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We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…
We investigate the nonlinear interaction between two photons in a single input pulse at an atomic two level nonlinearity. A one dimensional model for the propagation of light to and from the atom is used to describe the precise…
Photons are natural carriers of quantum information due to their ease of distribution and long lifetime. This thesis concerns various related aspects of quantum information processing with single photons. Firstly, we demonstrate N-photon…
We analyze the time-dependent interaction between a two-level atom and a spectrally encoded single-photon wave packet using the Heisenberg-Langevin equations and derive the atomic excitation probability. Spectral phase encoding broadens the…
The control and manipulation of quantum-entangled non-local states is a crucial step for the development of quantum information processing. A promising route to achieve such states on a wide scale is to couple solid-state quantum emitters…
Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…
Quantum technologies hold great promise for revolutionizing photonic applications such as cryptography. Yet their implementation in real-world scenarios is held back, mostly due to sensitivity of quantum light to scattering. Recent…
Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon…
A quantum system composed of two or more subsystems can be in an entangled state, i.e. a state in which the properties of the global system are well defined but the properties of each subsystem are not. Entanglement is at the heart of…
We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…
Entangled photon pairs form the foundation for many applications in the realm of quantum communication. For fiber-optic transfer of entangled photon pairs, time-bin encoding can potentially offer an improved stability compared to…
Quantum imaging enhances imaging systems performance, potentially surpassing fundamental limits such as noise and resolution. However, these schemes have limitations and are still a long way from replacing classical techniques. Therefore,…
The state of a two-particle system is called entangled when its quantum mechanical wave function cannot be factorized in two single-particle wave functions. Entanglement leads to the strongest counter-intuitive feature of quantum mechanics,…
Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of…
We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…
Pairs of entangled vortex photons can promise new prospects of application in quantum computing and cryptography. We investigate the possibility of generating such states via two-level atom emission induced by a single photon wave packet…
We propose an extension of coherent control using laser-synthesized free-electron matter waves. In contrast to coherent control schemes exploiting optical coherences to steer the dynamics of matter waves, we analyze the opposite and…
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…
The problem of the two-photon coherent generation of entanglement photon pairs in Quantum Optics has been intensively studied for the last years. It is important to note that the two-quantum cooperative effects play a main role in other…
We construct an entangled photon polarimeter capable of monitoring a two-qubit quantum state in real time. Using this polarimeter, we record a nine frames-per-second video of a two-photon state's transition from separability to…