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The formation of methanol (CH3OH) on icy grain mantles during the star formation cycle is mainly associated with the CO freeze-out stage. Yet there are reasons to believe that CH3OH also can form at an earlier period of interstellar ice…

Astrophysics of Galaxies · Physics 2018-05-02 D. Qasim , K. -J. Chuang , G. Fedoseev , S. Ioppolo , A. C. A. Boogert , H. Linnartz

SH$^+$ is a surprisingly widespread molecular ion in diffuse interstellar clouds. There, it plays an important role triggering the sulfur chemistry. In addition, SH$^+$ emission lines have been detected at the UV-illuminated edges of dense…

A continuous supersonic flow reactor has been used to measure rate constants for the C + NH3 reaction over the temperature range 50 to 296 K. C atoms were created by the pulsed laser photolysis of CBr4. The kinetics of the title reaction…

New insights into the formation of interstellar formamide, a species of great relevance in prebiotic chemistry, are provided by electronic structure and kinetic calculations for the reaction NH2 + H2CO -> NH2CHO + H. Contrarily to what…

Astrophysics of Galaxies · Physics 2015-08-19 V. Barone , C. Latouche , D. Skouteris , F. Vazart , N. Balucani , C. Ceccarelli , B. Lefloch

We simulate the multi-phase interstellar medium randomly heated and stirred by supernovae, with gravity, differential rotation and other parameters of the solar neighbourhood. Here we describe in detail both numerical and physical aspects…

Astrophysics of Galaxies · Physics 2013-04-03 F. A. Gent , A. Shukurov , A. Fletcher , G. R. Sarson , M. J. Mantere

We present far-IR (57-196 mu) spectra of 21 protostars in the Orion molecular clouds, obtained with the Photodetector Array Camera and Spectrometer (PACS) onboard the Herschel Space observatory, as part of the Herschel Orion Protostar…

To understand the chemistry of sulphur (S) in the interstellar medium, models need to be tested by observations of S-bearing molecules in different physical conditions. We analyse observations obtained with the IRAM 30m telescope towards 15…

Astrophysics of Galaxies · Physics 2023-10-17 F. Fontani , E. Roueff , L. Colzi , P. Caselli

The reaction N(4S) + NO -> O(3P) + N2 plays a pivotal role in the conversion of atomic to molecular nitrogen in dense interstellar clouds and in the atmosphere. Here we report a joint experimental and computational investigation of the N +…

Astrophysics of Galaxies · Physics 2023-05-10 Kevin M. Hickson , Juan Carlos San Vicente Veliz , Debasish Koner , Markus Meuwly

The chemical network governing interstellar sulfur has been the topic of unrelenting discussion for the past decades due to the conspicuous discrepancy between its expected and observed abundances in different interstellar environments.…

Astrophysics of Galaxies · Physics 2024-07-16 Julia C. Santos , Joan Enrique-Romero , Thanja Lamberts , Harold Linnartz , Ko-Ju Chuang

We report the first full-dimensional potential energy surface (PES) and quantum mechanical close-coupling calculations for scattering of SiO due to H$_2$. The full-dimensional interaction potential surface was computed using the explicitly…

A detailed interpretation of the detected emission lines of environments in which propyne (or methyl acetylene, CH$_3$CCH) is observed requires a knowledge of its collisional rate coefficients with the most abundant species in the…

Astrophysics of Galaxies · Physics 2024-02-28 M. Ben Khalifa , B. Darna , J. Loreau

We present and validate a new network of atmospheric thermo-chemical and photo-chemical sulfur reactions. We use a 1-D chemical kinetics model to investigate these reactions as part of a broader HCNO chemical network in a series of hot and…

Earth and Planetary Astrophysics · Physics 2021-07-07 Richard Hobbs , Paul Rimmer , Oliver Shorttle , Nikku Madhusudhan

Observations of CO+ suggest column densities on the order 10^12 cm^-2 that can not be reproduced by many chemical models. CO+ is more likely to be destroyed than excited in collisions with hydrogen. An anomalous excitation mechanism may…

Solar and Stellar Astrophysics · Physics 2015-05-13 Pascal Staeuber , Simon Bruderer

In light of its ubiquitous presence in the interstellar gas, the chemistry and reactivity of the HCO+ ion requires special attention. The availability of up-to-date collisional data between this ion and the most abundant perturbing species…

Astrophysics of Galaxies · Physics 2022-01-13 F. Tonolo , L. Bizzocchi , M. Melosso , F. Lique , L. Dore , V. Barone , C. Puzzarini

Hydride molecules lie at the base of interstellar chemistry, but the synthesis of sulfuretted hydrides is poorly understood. Motivated by new observations of the Orion Bar PDR - 1'' resolution ALMA images of SH+; IRAM 30m detections of H2S,…

Astrophysics of Galaxies · Physics 2021-03-03 J. R. Goicoechea , A. Aguado , S. Cuadrado , O. Roncero , J. Pety , E. Bron , A. Fuente , D. Riquelme , E. Chapillon , C. Herrera , C. A. Duran

Theoretical models predict the condensation of silicon carbide around host stars with C/O ratios higher than 0.65 (cf. C/O$_{\mathrm{Sun}}$ = 0.54), in addition to its observations in meteorites, interstellar medium and protoplanetary…

Earth and Planetary Astrophysics · Physics 2018-10-24 Kaustubh Hakim , Wim van Westrenen , Carsten Dominik

Hydrogen sulfide (H$_2$S) is thought to be efficiently formed on grain surfaces through the successive hydrogenation of S atoms. Its non-detection so far in astronomical observations of icy dust mantles thus indicates that effective…

Astrophysics of Galaxies · Physics 2023-08-17 Julia C. Santos , Harold Linnartz , Ko-Ju Chuang

C$^+$ is a critical constituent of many regions of the interstellar medium, as it can be a major reservoir of carbon and, under a wide range of conditions, the dominant gas coolant. Emission from its 158$\mu$m fine structure line is used to…

Astrophysics of Galaxies · Physics 2019-08-19 Laurent Wiesenfeld , Paul F. Goldsmith

The modelling of emission spectra of molecules seen in interstellar clouds requires the knowledge of collisional rate coefficients. Among the commonly observed species, N$_2$H$^+$ is of particular interest since it was shown to be a good…

Astrophysics of Galaxies · Physics 2015-06-23 François Lique , Fabien Daniel , Laurent Pagani , Nicole Feautrier

MoAlB as a typical member of the MAB phases has attracted much growing attention due to its unique properties. However, the low production of MoAlB powders limits its further development and potential applications. To respond this…

Materials Science · Physics 2022-06-28 Hang Yin , Xiaodong He , Guangping Song , Yongdong Yu , Yongting Zheng , Yuelei Bai