Related papers: Control of reactive collisions by quantum interfer…
Quantum mechanical scattering resonances for colliding particles occur when a continuum scattering state couples to a discrete bound state between them. The coupling also causes the bound state to interact with itself via the continuum and…
We report the creation of ultracold bosonic $^{23}$Na$^{87}$Rb Feshbach molecules via magneto-association. By ramping the magnetic field across an interspecies Feshbach resonance, at least 4000 molecules can be produced out of the near…
Scattering resonances are fundamental in science, spanning energy scales from stellar nuclear fusion to ultracold collisions. In ultracold quantum gases, magnetic Feshbach resonances have transformed quantum many-body research by enabling…
We propose a general method for optical control of magnetic Feshbach resonances in ultracold atomic gases with more than one molecular state in an energetically closed channel. Using two optical frequencies to couple two states in the…
Nuclear spin exchange occurs in ultracold collisions of fermionic alkaline-earth-like atoms due to a difference between s- and p-wave phase shifts. We study the use of an optical Feshbach resonance, excited on the ${}^1S_0 \to {}^3P_1$…
We present a theory for rigorous quantum scattering calculations of probabilities for chemical reactions of atoms with diatomic molecules in the presence of an external electric field. The approach is based on the fully uncoupled basis set…
Ultracold molecules offer remarkable opportunities to study chemical reactions at nearly zero temperature. Although significant progresses have been achieved in exploring ultracold bimolecular reactions, the investigations are usually…
We report the observation of a broad magnetic Feshbach resonance with a large background scattering length in an ultracold fermionic mixture of $^{23}$Na$^{40}$K molecules and $^{40}$K atoms, with both species prepared in their lowest…
Cross sections resulting from scattering that proceeds via an intermediate resonance are shown to be exceptionally controllable using a coherent superposition of only two intial states. Full quantum computations on F+HD(v=0;j=0,1) --> H+DF,…
We observe magnetically tuned collision resonances for ultracold Cs2 molecules stored in a CO2-laser trap. By magnetically levitating the molecules against gravity, we precisely measure their magnetic moment. We find an avoided level…
We report the investigation on dipolar collisions in rotational state mixtures of ultracold bosonic $^{23}$Na$^{87}$Rb molecules. The large resonant dipole-dipole interaction between molecules in rotational states of opposite parities…
Scattering resonances are an essential tool for controlling interactions of ultracold atoms and molecules. However, conventional Feshbach scattering resonances, which have been extensively studied in various platforms, are not expected to…
It is demonstrated that elastic collisions of ultracold atoms forming a heteronuclear collision complex can be manipulated by laboratory practicable dc electric fields. The mechanism of electric field control is based on the interaction of…
Fundamental entanglement related challenges have prevented quantum interference-based control (i.e. coherent control) of collisional cross sections from being implemented in the laboratory. Here, differential cross sections for reactive…
We develop a theoretical method for solving the quantum mechanical reactive scattering problem in the presence of external fields based on a hyperspherical coordinate description of the reaction complex combined with the total angular…
Controlling physical systems and their dynamics on the level of individual quanta propels both fundamental science and quantum technologies. Trapped atomic and molecular systems, neutral and charged, are at the forefront of quantum science.…
Advances in atomic physics have led to the possibility of a coherent transformation between ultra-cold atoms and molecules including between completely bosonic condensates. Such transformations are enabled by the magneto-association of…
Gaining control over chemical reactions on the quantum level is a central goal of the modern field of cold and ultracold chemistry. Here, we demonstrate a novel method to coherently steer reaction flux of a three-body recombination process…
We have carried out bound-state and low-energy quantum scattering calculations on He + NH (triplet Sigma) in magnetic fields, with the NH molecule in its n=1 rotationally excited states. We have explored the pattern of levels as a function…
Quantum control of reactive systems has enabled microscopic probes of underlying interaction potentials, the opening of novel reaction pathways, and the alteration of reaction rates using quantum statistics. However, extending such control…