. Nees , K. Krushelnick , A. G. R. Thomas

In this work, we present numerical analysis for a distributed optimal control problem, with box constraint on the control, governed by a subdiffusion equation which involves a fractional derivative of order $\alpha\in(0,1)$ in time. The…

Numerical Analysis · Mathematics 2017-12-22 Bangti Jin , Buyang Li , Zhi Zhou

We present and study novel optimal control problems motivated by the search for photovoltaic materials with high power-conversion efficiency. The material must perform the first step: convert light (photons) into electronic excitations. We…

Optimization and Control · Mathematics 2018-08-14 Gero Friesecke , Michael Kniely

We consider control-constrained linear-quadratic optimal control problems on evolving surfaces. In order to formulate well-posed problems, we prove existence and uniqueness of weak solutions for the state equation, in the sense of…

Optimization and Control · Mathematics 2015-03-19 Morten Vierling